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We consider ultralong-range polyatomic Rydberg molecules formed by combining a Rydberg cesium atom and a ground-state RbCs molecule. We explore the regime where the charge-dipole interaction due to the Rydberg electron with the diatomic…

We proposed utilizing a medium with a high optical depth (OD) and a Rydberg state of low principal quantum number, $n$, to create a weakly-interacting many-body system of Rydberg polaritons, based on the effect of electromagnetically…

We probe resonant dipolar interactions between ultracold $^{40}$K$^{87}$Rb molecules and Rydberg $^{87}$Rb atoms in an optically trapped ensemble. Through state-selective ionization detection of the KRb molecules, we observe resonant energy…

Atomic Physics · Physics 2025-04-10 Lingbang Zhu , Jeshurun Luke , Roy Shaham , Yi-Xiang Liu , Kang-Kuen Ni

Sufficiently high densities in Bose-Einstein condensates provide favorable conditions for the production of ultralong-range polyatomic molecules consisting of one Rydberg atom and a number of neutral ground state atoms. The chemical binding…

Atomic Physics · Physics 2017-05-10 Matthew T Eiles , Jesus Perez-Rios , F Robicheaux , Chris H Greene

Coupling photons to Rydberg excitations in a cold atomic gas yields unprecedentedly large optical nonlinearities at the level of individual light quanta, where the formation of nearby dark-state polaritons is blocked by the strong…

Quantum Physics · Physics 2017-07-19 Callum R. Murray , Thomas Pohl

We explore the electronic structure of ultralong-range pentaatomic Rydberg molecules from a merger of a Rydberg atom and two ground state heteronuclear diatomic molecules. Our focus is on the interaction of Rb($23s$) and Rb($n=20$, $l\ge…

We propose a new approach to excite ion-pair states of ultracold dimers. The central idea is a two-step process where first long-range Rydberg molecules are formed by photoassociation, which are then driven by stimulated emission towards…

Atomic Physics · Physics 2020-02-25 Michael Peper , Johannes Deiglmayr

We investigate the interaction of weak light fields with two-dimensional lattices of atoms, in which two-photon coupling establishes conditions of electromagnetically induced transparency and excites high lying atomic Rydberg states. This…

Quantum Physics · Physics 2022-03-30 Lida Zhang , Valentin Walther , Klaus Mølmer , Thomas Pohl

We describe the emergence of strong spatial correlations, akin to liquid-like behavior and crystallization effects, in low (one and two) dimensional gases of cold Rydberg atoms. The presence of an external electric field permanently…

We investigate the propagation of a single photon under conditions of electromagnetically induced transparency in two parallel one-dimensional atomic clouds which are coupled via Rydberg dipole-dipole interaction. Initially the system is…

Quantum Physics · Physics 2015-03-06 Daniel Viscor , Weibin Li , Igor Lesanovsky

We predict the existence of a class of ultracold giant molecules formed from trapped ultracold Rydberg atoms and polar molecules. The interaction which leads to the formation of such molecules is the anisotropic charge-dipole interaction…

Atomic Physics · Physics 2015-05-18 Seth T. Rittenhouse , H. R. Sadeghpour

We present a combined experimental and theoretical study of the effects of Rydberg interactions on Autler-Townes spectra of ultracold gases of atomic strontium. Realizing two-photon Rydberg excitation via a long-lived triplet state allows…

We analyze the fidelity of a deterministic quantum phase gate for two photons counterpropagating as polaritons through a cloud of Rydberg atoms under the condition of electromagnetically induced transparency (EIT). We provide analytical…

Quantum Gases · Physics 2020-04-22 Przemyslaw Bienias , Hans Peter Buechler

The formation of ultralong-range Rydberg molecules is a result of the attractive interaction between Rydberg electron and polarizable ground state atom in an ultracold gas. In the nondegenerate case the backaction of the polarizable atom on…

Atomic Physics · Physics 2015-07-10 A. Gaj , A. T. Krupp , P. Ilzhöfer , R. Löw , S. Hofferberth , T. Pfau

We study the influence of a lossless material medium on the coherent storage and quantum state transfer of a quantized probe light in an ensemble of $\Lambda $-type atoms. The medium is modeled as uniformly distributed two-level atoms with…

Quantum Physics · Physics 2009-11-13 Liang He , Yu-xi Liu , S. Yi , C. P. Sun , Franco Nori

We investigate the interaction between non-classical light with a tunable multiphoton component and a highly nonlinear medium based on cold Rydberg atoms. The non-classical field emitted by a DLCZ quantum memory is stored using Rydberg…

We study the possibility to use interaction between a polar molecule in the ground electronic and vibrational state and a Rydberg atom to construct two-qubit gates between molecular qubits and to coherently control molecular states. A polar…

Quantum Physics · Physics 2017-09-13 Elena Kuznetsova , Seth T. Rittenhouse , Hossein R. Sadeghpour , Susanne F. Yelin

A fascinating aspect of Rydberg atoms is their ability to form huge but very weakly bound molecules with a ground state atom, only held together by a scattering process between the latter and the Rydberg electron. Beyond the usual way of…

Atomic Physics · Physics 2012-07-31 Andrej Junginger , Jörg Main , Günter Wunner

Ultracold systems offer an unprecedented level of control of interactions between atoms. An important challenge is to achieve a similar level of control of the interactions between photons. Towards this goal, we propose a realization of a…

Quantum information processing with neutral atoms relies on Rydberg excitation for entanglement generation. While the use of heavy divalent or open-shell elements, such as strontium or ytterbium, has benefits due to their optically active…