Related papers: Frequency comb based four-wave-mixing spectroscopy
Frequency comb based multidimensional coherent spectroscopy is a novel optical method that enables high resolution measurement in a short acquisition time. The method's resolution makes multidimensional coherent spectroscopy relevant for…
Frequency combs can be generated in millimeter-sized optical resonators thanks to their ability to store extremely high light intensities and the nonlinearity of their materials. New frequencies are generated through a cascaded parametric…
The broadband, coherent nature of narrow-linewidth fiber frequency combs is exploited to measure the full complex spectrum of a molecular gas through multi-heterodyne spectroscopy. We measure the absorption and phase shift experienced by…
Multiheterodyne techniques using frequency combs -- light sources whose lines are perfectly evenly-spaced -- have revolutionized optical science. By beating an unknown signal with the many lines of a comb, its spectrum is recovered.…
A general mechanism for the generation of frequency combs referenced to atomic resonances is put forward. The mechanism is based on the periodic phase control of a quantum system's dipole response. We develop an analytic description of the…
Optical frequency combs are an essential tool for precision metrology experiments ranging in application from remote spectroscopic sensing of trace gases to the characterization and comparison of optical atomic clocks for precision…
High finesse frequency combs (HFC) with large ratio of the frequency spacing to the width of the spectral components have demonstrated remarkable results in many applications such as precision spectroscopy and metrology. We found that low…
Dual comb spectroscopy allows for high-resolution spectra to be measured over broad bandwidths, but an essential requirement for coherent integration is the availability of a phase reference. Usually, this means that the combs' phase and…
We report on the fabrication of high-Q, fused-quartz microresonators and the parametric generation of a frequency comb with 36 GHz line spacing using them. We have characterized the intrinsic stability of the comb in both the time and…
We demonstrate a new technique for the experimental measurement of the spectral coherence of microresonator optical frequency combs. Specifically, we use a spectral interference method, typically used in the context of supercontinuum…
Frequency-modulated (FM) combs are produced by mode-locked lasers in which the electric field has a linearly chirped frequency and nearly constant amplitude. This regime of operation occurs naturally in certain laser systems and constitutes…
While mid-infrared optical frequency combs have been widely utilized in areas such as trace gas sensing, chemical kinetics, and combustion science, the relatively low power per comb tooth has limited acquisition times and sensitivities. We…
We report on the experimental demonstration of a tunable monolithic optical frequency comb generator. The device is based on the four-wave mixing in a crystalline calcium fluoride whispering gallery mode resonator. The frequency spacing of…
Dual-comb spectroscopy is emerging as one of the most appealing applications of mid-infrared frequency combs for high-resolution molecular spectroscopy, as it leverages on the unique coherence properties of frequency combs combined with the…
Recent developments demonstrate that parametric four-wave mixing (FWM) in high-Q microresonators is a highly promising and effective approach for optical frequency comb generation, with applications including spectroscopy, optical clocks,…
Photonic chip-based frequency combs have emerged as a transformative platform, enabling compact, scalable, and high-performance multiwavelength sources with far-reaching impact across science and technology. Most commonly, these sources…
A theoretical analysis is carried out for the recently developed three-pulse photon echo spectroscopy employing dual frequency combs (DFC) as the light sources. In this method, the molecular sample interacts with three pulse trains derived…
Optical frequency combs [1-8] have resulted in significant advances in optical frequency metrology and found wide application to precise physical measurements [1-4, 9] and molecular fingerprinting [8]. A direct analogue of frequency combs…
Frequency metrology lies at the heart of precision measurement. Optical frequency combs provide a coherent link uniting the microwave and optical domains in the electromagnetic spectrum, with profound implications in timekeeping, sensing…
We experimentally demonstrate a versatile technique for performing dual-comb interferometry using a single frequency comb. By rapid switching of the repetition rate, the output pulse train can be delayed and heterodyned with itself to…