Related papers: Nonlinear response theory for Markov processes II:…
The nonlinear response of molecular systems undergoing Markovian stochastic reorientations is calculated up to fifth order in the amplitude of the external field. Time-dependent perturbation theory is used to compute the relevant response…
The theory of nonlinear response for Markov processes obeying a master equation is formulated in terms of time-dependent perturbation theory for the Green's functions and general expressions for the response functions up to third order in…
The four-time correlation function of a general dynamical variable obeying Gaussian statistics is calculated for the trap model with a Gaussian density of states. It is argued that for energy-independent variables this function is…
The nonlinear response to an oscillating field is calculated for a kinetic trap model with an exponential density of states and the results are compared to those for the model with a Gaussian density of states. The calculations are limited…
The dielectric response of non-interacting dipoles is discussed in the framework of the classical model of stochastic reorientations in an asymmetric double well potential (ADWP). In the nonlinear regime, this model exhibits some…
The linear and nonlinear dynamical susceptibilities of a two level system are calculated as it undergoes a transition to a decoherent state. Analogously to the Glover-Tinkham-Ferrell sum rule of superconductivity, spectral weight in the…
The nonlinear oscillator model is useful to basically understand the most important properties of nonlinear optical processes. It has been shown to give the correct asymptotic behaviour and to provide the general feature of harmonic…
The linear response is investigated in a long-range Hamiltonian system from the view point of dynamics, which is described by the Vlasov equation in the limit of large population. Due to existence of the Casimir invariants of the Vlasov…
A nonlinear response theory is provided by use of the transient linearization method in the spatially one-dimensional Vlasov systems. The theory inclusively gives responses to external fields and to perturbations for initial stationary…
Nonlinear absorption in four and five energy level systems have been studied with the aid of steady-state rate equation approach. We report on the tunability of saturable and reverse saturable absorption as a function of spectroscopic…
We study the second order response functions of a colloidal particle being subjected to an anharmonic potential. Contrary to typical response measurements which require an external perturbation, here we experimentally confirm a recently…
This work presents the Second-Order Sensitivity Analysis Methodology (2nd-ASAM) for nonlinear systems. This methodology yields exactly and efficiently the second-order functional derivatives of system responses (associated with physical,…
Nonlinear response occurs naturally when a strong perturbation takes a system far from equilibrium. Despite of its omnipresence in nanoscale systems, it is difficult to predict in a general and efficient way. Here we introduce a way to…
We derive the exact beyond-linear fluctuation dissipation relation, connecting the response of a generic observable to the appropriate correlation functions, for Markov systems. The relation, which takes a similar form for systems governed…
While linear response theory, manifested by the fluctuation dissipation theorem, can be applied at any level of coarse graining, nonlinear response theory is fundamentally of microscopic nature. For perturbations of equilibrium systems, we…
Using non-linear response theory the time signals relevant for nonresonant spectral hole burning are calculated. The step-reponse function following the application of a high amplitude ac field (pump) and an intermediate waiting period is…
We argue that for generic systems close to a critical point, an extended Fluctuation-Dissipation relation connects the low frequency non-linear (cubic) susceptibility to the four-point correlation function. In glassy systems, the latter…
We present a model to probe metamagnetic properties in systems with an arbitrary number of interacting spins. Thermodynamic properties such as the magnetization per particle $m(B,T,N)$, linear susceptibility $\chi_1(T)$, nonlinear…
Linear Response theory aims to predict how added forcing alters the statistical properties of an unforced system. These kinds of questions have been studied predominantly for autonomous dynamical systems, yet many systems in the physical,…
We investigate response to an external magnetic field in the Hamiltonian mean-field model, which is a paradigmatic toy model of a ferromagnetic body and consists of plane rotators like the XY spins. Due to long-range interactions, the…