English
Related papers

Related papers: Dissociation rates from single-molecule pulling ex…

200 papers

We treat the noise-activated escape from a one-dimensional potential well of an overdamped particle, to which a periodic force of fixed frequency is applied. We determine the boundary layer behavior, and the physically relevant length…

Statistical Mechanics · Physics 2007-05-23 Robert S. Maier , D. L. Stein

We study the influence of the velocity dependence of friction on the escape of a Brownian particle from the deep potential well ($E_{b} \gg k_{B}T$, $E_{b}$ is the barrier height, $k_{B}$ is the Boltzmann constant, $T$ is the bath…

Statistical Mechanics · Physics 2009-11-13 M. F. Gelin , D. S. Kosov

Active matter and driven systems exhibit statistical fluctuations in density and particle positions, providing an indirect indicator of dissipation across multiple length and time scales. Here, we quantitatively relate these measurable…

Statistical Mechanics · Physics 2024-12-19 Aishani Ghosal , Jason R. Green

We investigate the Kramers escape from a potential well of a test particle driven by fractional Gaussian noise with Hurst exponent 0<H<1. From a numerical analysis we demonstrate the exponential distribution of escape times from the well…

The dynamics of active particles is of interest at many levels and is the focus of theoretical and experimental research. There have been many attempts to describe the dynamics of particles affected by random active forces in terms of an…

Statistical Mechanics · Physics 2020-01-08 Dan Wexler , Nir S. Gov , Kim Ø. Rasmussen , Golan Bel

There has been an increasing interest in the quantification of nearly deterministic work extraction from a finite number of copies of microscopic particles in finite time. This paradigm, so called single-shot epsilon-deterministic work…

Quantum Physics · Physics 2017-11-22 Sina Salek , Karoline Wiesner

In this report I discuss fluctuation theorems and transient violations of the second law of thermodynamics in small systems. Special emphasis is placed on free-energy recovery methods in the framework of non-equilibrium single-molecule…

Statistical Mechanics · Physics 2015-06-24 F. Ritort

The escape rate of a Brownian particle over a potential barrier is accurately described by the Kramers theory. A quantitative theory explicitly taking the activity of Brownian particles into account has been lacking due to the inherently…

Soft Condensed Matter · Physics 2017-02-01 A. Sharma , R. Wittmann , J. M. Brader

We formulate a predictive theory at the level of forces of activated relaxation in hard sphere fluids and thermal liquids that covers in a unified manner the apparent Arrhenius, crossover and deeply supercooled regimes. The alpha relaxation…

Soft Condensed Matter · Physics 2013-10-23 Stephen Mirigian , Kenneth S. Schweizer

When a Brownian particle, initially being in the potential well, overcomes the barrier and moves to the absorptive border, it still has a chance to be scattered back to the well by thermal fluctuations. We study this phenomenon carefully…

Nuclear Theory · Physics 2018-03-21 Maria Chushnyakova , Igor Gontchar

The Kramers turnover problem, that is obtaining a uniform expression for the rate of escape of a particle over a barrier for any value of the external friction was solved in the eighties. Two formulations were given, one by Melnikov and…

Chemical Physics · Physics 2015-06-15 Eli Pollak , Joachim Ankerhold

There has been great interest in applying the results of statistical mechanics to single molecule experiements. Recent work has highlighted so-called non-equilibrium work-energy relations and Fluctuation Theorems which take on an…

Soft Condensed Matter · Physics 2015-06-25 R. Dean Astumian

Information on dissipation in the entrance channel of heavy-ion collisions is extracted by macroscopic reduction procedure of Time-Dependent Hartree-Fock theory. The method gives access to a fully microscopic description of the friction…

Nuclear Theory · Physics 2009-03-04 Kouhei Washiyama , Denis Lacroix , Sakir Ayik

We study the dynamics of one-dimensional active particles confined in a double-well potential, focusing on the escape properties of the system, such as the mean escape time from a well. We first consider a single-particle both in near and…

Statistical Mechanics · Physics 2022-03-15 Lorenzo Caprini , Fabio Cecconi , Umberto Marini Bettolo Marconi

The reactive process of barrier escaping from the metastable potential well is studied together with the extension of Kramers' rate formula to the fractional case. Characteristic quantities are computed for an thimbleful of insight into the…

Chemical Physics · Physics 2015-02-24 Chun-Yang Wang

We generalize the force-level Nonlinear Langevin Equation theory of single particle hopping to include collective effects associated with long range elastic distortion of the liquid. The activated alpha relaxation event is of a mixed…

Disordered Systems and Neural Networks · Physics 2015-06-18 Stephen Mirigian , Kenneth S. Schweizer

We consider the motion of a particle in a force field subjected to adiabatic, fluctuations of external origin. We do not put the restriction on the type of stochastic process that the noise is Gaussian. Based on a method developed earlier…

Statistical Mechanics · Physics 2007-05-23 Suman Kumar Banik , Jyotipratim Ray Chaudhuri , Deb Shankar Ray

Many processes in chemistry, physics, and biology depend on thermally activated events in which the system changes its state by surmounting an activation barrier. Examples range from chemical reactions, protein folding, and nucleation…

Chemical Physics · Physics 2023-04-26 Pierpaolo Pravatto , Barbara Fresch , Giorgio J. Moro

We explore the dependence of the thermally activated barrier crossing rate on various model parameters for a dimer that undergoes a Brownian motion on a piecewise linear bistable potential employing the method of adiabatic elimination of…

Statistical Mechanics · Physics 2014-07-15 Mesfin Asfaw

We follow the dynamics of an ensemble of interacting self-propelled semi-flexible polymers in contact with a thermal bath. We characterize structure and dynamics of the passive system and as a function of the motor activity. We find that…

Soft Condensed Matter · Physics 2014-04-14 Davide Loi , Stefano Mossa , Leticia F. Cugliandolo