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Two strategies for enhancing photovoltaic (PV) performance in chalcopyrite solar cells were investigated: Cu1-xKxIn1-yGaySe2 absorbers with low K content (K/(K+Cu), or x ~ 0.07) distributed throughout the bulk, and CuIn1-yGaySe2 absorbers…

Mesoscale and Nanoscale Physics · Physics 2017-04-07 Christopher P. Muzzillo , Timothy J. Anderson

Co-evaporation of Cu-KF-In-Se was performed on substrates with varied surface Na compositions. Compositions of interest for photovoltaic absorbers were studied, with ratios of (K+Cu)/In ~ 0.85 and K/(K+Cu) ~ 0 - 0.57. Soda-lime glass (SLG)…

Materials Science · Physics 2018-04-04 Christopher P. Muzzillo , Ho Ming Tong , Timothy J. Anderson

Films of Cu-K-In-Se were co-evaporated at varied K/(K+Cu) compositions and substrate temperatures (with constant (K+Cu)/In ~ 0.85). Increased Na composition on the substrate's surface and decreased growth temperature were both found to…

Materials Science · Physics 2017-03-21 Christopher P. Muzzillo , Ho Ming Tong , Timothy J. Anderson

Cu2ZnSnS(e)4 (CZTS(e)) solar cells have attracted much attention due to the elemental abundance and the non-toxicity. However, the record efficiency of 12.6% for Cu2ZnSn(S,Se)4 (CZTSSe) solar cells is much lower than that of Cu(In,Ga)Se2…

Applied Physics · Physics 2018-03-14 Shoushuai Gao , Zhenwu Jiang , Li Wu , Jianping Ao , Yu Zeng , Yun Sun , Yi Zhang

Inorganic CdTe and FeSi2-based solar cells have recently drawn a lot of attention because they offer superior thermal stability and good optoelectronic properties compared to conventional solar cells. In this work, a unique alternative…

Interface recombination at the absorber buffer interface impedes the efficiency of a solar cell with an otherwise excellent absorber. The internal voltage or the quasi-Fermi level splitting (qFLs) measures the quality of the absorber.…

In this work, first principle calculations of Cu$_2$ZnSnS$_4$ (CZTS), Cu$_2$ZnGeS$_4$ (CZGS) and Cu$_2$ZnSiS$_4$ (CZSS) are performed to highlight the impact of the cationic substitution on the structural, electronic and optical properties…

Applied Physics · Physics 2022-02-22 Thomas Ratz , Jean-Yves Raty , Guy Brammertz , Bart Vermang , Ngoc Duy Nguyen

Recent technical and commercial successes of existing thin film solar cell technologies motivates exploration of next-generation photovoltaic (PV) absorber materials. Of particular scientific interest are compounds like CuSbSe$_2$, which do…

Materials Science · Physics 2015-05-12 Adam Welch , Lauryn Baranowski , Pawel Zawadzki , Stephan Lany , Colin Wolden , Andriy Zakutayev

Kesterite is a leading candidate among inorganic thin-film photovoltaic technologies, offering sustainable and environmentally friendly solutions without reliance on critical raw materials. This study investigates the performance of…

Wide-gap Cu(In,Ga)S2 solar cells with In2O3:Sn (ITO) as transparent back contact are evaluated for the application as top cells in tandem devices. The effect of Na on the solar cell performance is investigated by supplying additional Na by…

Ternary chalcostibite copper antimony selenide (CuSbSe2) is a promising absorber material for next generation thin film solar cells due to the non-toxic nature, earth-abundance, low-cost fabrication technique, optimum bandgap and high…

Chalcopyrite semiconductors are of considerable interest for application as absorber layers in thin-film photovoltaic cells. When growing films of these compounds, however, they are often found to contain CuAu- like domains, a metastable…

Materials Science · Physics 2017-04-05 Marnik Bercx , Nasrin Sarmadian , Rolando Saniz , Bart Partoens , Dirk Lamoen

Reducing the thickness of Cu(In,Ga)Se2 solar cells is a key objective in order to reduce production cost and to improve sustainability. The major challenge for sub-micron Cu(In,Ga)Se2 cells is the recombination at the backside. In standard…

Dual-absorber solar cells represent a promising approach to surpass the efficiency limit of single-junction devices by extending spectral absorption and minimizing thermalization losses. Among earth-abundant thin-film materials, kesterites…

Materials Science · Physics 2025-11-14 Hasib Md Abid Bin Farid , Md Tashfiq Bin Kashem

Cu-based chalcogenides are promising materials for thin-film solar cells with more than 20% measured cell efficiency. Using first-principles calculations based on density functional theory, the optoelectronic properties of a group of…

Materials Science · Physics 2016-09-21 Nasrin Sarmadian , Rolando Saniz , Bart Partoens , Dirk Lamoen

This study underscores the pivotal role of sodium (Na) supply in optimizing the optoelectronic properties of wide bandgap (~1.6 eV) Cu(In,Ga)S2 (CIGS) thin film absorbers for high efficiency solar cells. Our findings demonstrate that the…

Traditional CdS buffer layer in selenium-free Cu(In,Ga)S2 solar cells leads to reduced open-circuit voltage because of a negative conduction band offset at the Cu(In,Ga)S2/CdS interface. Reducing this loss necessitates the substitution of…

In this article, we demonstrate CdSe-CuSbSe2-based double junction two-terminal tandem solar cells simulated with SCAPS-1D. The highest performance of the tandem cell has been confirmed by optimizing the electrical and optical properties of…

Cu based ternary chalcogenides are gathering attention for sustainable energy applications due to their reduced complexity compared to quaternary alternatives. We used drift diffusion modeling to evaluate the feasibility of photovoltaics…

Materials Science · Physics 2026-05-12 Saptarshi Mandal , Surbhi Ramawat , Sumit Kukreti , Ambesh Dixit

Thin-film solar cells reach high efficiencies and have a low carbon footprint in production. Tandem solar cells have the potential to significantly increase the efficiency of this technology, where the bottom-cell is generally composed of a…

Applied Physics · Physics 2025-12-01 Thomas Paul Weiss , Mohit Sood , Aline Vanderhaegen , Susanne Siebentritt
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