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Related papers: Is 1T-TaS$_2$ a 40 year old quantum spin liquid?

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To reveal the nature of elementary excitations in a quantum spin liquid (QSL), we measured low temperature thermal conductivity and specific heat of 1T-TaS$_2$, a QSL candidate material with frustrated triangular lattice of spin-1/2. The…

Strongly Correlated Electrons · Physics 2020-02-05 H. Murayama , Y. Sato , X. Z. Xing , T. Taniguchi , S. Kasahara , Y. Kasahara , M. Yoshida , Y. Iwasa , Y. Matsuda

When electron-electron interaction dominates over other electronic energy scales, exotic, collective phenomena often emerge out of seemingly ordinary matter. The strongly correlated phenomena, such as quantum spin liquid and unconventional…

Quantum spin liquids are exotic Mott insulators that carry extraordinary spin excitations and thus, when doped, expected to afford novel metallic states coupled to the unconventional magnetic excitations. The organic triangular-lattice…

Strongly Correlated Electrons · Physics 2025-01-07 H. Oike , Y. Suzuki , H. Taniguchi , K. Miyagawa , K. Kanoda

The quest for entangled spin excitations has stimulated intense research on frustrated magnetic systems. For almost two decades, the triangular-lattice Mott insulator $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ has been the hottest candidate for…

Strongly Correlated Electrons · Physics 2023-06-06 A. Pustogow , Y. Kawasugi , H. Sakurakoji , N. Tajima

Quantum spin liquids (QSLs) form an extremely unusual magnetic state in which the spins are highly correlated and fluctuate coherently down to the lowest temperatures, but without symmetry breaking and without the formation of any static…

Quantum spin liquids (QSLs) are highly entangled, disordered magnetic states that arise in frustrated Mott insulators and host exotic fractional excitations such as spinons and chargons. Despite being charge insulators some QSLs are…

Combination of low-dimensionality and electron correlation is vital for exotic quantum phenomena such as the Mott-insulating phase and high-temperature superconductivity. Transition-metal dichalcogenide (TMD) 1T-TaS2 has evoked great…

If a material with an odd number of electrons per unit cell turns out to be insulating, Mott localisation may be invoked as an explanation. This is widely accepted for the layered compound 1T-TaS2, which has a low-temperature insulating…

Strongly Correlated Electrons · Physics 2020-06-24 C. J. Butler , M. Yoshida , T. Hanaguri , Y. Iwasa

Recent theoretical investigations of quantum spin liquids have described phenomenology amenable to experimental observation using scanning tunneling microscopy. This includes characteristic resonances found at the edge of the upper Hubbard…

Strongly Correlated Electrons · Physics 2023-04-17 C. J. Butler , M. Yoshida , T. Hanaguri , Y. Iwasa

Quantum materials exhibiting magnetic frustration are connected to diverse phenomena including high-Tc superconductivity, topological order and quantum spin liquids (QSLs). A QSL is a quantum phase (QP) related to a quantum-entangled…

Strongly Correlated Electrons · Physics 2021-08-03 Samuel Mañas-Valero , Benjamin Huddart , Tom Lancaster , Eugenio Coronado , Francis Pratt

Transition metal dichalcogenides (TMDs) have emerged as a promising class of materials for spintronics, with the aim of promoting efficient spin-charge conversion (SCC) in TMD/ferromagnet (FM)-based devices. The MoTe$_2$ semimetal with…

The transition metal dichalcogenides 1T-TaS$_2$ and 1T-TaSe$_2$ have been extensively studied for the complicated correlated electronic properties. The origin of different surface electronic states remains controversial. We apply scanning…

Strongly Correlated Electrons · Physics 2022-01-11 Wenhao Zhang , Zongxiu Wu , Kunliang Bu , Ying Fei , Yuan Zheng , Jingjing Gao , Xuan Luo , Zheng Liu , Yu-ping Sun , Yi Yin

We investigate, using a first-principles density-functional methodology, the nature of magnetism in monolayer $1T$-phase of tantalum disulfide ($1T$-TaS$_2$ ). Magnetism in the insulating phase of TaS$_2$ is a longstanding puzzle and has…

Materials Science · Physics 2022-02-23 Diego Pasquier , Oleg V. Yazyev

A new frontier in condensed matter physics is to stack atomically thin layered-materials with different properties and create intriguing phenomena which do not exist in any of the constituent layers. Transition metal dichalcogenide…

Coexistence of localized and extended excitations is central to the macroscopic properties of correlated materials. For 5d transition metal compounds, electron correlations alone generally do not lead to a metal-insulator (Mott) transition,…

Quantum spin liquid represents an intriguing state where electron spins are highly entangled yet spin fluctuation persists even at 0 K. Recently, the hexaaluminates \textit{R}MgAl$_{11}$O$_{19}$ (\textit{R} = rare earth) have been proposed…

Strongly Correlated Electrons · Physics 2025-04-01 Yantao Cao , Akihiro Koda , M. D. Le , V. Pomjakushin , Benqiong Liu , Zhendong Fu , Zhiwei Li , Jinkui Zhao , Zhaoming Tian , Hanjie Guo

We point out that there are two different chiral spin liquid states on the triangular lattice and discuss the conducting states that are expected on doping them. These states labeled CS1 and CS2 are associated with two distinct topological…

Strongly Correlated Electrons · Physics 2021-05-05 Xue-Yang Song , Ashvin Vishwanath , Ya-Hui Zhang

We describe a new possible route to the metal-insulator transition in doped semiconductors such as Si:P or Si:B. We explore the possibility that the loss of metallic transport occurs through Mott localization of electrons into a quantum…

Strongly Correlated Electrons · Physics 2012-10-15 Andrew C. Potter , Maissam Barkeshli , John McGreevy , T. Senthil

We present the ultra-low-temperature thermal conductivity measurements on single crystals of the prototypical charge-density-wave material 1$T$-TaS$_2$, which was recently argued to be a candidate for quantum spin liquid. Our experiments…

Strongly Correlated Electrons · Physics 2017-10-16 Y. J. Yu , Y. Xu , L. P. He , M. Kratochvilova , Y. Y. Huang , J. M. Ni , Lihai Wang , Sang-Wook Cheong , Je-Geun Park , S. Y. Li

In this paper, we study the non-magnetic insulator state near Mott transition of 2D pi-flux Hubbard model on square lattice and find that such non-magnetic insulator state is quantum spin liquid state with nodal fermionic excitations -…

Strongly Correlated Electrons · Physics 2015-03-13 Su-Peng Kou , Lan-Feng Liu , Jing He , Ya-Jie Wu