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A 790-nm-driven high-harmonic generation source with a repetition rate of 6 kHz is combined with a toroidal-grating monochromator and a high-detection-efficiency photoelectron time-of-flight momentum microscope to enable time- and…

Attosecond laser pulses open the door to resolve microscopic electron dynamics in time. Experiments performed include the decay of a core hole, the time-resolved measurement of photo ionization and electron tunneling. The processes…

Atomic and Molecular Clusters · Physics 2011-11-09 Ionut Georgescu , Ulf Saalmann , Jan M. Rost

Photons, electrons, and their interplay are at the heart of photonic devices and modern instruments for ultrafast science [1-10]. Nowadays, electron beams of the highest intensity and brightness are created by photoemission with short laser…

The ultrafast response of metals to light is governed by intriguing non-equilibrium dynamics involving the interplay of excited electrons and phonons. The coupling between them gives rise to nonlinear diffusion behavior on ultrashort…

The precision measurement of real-time electron temporal profiles is crucial for advancing electron and X-ray devices used in ultrafast imaging and spectroscopy. While high temporal resolution and large temporal window can be achieved…

The ultrafast dynamics of charge carriers in solids plays a pivotal role in emerging optoelectronics, photonics, energy harvesting, and quantum technology applications. However, the investigation and direct visualization of such…

The pursuit of ever-shorter time scales is a frontier in modern physics, exemplified by the synthesis of attosecond light pulses -- an achievement made possible by coherently superimposing a broad range of photon energies, as required by…

Mesoscale and Nanoscale Physics · Physics 2025-04-25 Xin Jin , Cruz I. Velasco , F. Javier García de Abajo

Ultrafast electronic dynamics are typically studied using pulsed lasers. We demonstrate a complementary experimental approach: quantum simulation of ultrafast dynamics using trapped ultracold atoms. Counter-intuitively, this technique…

Field-emission of electrons underlies major advances in science and technology, ranging from imaging the atomic-scale structure of matter to signal processing at ever-higher frequencies. The advancement of these applications to their…

Optics · Physics 2023-02-22 H. Y. Kim , M. Garg , S. Mandal , L. Seiffert , T. Fennel , E. Goulielmakis

Femtosecond-scale ultrafast imaging is an essential tool for visualizing ultrafast dynamics in molecular biology, physical chemistry, atomic physics, and fluid dynamics. Pump-probe imaging and a streak camera are the most widely used…

Optics · Physics 2020-03-18 Jungho Moon , Seok-Chan Yoon , Yong-sik Lim , Wonshik Choi

In this manuscript we present a theoretical framework and its numerical implementation to simulate the out-of-equilibrium electron dynamics induced by the interaction of ultrashort laser pulses in condensed-matter systems. Our approach is…

We study the ultrafast dynamics of surface electromagnetic waves photogenerated on aluminum film perforated with subwavelength holes array by means of transient photomodulation with 100 fs time resolution. We observed a pronounced blueshift…

Materials Science · Physics 2009-11-13 A. S. Kirakosyan , M. Tong , T. V. Shahbazyan , Z. V. Vardeny

State-of-the-art attosecond metrology deals with the detection and characterization of photon pulses with typical energies up to the hundreds of eV and time resolution of several tens of attoseconds. Such short pulses are used for example…

Instrumentation and Detectors · Physics 2015-06-04 Andreas Ipp , Jörg Evers , Christoph H. Keitel , Karen Z. Hatsagortsyan

One of the frontiers of modern electron scattering instrumentation is improving temporal resolution in order to enable the observation of dynamical phenomena at their fundamental time-scales. We analyze how a radiofrequency cavity can be…

Accelerator Physics · Physics 2019-01-16 David Cesar , Pietro Musumeci

In the quest for dynamic multimodal probing of a material's structure and functionality, it is critical to be able to quantify the chemical state on the atomic and nanoscale using element specific electronic and structurally sensitive tools…

Ultrafast spectroscopies can access the dynamics of electrons and nuclei at short timescales, shedding light on nonequilibrium phenomena in materials. However, development of accurate calculations to interpret these experiments has lagged…

Materials Science · Physics 2021-05-05 Xiao Tong , Marco Bernardi

When an electromagnetic (EM) wave is propagating in a medium whose properties are varied abruptly in time, the wave experiences refractions and reflections known as "time-refractions" and "time-reflections", both manifesting spectral…

Applied Physics · Physics 2023-10-05 Thomas R. Jones , Alexander V. Kildishev , Mordechai Segev , Dimitrios Peroulis

We demonstrate the compression of electron pulses in a high-brightness ultrafast electron diffraction (UED) instrument using phase-locked microwave signals directly generated from a mode-locked femtosecond oscillator. Additionally, a…

Plasma Physics · Physics 2017-08-03 Martin R. Otto , Laurent P. Rene de Cotret , Mark J. Stern , Bradley J. Siwick

Quantum tunnelling of electrons can be confined to the sub-cycle time scale of strong light fields, contributing decisively to the extreme time resolution of attosecond science. Because tunnelling also enables atomic-scale spatial…