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Related papers: {H$_2^+$, HeH and H$_2$}: approximating potential …

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Basics of the Born-Oppenheimer (B-O) approximation are reviewed. Assuming the domain of applicability of B-O approximation is limited to 4 significant digits (s.d.) in energy spectrum, where mass, relativistic and QED corrections do NOT…

Atomic Physics · Physics 2025-04-10 Horacio Olivares-Pilon , Alexander V Turbiner

Matching for a wavefunction the WKB expansion at large distances and Taylor expansion at small distances leads to a compact, few-parametric uniform approximation found in {\it J. Phys. B44, 101002 (2011)}. The ten low-lying eigenstates of…

Quantum Physics · Physics 2019-08-13 Horacio Olivares-Pilón , Alexander V. Turbiner

An analytical representation for the potential energy curve for the ground state $X^1\Sigma^+$ of the hydrogen fluoride molecule (HF) is presented in the frame of the Born-Oppenheimer approximation. The analytical expression for the…

Chemical Physics · Physics 2021-10-29 Laura E. Angeles Gantes , Horacio Olivares-Pilón

Following the first principles the elements of the analytic theory of potential curves for diatomic molecules (diatomics) are presented. It is based on matching the perturbation theory at small internuclear distances $R$ and multipole…

Atomic Physics · Physics 2022-07-14 Alexander V. Turbiner , Horacio Olivares-Pilón

This work presents the bound-state spectra of Morse oscillator, which remains one of the oldest important model potentials for molecules. Accurate ro-vibrational energies are obtained by means of a generalized pseudospectral method that…

Quantum Physics · Physics 2013-07-19 Amlan K. Roy

The experimentally-observed non-trivial electronic structure of the Cr$_2$ dimer has made the calculation of its potential energy curve a theoretical challenge in the last decades. By matching the perturbation theory at small internuclear…

Chemical Physics · Physics 2024-08-27 Horacio Olivares-Pilón , Daniel Aguilar-Díaz , Alexander V. Turbiner

The analytic Born-Oppenheimer (B-O) potential curve for the ground state $X^1\Sigma^+$ of the molecule (H,D,T)Cl is constructed for the whole range of internuclear distances $R \in [0,\infty)$ with an accuracy of 3-5 figures in comparison…

Chemical Physics · Physics 2023-08-15 Horacio Olivares-Pilón , Alexander V. Turbiner

We calculate accurate potential energy curves for a ground-state He$^+$ ion interacting with a He atom in the lowest-energy metastable $^3\!S$ electronic state. We employ the full configuration interaction method, equivalent to exact…

Atomic Physics · Physics 2023-11-30 Jacek Gȩbala , Michał Przybytek , Marcin Gronowski , Michał Tomza

A potential energy curve (PEC) accurate to a fraction of 1 ppm ($1:10^6$) is computed for the $^3\Sigma_\mathrm{u}^+$ state of He$_2$ endowed with relativistic and QED corrections. The nuclear Schr\"odinger equation is solved on this PEC…

Chemical Physics · Physics 2026-02-25 Ádám Margócsy , Balázs Rácsai , Péter Jeszenszki , Edit Mátyus

We present high-precision non-relativistic variational calculations of bound vibrational-rotational state energies for the $H_2^+$ and $D_2^+$ molecular ions in each of the lowest electronic states of $\Sigma_g$, $\Sigma_u$, and $\Pi_u$…

Atomic Physics · Physics 2007-05-23 J. M. Taylor , Zong-Chao Yan , A. Dalgarno , J. F. Babb

Potential energy surfaces of the hydrogen molecular ion H$_2^+$ in the Born-Oppenheimer approximation are computed by means of the Riccati-Pad\'e method (RPM). The convergence properties of the method are analyzed for different states. The…

Chemical Physics · Physics 2022-10-25 Francisco Marcelo Fernández , Javier Garcia

We demonstrate high accuracy calculations for the HeH$^+$ molecule using newly developed analytic formulas for two-center two-electron integrals with exponential functions. The Born-Oppenheimer potential for the ground electronic…

Chemical Physics · Physics 2015-06-04 Krzysztof Pachucki

The main motivation for this work is the exploration of rotational-vibrational states corresponding to electronic excitations in a pre-Born-Oppenheimer quantum theory of molecules. These states are often embedded in the continuum of the…

Chemical Physics · Physics 2018-10-15 Edit Mátyus

Bound-state spectra of shifted Deng-Fan oscillator potential are studied by means of a generalized pseudospectral method. Very accurate results are obtained for \emph{both low as well as high} states by a non-uniform optimal discretization…

Chemical Physics · Physics 2014-09-09 Amlan K. Roy

We present an ab initio study of the HeH$^+$ molecule. Using the quantum chemistry package MOLPRO and a large adapted basis set, we have calculated the adiabatic potential energy curves of the first 20 $^1 \Sigma^+$, 19 $^3\Sigma^+$, 12…

Atomic Physics · Physics 2015-05-14 J. Loreau , J. Lievin , P. Palmeri , P. Quinet , N. Vaeck

We report on accurate variational calculations of the Born-Oppenheimer potential for excited states of the hydrogen molecule with $\Pi$, $\Delta$, and $\Phi$ symmetries. The obtained potential energy curves reach the relative precision of…

Atomic Physics · Physics 2023-01-11 Michał Siłkowski , Krzysztof Pachucki

Accurate low and high-lying bound states of Tietz-Hua oscillator potential are presented. The radial Schr\"odinger equation is solved efficiently by means of the generalized pseudospectral method that enables optimal spatial discretization.…

Chemical Physics · Physics 2014-09-10 Amlan K. Roy

In this work, we use the Born-Oppenheimer approximation where the potential between atoms can be approximated as a function of distance between the two nuclei to study the four-quark bound states. By the approximation, Heitler and London…

High Energy Physics - Phenomenology · Physics 2015-09-02 Xue-Wen Liu , Hong-Wei Ke , Yi-Bing Ding , Xue-Qian Li

The non-relativistic three-body Schr\"odinger equation of the heteronuclear molecular ion HD$^+$ is solved in perimetric coordinates using the Lagrange-mesh method. Energies and wave functions of the four lowest vibrational bound or…

Atomic and Molecular Clusters · Physics 2015-06-16 Horacio Olivares Pilón , Daniel Baye

The Born-Oppenheimer potential for the $^1\Sigma_g^+$ state of H$_2$ is obtained in the range of 0.1 -- 20 au, using analytic formulas and recursion relations for two-center two-electron integrals with exponential functions. For small…

Chemical Physics · Physics 2015-05-19 Krzysztof Pachucki
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