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We suggest a new method of studying coherence in finite level systems coupled to the environment and use it for the Hamiltonian that has been used to describe the light-harvesting pigment-protein complex. The method works with the adiabatic…

Quantum Physics · Physics 2013-06-07 Pallavi Bhattacharyya , K. L. Sebastian

Two-dimensional (2D) fluorescence-excitation (2D-FLEX) spectroscopy is a recently proposed nonlinear femtosecond technique for the detection of photoinduced dynamics. The method records a time-resolved fluorescence signal in its excitation-…

Chemical Physics · Physics 2024-06-24 Sebastian V. Pios , Maxim F. Gelin , Luis Vasquez , Jürgen Hauer , Lipeng Chen

Density functional theory is a successful branch of numerical simulations of quantum systems. While the foundations are rigorously defined, the universal functional must be approximated resulting in a `semi'-ab initio approach. The search…

Quantum Physics · Physics 2017-11-22 James Daniel Whitfield , Norbert Schuch , Frank Verstraete

We derive and showcase a novel approach to approximating Fourier transforms in higher dimensions, focusing specifically on the case of 2D radially concentrated ('ring-like') functions. We first reduce the problem to that of evaluating the…

High Energy Astrophysical Phenomena · Physics 2026-04-08 Filip Niewiński , Michael D. Johnson

The fluctuation exchange (FLEX) approximation is applied to study the Holstein-Hubbard model. Due to the retarded nature of the phonon-mediated electron-electron interaction, neither fast Fourier transform (FFT) nor previously developed NRG…

Strongly Correlated Electrons · Physics 2009-10-31 C. -H. Pao , H. -B. Schuttler

We present theoretical and experimental results showing the effects of incoherent population mixing on two-dimensional (2D) coherent excitation spectra that are measured via a time-integrated population and phase-sensitive detection. The…

Exact and asymptotic lineshape expressions are derived from the semi-classical density matrix representation describing a set of closed three-level atomic or molecular states including decoherences, relaxation rates and light-shifts. An…

Atomic Physics · Physics 2012-11-22 Thomas Zanon , Emeric de Clercq , Ennio Arimondo

Attosecond nonlinear Fourier transform (NFT) pump probe spectroscopy is an experimental technique which allows investigation of the electronic excitation, ionization, and unimolecular dissociation processes. The NFT spectroscopy utilizes…

Chemical Physics · Physics 2021-02-11 Sergy Grebenshchikov , Sergio Carbajo

We present a methodology for simulating multi-dimensional electronic spectra of molecular aggregates with coupling of electronic excitation to a structured environment using the stochastic non-Markovian quantum state diffusion (NMQSD)…

Quantum Physics · Physics 2022-09-28 Lipeng Chen , Doran I. G. Bennett , Alexander Eisfeld

This paper presents an analytical formula that closely approximates the fully nonlinear power spectrum of matter fluctuations for redshift $z\approx 5$ to 0 over a wide range of cosmologically interesting flat models with varying matter…

Astrophysics · Physics 2009-10-30 Chung-Pei Ma

This paper introduces a generalised 3rd-order Spectral Representation Method for the simulation of multi-dimensional stochastic fields with asymmetric non-linearities. The simulated random fields satisfy a prescribed Power Spectrum and…

Statistics Theory · Mathematics 2020-07-06 Lohit Vandanapu , Michael D. Shields

We mainly concerned with a decoupled fractional Laplacian wave equation in this paper. A new time-space domain radial basis function (RBF) collocation method is introduced to solve the fractional wave equation, which describes seismic wave…

Computational Physics · Physics 2018-06-07 Yiran Xu , Jingye Li , Guofei Pang , Zhikai Wang , Xiaohong Chen , Benfeng Wang

We develop a density matrix formalism to describe coupled electron-nuclear dynamics. To this end we introduce an effective Hamiltonian formalism that describes electronic transitions and small (quantum) nuclear fluctuations along a…

Chemical Physics · Physics 2020-09-07 Eugene Stolyarov , Alexander White , Dmitry Mozyrsky

The quasi-2D electrostatic systems, characterized by periodicity in two dimensions with a free third dimension, have garnered significant interest in many fields. We apply the sum-of-Gaussians (SOG) approximation to the Laplace kernel,…

Numerical Analysis · Mathematics 2024-12-09 Xuanzhao Gao , Shidong Jiang , Jiuyang Liang , Zhenli Xu , Qi Zhou

We introduce a new computational approach for femtosecond pulse propagation in the transparency region of gases that permits full resolution in three space dimensions plus time while fully incorporating quantum coherent effects such as…

Optics · Physics 2012-07-02 M. Kolesik , E. M. Wright , J. Andreasen , J. M. Brown , D. R. Carlson , R. J. Jones

Developing an analytical theory for atomic coherence driven by ultrashort laster pulses has proved to be challenging due to the breakdown of the rotating wave approximation (RWA). In this paper, we present an approximate, closed-form…

Quantum Physics · Physics 2021-11-30 Nazar Pyvovar , Bing Zeng , Lingze Duan

In this work, we developed analytic asymptotic methods for computing the Fourier modes of gravitational waves from post-Newtonian binary systems in the quasi-Keplerian parametrization in the high eccentricity regime. We have also derived…

General Relativity and Quantum Cosmology · Physics 2026-04-29 Xiaolin Liu , Zhoujian Cao

We propose an analytical procedure to fully solve a two-level system coupled to phonons. Instead of using the common formulation in terms of linear and quadratic system-phonon couplings, we introduce different phonons depending on the…

Quantum Physics · Physics 2019-01-10 Aurélia Chenu , Shiue-Yuan Shiau , Monique Combescot

We demonstrate a method that merges the quantum filter diagonalization (QFD) approach for hybrid quantum/classical solution of the time-independent electronic Schr\"odinger equation with a low-rank double factorization (DF) approach for the…

Quantum Physics · Physics 2022-03-21 Jeffrey Cohn , Mario Motta , Robert M. Parrish

A fully analytical approximation for the observable characteristics of many-electron atoms is developed via a complete and orthonormal hydrogen-like basis with a single-effective charge parameter for all electrons of a given atom. The basis…

Quantum Physics · Physics 2017-12-06 O. D. Skoromnik , I. D. Feranchuk , A. U. Leonau , C. H. Keitel