Related papers: Enhanced nonlinear optical response from individua…
Second harmonic generation (SHG) with a material of large transparency is an attractive way of generating coherent light sources at exotic wavelength range such as VUV, UV and visible light. It is of critical importance to improve nonlinear…
Second order optical nonlinear processes involve the coherent mixing of two electromagnetic waves to generate a new optical frequency, which plays a central role in a variety of applications, such as ultrafast laser systems, rectifiers,…
We report the observation of optical second harmonic generation (SHG) in single-layer indium selenide (InSe). We measure a second harmonic signal of $>10^3$ $\textrm{cts/s}$ under nonresonant excitation using a home-built confocal…
Twisting two dissimilar monolayer semiconductors induces structural chirality that remains largely elusive in linear optics but becomes remarkably pronounced in the nonlinear regime. Here we demonstrate that MoS2/WSe2 heterobilayers exhibit…
Nonlinear optical materials of atomic thickness--such as non-centrosymmetric 2H transition metal dichalcogenide monolayers--have a second order nonlinear susceptibility ($\chi^{(2)}$) whose intensity can be tuned by strain. However, whether…
We conduct a theoretical and numerical study on the second-harmonic (SH) optical response of a nano-structured metamaterial composed of a periodic array of inclusions. Both the inclusions and their surrounding matrix are made of…
Noble metals with well-defined crystallographic orientation constitute an appealing class of materials for controlling light-matter interactions on the nanoscale. Nonlinear optical processes, being particularly sensitive to anisotropy, are…
The effective second-harmonic generation (SHG) coefficient is a crucial data that quantifies the efficiency of transforming fundamental frequency light into its second harmonic. With the help of the symmetry of nonlinear optical…
The nonlinear properties of a metamaterial sample composed of double-layer metallic patterns and voltage controllable diodes are experimentally investigated. Second harmonics and spectrum modulations are clearly observed in a wide band of…
To add the detailed information to the existed knowledge of nonlinear optics field, the nonlinear optical processes of the second and third order have been discussed in their respective susceptibility tensors in the presence of degenerate…
We employ transformation optics to optimize the generic nonlinear wave interaction of second-harmonic generation from a pair of touching metallic wires. We demonstrate a 10 orders of magnitude increase in the second-harmonic scattering…
Optical coating, an integral part of many optical systems, is prone to damage from environmental exposure and laser irradiation. This underscores the need for reliable and sensitive coating diagnostics. We introduce second harmonic…
The study of the non-linear response of matter to high electric fields has recently encompassed harmonic generation in solids at near-infrared (NIR) driving wavelengths. Interest has been driven by the prospect of ultrafast signal…
The microscopic structure of two amorphous materials with extreme nonlinear optical properties has been studied. One of these materials exhibits second harmonic generation, while another material of similar molecular structure emits…
Plasmonic enhancement of nonlinear optical processes confront severe limitations arising from the strong dispersion of metal susceptibilities and small interaction volumes that hamper desirable phase-matching-like conditions. Maximizing…
The ability to engineer metamaterials with tunable nonlinear optical properties is crucial for nonlinear optics. Traditionally, metals have been employed to enhance nonlinear optical interactions through field localization. Here, inspired…
We report on the linear and nonlinear optical response of metamaterials evoked by first and second order multipoles. The analytical ground on which our approach bases permits for new insights into the functionality of metamaterials. For the…
We demonstrate analytically and numerically that a subwavelength-core dielectric photonic nanowire embedded in a properly designed photonic crystal fiber cladding shows evidence of a previously unknown kind of nonlinearity (the magnitude of…
We present a theoretical study of the optical response of a nonlinear oscillator formed by coupling a metal nanoparticle local surface plasmon resonance to excitonic degrees of freedom in a monolayer transition-metal dichalcogenide. We show…
We theoretically predict efficient optical second-harmonic generation (SHG) from a few hundred nanometer thick slab consisting of a quadratic nonlinear anisotropic medium whose linear principal permittivities are, at the fundamental…