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We report the first observation of Rabi oscillations in the spin-7/2 ensemble of trivalent gadolinium ions hosted in CaWO$_4$ single crystal. A number of transitions within the lowest electronic multiplet $^8S_{7/2}$ of Gd$^{3+}$ ion are…

Mesoscale and Nanoscale Physics · Physics 2017-02-27 E. I. Baibekov , M. R. Gafurov , D. G. Zverev , I. N. Kurkin , A. A. Rodionov , B. Z. Malkin , B. Barbara

Using a general parametrization of the spin structure of the matrix element for the elastic $e^-+^4He$ scattering and for the annihilation $e^++e^-\to \pi^++\pi^-$ reactions in terms of two complex amplitudes, we derive general properties…

Nuclear Theory · Physics 2014-11-18 G. I. Gakh , E. Tomasi--Gustafsson

Defects in silicon carbide are of intense and increasing interest for quantum-based applications due to this material's properties and technological maturity. We calculate the multi-particle symmetry adapted wave functions of the negatively…

Mesoscale and Nanoscale Physics · Physics 2016-03-23 Ö. O. Soykal , Pratibha Dev , Sophia E. Economou

We study the exchange constants of MnV$_2$O$_4$ using magnetic force theorem and local spin density approximation of density functional theory supplemented with a correction due to on-site Hubbard interaction U. We obtain the exchanges for…

Materials Science · Physics 2013-08-13 R. Nanguneri , S. Y. Savrasov

A nonadiabatic scheme for the description of the coupled electron and nuclear motions in the ozone molecule was proposed recently. An initial coherent nonstationary state was prepared as a superposition of the ground state and the excited…

Atomic and Molecular Clusters · Physics 2015-06-18 A. Perveaux , D. Lauvergnat , B. Lasorne , F. Gatti , M. A. Robb , G. J. Halász , Á. Vibók

A quantitative theoretical study of the dissociative recombination of SH$^+$ with electrons has been carried out. Multireference, configuration interaction calculations were used to determine accurate potential energy curves for SH$^+$ and…

Instrumentation and Methods for Astrophysics · Physics 2024-05-31 D. O. Kashinski , D. Talbi , A. P. Hickman , O. E. Di Nallo , F. Colboc , K. Chakrabarti , I. F. Schneider , J. Zs Mezei

Sr$_2$IrO$_4$ is an extensively studied spin-orbit coupling induced insulator with antiferromagnetic ground state. The delicate balance between competing energy scales plays crucial role for its low temperature phase, and the route of…

Strongly Correlated Electrons · Physics 2017-10-31 Imtiaz Noor Bhatti , R. S. Dhaka , A. K. Pramanik

The coupled valence and spin state transition (VSST) taking place in (Pr0.7Sm0.3)0.7Ca0.3CoO3 was investigated by soft x-ray absorption spectroscopy (XAS) experiments carried out at the Pr-M4,5, Co-L2,3, and O-1s edges. This VSST is found…

Strongly Correlated Electrons · Physics 2015-06-15 F. Guillou , Q. Zhang , Z. Hu , C. Y. Kuo , Y. Y. Chin , H. J. Lin , C. T. Chen , A. Tanaka , L. H. Tjeng , V. Hardy

The relative intensity distribution in the rotationally resolved laser-induced fluorescence spectra belonging to the $E(4)^1\Sigma^+\to (a^3\Sigma^+_1,X^1\Sigma^+)$ band systems of the KCs molecule was analyzed. The experimental intensities…

Atomic Physics · Physics 2022-09-14 I. Klincare , M. Tamanis , R. Ferber , E. A. Pazyuk , A. V. Stolyarov , I. Havalyova , A. Pashov

An investigation of the rotational spectrum of the interstellar molecule thioformaldehyde between 110 and 377 GHz through a pyrolysis reaction revealed a multitude of absorption lines assignable to H$_2$CS and H$_2$C$^{34}$S in their lowest…

Molecular hydrogen ions are of metrological relevance due to the possibility of precise theoretical evaluation of their spectrum and of external-field-induced shifts. In homonuclear molecular ions the electric dipole $E1$ transitions are…

Atomic Physics · Physics 2021-01-20 P. Danev , D. Bakalov , V. I. Korobov , S. Schiller

Para- and ortho- isomers of water have different chemical and physical properties. Excitations by magnetic field, laser emission or hydrodynamic cavitation are reported to change energetic levels and spin configurations of water molecules…

Chemical Physics · Physics 2022-05-18 Serge Kernbach

The reflectivity of single-crystalline CoO has been studied by optical spectroscopy for wave numbers ranging from 100 to 28,000\wn and for temperatures 8 $< T <$ 325 K\@. A splitting of the cubic IR-active phonon mode on passing the…

Strongly Correlated Electrons · Physics 2009-01-20 Ch. Kant , T. Rudolf , F. Schrettle , F. Mayr , J. Deisenhofer , P. Lunkenheimer , M. V. Eremin , A. Loidl

We report the results of various measurements, namely magnetization, complex dielectric permittivity and electric polarization (P) on Dy2BaNiO5 as a function of temperature (T) and magnetic-field (H), apart from heat-capacity (C), with the…

Materials Science · Physics 2015-06-15 Kiran Singh , Tathamay Basu , S. Chowki , N. Mahapotra , K. Iyer , P. L. Paulose , E. V. Sampathkumaran

The determination of transport mechanisms in organic light-emitting diodes (OLEDs) is crucial for optimizing device performance. Magnetic field measurements enable the differentiation of spin state interconversion mechanisms, but data…

The Interacting Boson plus broken-pairs Model has been used to describe high-spin bands in spherical and transitional nuclei. In the spherical nucleus $^{104}$Cd the model reproduces the structure of high-spin bands built on a vibrational…

Nuclear Theory · Physics 2007-05-23 G. Bonsignori , D. Vretenar , S. Cacciamani , L. Corradini

Open-shell non-rigid molecular systems exhibiting an internal rotation are likely candidates for a coupling between the spin angular momentum of the unpaired electron and the torsional motion. This electron spin-torsion coupling lacked both…

Photodissociation cross sections for the SH$^+$ radical are computed from all rovibrational (RV) levels of the ground electronic state X$~^3\Sigma^-$ for wavelengths from threshold to 500~\AA. The five electronic transitions, $2~ ^3\Sigma^-…

Earth and Planetary Astrophysics · Physics 2016-05-04 E. C. McMillan , G. Shen , J. F. McCann , B. M. McLaughlin , P. C. Stancil

Spin transfer in high energy fragmentation process is determined by the hadronization mechanism and spin structure of hadrons.It can be studied by measuring the polarizations of hyperons and/or vector mesons in e+e- annihilation, in the…

High Energy Physics - Phenomenology · Physics 2009-11-10 Zuo-Tang Liang

New ab-initio surface hopping simulations of the excited state dynamics of CS$_2$ including spin-orbit coupling are compared to new experimental measurements using a multiphoton ionisation probe in a photoelectron spectroscopy experiment.…