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Related papers: Reassessing Graphene Absorption and Emission Spect…

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Many recent experiments investigated potential and attractive means of modifying many-body interactions in two-dimensional materials through time-resolved spectroscopy techniques. However, the role of ultrafast phonon-assisted processes in…

Materials Science · Physics 2020-01-28 Dino Novko , Marko Kralj

The unique terahertz properties of graphene has been identified for novel optoelectronic applications. In a graphene sample with bias voltage added, there is an enhanced absorption in the far infrared region and a diminished absorption in…

Mesoscale and Nanoscale Physics · Physics 2017-05-18 Yuan Yang , Grigory Kolesov , Lucas Kocia , Eric J. Heller

Ultrafast electron-phonon relaxation dynamics in graphene hides many distinct phenomena, such as hot phonon generation, dynamical Kohn anomalies, and phonon decoupling, yet still remains largely unexplored. Here, we unravel intricate…

Materials Science · Physics 2023-09-19 Nina Girotto , Dino Novko

We present a microscopic explanation of the controversially discussed transient negative differential transmission observed in degenerate optical pump-probe measurements in graphene. Our approach is based on the density matrix formalism…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Faris Kadi , Torben Winzer , Ermin Malic , Andreas Knorr

We examine the intrinsic energy dissipation steps in electrically biased graphene channels. By combining in-situ measurements of the spontaneous optical emission with a Raman spectroscopy study of the graphene sample under conditions of…

Mesoscale and Nanoscale Physics · Physics 2015-03-13 Stéphane Berciaud , Melinda Y. Han , Louis E. Brus , Philip Kim , Tony F. Heinz

The unique optical properties of graphene, with broadband absorption and ultrafast response, make it a critical component of optoelectronic and spintronic devices. Using time-resolved momentum microscopy with high data rate and high dynamic…

Indirect transitions of electrons in graphene and graphite are investigated by means of angle-resolved photoemission spectroscopy (ARPES) with several different incident photon energies and light polarizations. The theoretical calculations…

We study theoretically the strong-field absorption of an ultrafast optical pulse by a gapped graphene monolayer. At low field amplitudes, the absorbance in the pristine graphene is equal to the universal value of $2.3$ percent. Although the…

Mesoscale and Nanoscale Physics · Physics 2020-05-06 S. Azar Oliaei Motlagh , Ahmal Jawad Zafar , Aranyo Mitra , Vadym Apalkov , Mark I. Stockman

We study, by means of a Monte Carlo simulator, the hot phonon effect on the relaxation dynamics in photoexcited graphene and its quantitative impact as compared to considering an equilibrium phonon distribution. Our multi-particle approach…

Mesoscale and Nanoscale Physics · Physics 2016-02-02 José M. Iglesias , María J. Martín , Elena Pascual , Raúl Rengel

We devise a theory of adsorption of low-energy atoms on suspended graphene membranes maintained at 10 K based on a model of atom-acoustic phonon interactions. Our primary technique includes a non-perturbative method which treats the…

Mesoscale and Nanoscale Physics · Physics 2020-01-06 Sanghita Sengupta

Since graphene has no band gap, photoluminescence is not expected from relaxed charge carriers. We have, however, observed significant light emission from graphene under excitation by ultrashort (30-fs) laser pulses. Light emission was…

Mesoscale and Nanoscale Physics · Physics 2010-09-20 Chun Hung Lui , Kin Fai Mak , Jie Shan , Tony F. Heinz

The ultrafast relaxation and recombination dynamics of photogenerated electrons and holes in epitaxial graphene are studied using optical-pump Terahertz-probe spectroscopy. The conductivity in graphene at Terahertz frequencies depends on…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Paul A. George , Jared Strait , Jahan Dawlaty , Shriram Shivaraman , Mvs Chandrashekhar , Farhan Rana , Michael G. Spencer

We report optical pumping and X-ray absorption spectroscopy experiments at the PAL free electron laser that directly probe the electron dynamics of a graphene monolayer adsorbed on copper in the femtosecond regime. By analyzing the results…

Graphene is widely recognized for its ultrafast and broadband photocurrent response, but whether the broadband ultrafast characteristics are preserved at mid-infrared wavelengths with photon energies below the optical phonon energy remains…

We examine the photoconductivity of an intrinsic graphene associated with far- and mid-infrared irradiation at low temperatures. The model under consideration accounts for the excitation of the electron-hole pairs by incident radiation, the…

Materials Science · Physics 2008-05-27 F. T. Vasko V. Ryzhii

We report the ultrafast dynamics of the 47.4 THz coherent phonons of graphite interacting with a photoinduced non-equilibrium electron-hole plasma. Unlike conventional materials, upon photoexcitation the phonon frequency of graphite…

Other Condensed Matter · Physics 2008-03-13 Kunie Ishioka , Muneaki Hase , Masahiro Kitajima , Ludger Wirtz , Angel Rubio , Hrvoje Petek

For many of the envisioned optoelectronic applications of graphene it is crucial to understand the sub-picosecond carrier dynamics immediately following photoexcitation, as well as the effect on the electrical conductivity - the…

The broadband and ultrafast photoresponse of graphene has been extensively studied in recent years, although the photoexcited carrier dynamics is still far from being completely understood. Different experimental approaches imply either one…

Mesoscale and Nanoscale Physics · Physics 2017-08-22 Sergey Menabde , Hyunwoo Cho , Namkyoo Park

Saturable absorption is a non-perturbative nonlinear optical phenomenon that plays a pivotal role in the generation of ultrafast light pulses. Here we show that this effect emerges in graphene at unprecedentedly low light intensities, thus…

Mesoscale and Nanoscale Physics · Physics 2017-03-15 A. Marini , J. D. Cox , F. J. Garcia de Abajo

High intensity laser pulses were recently shown to induce a population inverted transient state in graphene [T. Li et al. Phys. Rev. Lett. 108, 167401 (2012)]. Using a combination of hydrodynamic arguments and a kinetic theory we determine…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Junhua Zhang , Tianqi Li , Jigang Wang , Joerg Schmalian
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