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This article is an introduction to a new approach to first principles electronic structure calculation. The starting point is the Hartree-Fock-Roothaan equation, in which molecular integrals are approximated by polynomials by way of Taylor…

Computational Physics · Physics 2019-07-18 Akihito Kikuchi

We examine the relative performance of algorithms for the calculation of curvature in spacetime. The classical coordinate component method is compared to two distinct versions of the Newman-Penrose tetrad approach for a variety of…

General Relativity and Quantum Cosmology · Physics 2009-10-28 Denis Pollney , Peter Musgrave , Kevin Santosuosso , Kayll Lake

Linear-scaling electronic structure methods based on the calculation of moments of the underlying electronic Hamiltonian offer a computationally efficient and numerically robust scheme to drive large-scale atomistic simulations, in which…

Materials Science · Physics 2017-01-09 Eunan J. McEniry , Ralf Drautz

Quantum computers hold promise to improve the efficiency of quantum simulations of materials and to enable the investigation of systems and properties more complex than tractable at present on classical architectures. Here, we discuss…

Quantum Physics · Physics 2022-05-03 Christian Vorwerk , Nan Sheng , Marco Govoni , Benchen Huang , Giulia Galli

Evaluating multi-center molecular integrals with Cartesian Gaussian-type basis sets has been a long-standing bottleneck in electronic structure theory calculation for solids and molecules. We have developed a vector-coupling and…

Quantum Physics · Physics 2024-05-17 Hang Hu , Gilles Peslherbe , Hsu Kiang Ooi , Anguang Hu

We present an approach to solid-state electronic-structure calculations based on the finite-element method. In this method, the basis functions are strictly local, piecewise polynomials. Because the basis is composed of polynomials, the…

Condensed Matter · Physics 2009-10-31 J. E. Pask , B. M. Klein , C. Y. Fong , P. A. Sterne

In this paper, we propose and analyze some practical Newton methods for electronic structure calculations. We show the convergence and the local quadratic convergence rate for the Newton method when the Newton search directions are…

Optimization and Control · Mathematics 2020-01-28 Xiaoying Dai , Liwei Zhang , Aihui Zhou

This paper discusses the error and cost aspects of ill-posed integral equations when given discrete noisy point evaluations on a fine grid. Standard solution methods usually employ discretization schemes that are directly induced by the…

Numerical Analysis · Mathematics 2025-04-04 Michael Griebel , Tim Jahn

Results are expoundd for the investigation of efficiency of the critical-component method for solving degenerate and ill-posed systems of linear algebraic equations

Rings and Algebras · Mathematics 2025-10-20 G. A. Emel'yanenko , M. G. Emelianenko , T. T. Rakhmonov , E. B. Dushanov , G. Yu. Konovalova

Highly oscillatory integrals of composite type arise in electronic engineering and their calculations is a challenging problem. In this paper, we propose two Gaussian quadrature rules for computing such integrals. The first one is…

Numerical Analysis · Mathematics 2025-04-01 Menghan Wu , Haiyong Wang

In this paper, we propose a numerical method of computing Hadamard finite-part integrals with an integral power singularity at the endpoint on a half infinite interval, that is, a finite value assigned to a divergent integral with an…

Numerical Analysis · Mathematics 2019-10-03 Hidenori Ogata

We introduce a new basis function (the spherical gaussian) for electronic structure calculations on spheres of any dimension $D$. We find \alert{general} expressions for the one- and two-electron integrals and propose an efficient…

Chemical Physics · Physics 2015-06-09 Peter M. W. Gill , Pierre-François Loos , Davids Agboola

In this paper, we present a Clenshaw-Curtis-Filon-type method for the weakly singular oscillatory integral with Fourier and Hankel kernels. By interpolating the non-oscillatory and nonsingular part of the integrand at $(N+1)$…

Numerical Analysis · Mathematics 2016-04-18 Zhenhua Xu

We propose an efficient algorithm for the approximation of fractional integrals by using Runge--Kutta based convolution quadrature. The algorithm is based on a novel integral representation of the convolution weights and a special…

Numerical Analysis · Mathematics 2019-07-29 Lehel Banjai , María López-Fernández

A new highly accurate numerical approximation scheme based on a Gauss type Clenshaw-Curtis Quadrature for Fredholm integral equations of the second kind, whose kernel is either discontinuous or not smooth along the main diagonal, is…

Numerical Analysis · Mathematics 2025-10-20 Sheon-Young Kang , Israel Koltracht , George Rawitscher

Numerical evaluations of Feynman integrals often proceed via a deformation of the integration contour into the complex plane. While valid contours are easy to construct, the numerical precision for a multi-loop integral can depend…

High Energy Physics - Phenomenology · Physics 2023-05-22 Ramon Winterhalder , Vitaly Magerya , Emilio Villa , Stephen P. Jones , Matthias Kerner , Anja Butter , Gudrun Heinrich , Tilman Plehn

We consider the numerical computation of resonances for metallic grating structures with dispersive media and small slit holes. The underlying eigenvalue problem is nonlinear and the mathematical model is multiscale due to the existence of…

Numerical Analysis · Mathematics 2024-03-08 Yingxia Xi , Junshan Lin , Jiguang Sun

A novel low complexity method to perform self-consistent electronic-structure calculations using the Kohn-Sham formalism of density functional theory is presented. Localization constraints are neither imposed nor required thereby allowing…

Computational Physics · Physics 2007-05-23 M. J. Rayson

The authors present SHarmonic, a new implementation of the spherical harmonics targeted for electronic-structure calculations. Their approach is to use explicit formulas for the harmonics written in terms of normalized Cartesian…

Computational Physics · Physics 2025-10-08 Xavier Andrade , Jacopo Simoni , Yuan Ping , Tadashi Ogitsu , Alfredo A. Correa

This overview is devoted to splitting methods, a class of numerical integrators intended for differential equations that can be subdivided into different problems easier to solve than the original system. Closely connected with this class…

Numerical Analysis · Mathematics 2024-05-08 Sergio Blanes , Fernando Casas , Ander Murua