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An exact expression of the bridge-mediated donor-acceptor effective coupling, is derived. For systems represented by a tight-binding Hamiltonian with nearest-neighbor interactions, we show that the effective coupling, is equal to the…

Soft Condensed Matter · Physics 2007-05-23 D. J. Bicout , F. Varchon , E. Kats

Electron transfer (ET) across molecular chains including an impurity is studied based on a recently improved real-time path integral Monte Carlo (PIMC) approach [J. Chem. Phys. {\bf 121}, 12696 (2004)]. The reduced electronic dynamics is…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Lothar Muehlbacher , Joachim Ankerhold

We investigate electron transfer processes in donor-acceptor systems with a coupling of the electronic degrees of freedom to a common bosonic bath. The model allows to study many-particle effects and the influence of the local Coulomb…

Strongly Correlated Electrons · Physics 2007-05-23 Sabine Tornow , Ning-Hua Tong , Ralf Bulla

Sequential tunneling model is used to study electron transport in molecular rectifiers based on structures of donor-bridge-acceptor type. The device is made of two metallic electrodes connected by a molecule, which contains acceptor and…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Kamil Walczak

A minimal model for coherent transport through a donor/acceptor molecular junction is presented. The two donor and acceptor sites are described by single levels energetically separated by an intramolecular tunnel barrier. In the limit of…

Disordered Systems and Neural Networks · Physics 2009-11-11 Florian Pump , Gianaurelio Cuniberti

We propose an analytical method for understanding the problem of multi-channel electron transfer reaction in solution, modeled by a particle undergoing diffusive motion under the influence of one donor and several acceptor potentials. The…

Quantum Physics · Physics 2015-06-30 Aniruddha Chakraborty

For the first time we calculate the electron transmission phase through a quantum point contact (QPC). The QPC is considered in the saddle point approximation in the single-electron picture. We show that when the electron energy is close to…

Mesoscale and Nanoscale Physics · Physics 2014-10-29 Bryce G. C. Lackenby , Oleg P. Sushkov

We examine the effects of electron-electron interactions on transport between edge states in a multilayer integer quantum Hall system. The edge states of such a system, coupled by interlayer tunneling, form a two-dimensional, chiral metal…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 J. W. Tomlinson , J. -S. Caux , J. T. Chalker

The microscopic theory of chemical reactions is based on transition state theory, where atoms or ions transfer classically over an energy barrier, as electrons maintain their ground state. Electron transfer is fundamentally different and…

The thermoelectric transport through a molecular bridge is discussed, with an emphasis on the effects of inelastic processes of the transport electrons caused by the coupling to the vibrational modes of the molecule. In particular it is…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 O. Entin-Wohlman , Y. Imry , A. Aharony

Tunneling of electrons through the barriers in heterostructures has been studied, within unified transfer matrix approach. The effect of barrier width on the transmission coefficient of the electrons has been investigated for different…

Mesoscale and Nanoscale Physics · Physics 2010-02-10 Jatindranath Gain , Madhumita Das Sarkar , Sudakshina Kundu

The conductance of a molecular junction is commonly determined by either charge-transfer-doping, where alignment of the Fermi energy to the molecular levels is achieved, or tunnelling through the tails of molecular resonances within the…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 R. Gutierrez , G. Fagas , K. Richter , F. Grossmann , R. Schmidt

The effects of different contact geometries, bond dimerization, and gate voltage on quantum transport through a C$_{60}$ molecule are studied by the Landauer-B\"{u}ttiker formula based on the Green's function technique. It is shown that the…

Mesoscale and Nanoscale Physics · Physics 2008-08-12 Alireza Saffarzadeh

We investigate heavy-ion multinucleon transfer reactions using the coupled-channels formalism. We first use the semi-classical approximation and show that a direct coupling between the entrance and the pair transfer channels improves a fit…

Nuclear Theory · Physics 2015-11-25 Guillaume Scamps , Kouichi Hagino

The effect of a thermal environment on electron (or hole) transfer through molecular bridges and on the electron conduction properties of such bridges is studied. Our steady state formalism based on an extension of the Redfield theory (D.…

Condensed Matter · Physics 2009-11-07 Dvira Segal , Abraham Nitzan

We investigate time-dependent electron transfer (ET) in benchmark donor-bridge-acceptor systems. For the small bridge sizes studied, we obtain results far different from the perturbation theory which underlies scattering-based approaches,…

Mesoscale and Nanoscale Physics · Physics 2016-09-23 D. Psiachos

We study the energy-transfer rate for electrons in a double-quantum-well structure, where the layers are coupled through screened Coulomb interactions. The energy-transfer rate between the layers (similar to the Coulomb drag effect in which…

Condensed Matter · Physics 2009-11-07 R. T. Senger , B. Tanatar

We propose an analytical model based on diffusion-reaction equation approach for electrochemical electron transfer reaction, where the rate is limited by the electron transfer process. The electron transfer from an ion in solution to the…

Other Condensed Matter · Physics 2015-05-29 Aniruddha Chakraborty

In all theoretical treatments of electron transport through single molecules between two metal electrodes, a clear distinction has to be made between a coherent transport regime with a strong coupling throughout the junction and a Coulomb…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Robert Stadler , Jerome Cornil , Victor Geskin

Outer sphere electron transfer rates can be calculated from simulation data by sampling the equilibrium statistics of the canonical reaction coordinate -- the vertical energy gap. For these calculations, electron transfer is typically…

Chemical Physics · Physics 2025-09-23 Yoonjae Park , Adam P. Willard