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The phenomenon of Quantum Tunneling of Mesoscopic Spins is reviewed in the light of the behavior of the archetype of these systems: the molecular complex Mn12-ac. Most observations can be understood in the framework of the reduced Hilbert…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 B. Barbara , I. Chiorescu , R. Giraud , A. G. M. Jansen , A. Caneschi

We report a quasi-one-dimensional S = 1 spin chain compound BaNiTe2O7. This magnetic system has been investigated by magnetic susceptibility, specific heat, and neutron powder diffraction. These results indicate that BaNiTe2O7 develops a…

We investigated the nature of the spin glass-like phase transition in the geometrically frustrated pyrochlore lattices Y$_{2}$Mo$_{2}$O$_{7}$ using the local probes nuclear and muon magnetic resonances, and the field-dependent long range…

Strongly Correlated Electrons · Physics 2010-09-24 Oren Ofer , Amit Keren , Jason S. Gardner , Yang Ren , W. A. MacFarlane

The magnetism of double perovskites is a complex phenomenon, determined from intra- or interatomic magnetic moment interactions, and strongly influenced by geometry. We take advantage of the complementary length and time scales of the muon…

Effects of the Zn- and Ni-substitution on the Cu-spin dynamics in the electron-doped Pr0.86LaCe0.14Cu1-y(Zn,Ni)yO4+a-d with y = 0, 0.01, 0.02, 0.05 and different values of the reduced oxygen content d have been studied using zero-field…

Superconductivity · Physics 2009-11-11 Risdiana , T. Adachi , Y. Koike , I. Watanabe

We report positive muon spin relaxation measurements on the triangular lattice magnetic system FeGa2S4. A magnetic transition not previously detected by specific heat and magnetic susceptibility measurements is found in zero field at T^*…

Strongly Correlated Electrons · Physics 2012-04-25 P. Dalmas de Reotier , A. Yaouanc , D. E. MacLaughlin , Songrui Zhao , T. Higo , S. Nakatsuji , Y. Nambu , C. Marin , G. Lapertot , A. Amato , C. Baines

Using Raman scattering spectroscopy, we uncover a complex magnetic behavior of Nd$_2$Ir$_2$O$_7$ , which stands out among magnetic pyrochlores by the lowest temperature of the all-in-all-out (AIAO) Ir moments ordering…

We report on the spin structure of the pyrochlore iridate Nd$_2$Ir$_2$O$_7$ that could be directly determined by means of powder neutron diffraction. Our magnetic structure refinement unravels a so-called all-in/all-out magnetic structure…

Strongly Correlated Electrons · Physics 2016-10-14 H. Guo , C. Ritter , A. C. Komarek

The ferromagnetic (FM) nature of Nd2Fe14B has been investigated with muon spin rotation and relaxation ({\mu}^+SR) measurements on an aligned, sintered plate-shaped sample. A clear muon spin precession frequency (f_{FM}) corresponding to…

We present a model which accounts for the high field magnetisation at very low temperature in two pyrochlore frustrated systems, Er2Ti2O7 and Tb2Ti2O7. The two compounds present very different ground states: Er2Ti2O7, which has a planar…

Strongly Correlated Electrons · Physics 2015-06-15 Pierre Bonville , Sylvain Petit , Isabelle Mirebeau , Julien Robert , Elsa Lhotel , Carley Paulsen

Rare-earth pyrochlores are known to exhibit exotic magnetic phenomena. We report a study of crystal growth and characterizations of a new rare-earth compound Er$_2$AlSbO$_7$, in which Al$^{3+}$ and Sb$^{5+}$ ions share the same positions…

We have investigated the spin dynamics in the bilayered perovskite Sr3Ru2O7 as a function of magnetic field and temperature using 17O-NMR. This system sits close to a metamagnetic quantum critical point (MMQCP) for the field perpendicular…

Strongly Correlated Electrons · Physics 2007-05-23 Kentaro Kitagawa , Kenji Ishida , Robin S. Perry , Takashi Tayama , Toshiro Sakakibara , Yoshiteru Maeno

The macroscopic magnetizations of a RuSr2(Eu0.7Ce0.3)2Cu2O10+d sample were investigated. A ferromagnet-like transition occurs around T_M in the low-field magnetization. Highly nonlinear M(H), non-Curie-Weiss susceptibility, and slow…

Superconductivity · Physics 2009-11-07 Y. Y. Xue , B. Lorenz , D. H. Cao , C. W. Chu

Electron spin resonance study of frustrated pyrochlore Gd2Ti2O7 is performed in a wide frequency band for a temperature range 0.4-30 K, which covers paramagnetic and magnetically ordered phases. The paramagnetic resonance reveals the…

Strongly Correlated Electrons · Physics 2012-02-02 S. S. Sosin , A. I. Smirnov , L. A. Prozorova , G. Balakrishnan , M. E. Zhitomirsky

A detailed zero and transverse field (ZF&TF) muon spin rotation (muSR) investigation of magnetism and the magneto-electric coupling in Cu2OSeO3 is reported. An internal magnetic field B_int(T=0) = 85.37(25) mT was found, in agreement with a…

Strongly Correlated Electrons · Physics 2015-05-28 A. Maisuradze , Z. Guguchia , B. Graneli , H. M. Ronnow , H. Berger , H. Keller

We report low-temperature muon spin relaxation/rotation (muSR) measurements on single crystals of the actinide superconductor UTe2. Below 5 K we observe a continuous slowing down of magnetic fluctuations that persists through the…

Neutron diffraction studies have been carried out on a single crystal of oxygen-deficient perovskite TbBaCo2O5.5 in the temperature range of 7-370 K. There have been observed several magnetic or structural transitions. Among these, the…

Strongly Correlated Electrons · Physics 2009-11-10 Minoru Soda , Yukio Yasui , Toshiaki Fujita , Takeshi Miyashita , Masatoshi Sato , Kazuhisa Kakurai

A detailed investigation of Ba$_2$MnGe$_2$O$_7$ was performed in its low-temperature magnetoelectric state combining neutron diffraction with magnetization measurements on single crystals. In the paramagnetic state at 10 K, polarized…

Strongly Correlated Electrons · Physics 2023-03-07 A. Sazonov , H. Thoma , R. Dutta , M. Meven , A. Gukasov , R. Fittipaldi , V. Granata , T. Masuda , B. Náfrádi , V. Hutanu

A prominent character of two-dimensional magnetic systems is the enhanced spin fluctuations, which however reduce the ordering temperature. Here we report that a magnetic field of only one-thousandth of the Heisenberg superexchange…

Double hydroxide perovskites with magnetic transition-metal ions were recently identified as a unique class of materials that combine magnetic frustration with correlated proton disorder-a prerequisite for quantum-disordered fluctuating…