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The Kagome-lattice-based material, Volborthite, $\mathrm{Cu_3 V_2 O_7 (OH)_2 \cdot 2 H_2 O}$, has been considered as a promising platform for discovery of unusual quantum ground states due to the frustrated nature of spin interactions. Here…

Strongly Correlated Electrons · Physics 2017-07-19 Li Ern Chern , Kyusung Hwang , Tomonari Mizoguchi , Yejin Huh , Yong Baek Kim

Magnetic properties of the spin-1/2 kagome-like compound volborthite are studied using a high-quality polycrystalline sample. It is evidenced from magnetization and specific heat measurements that the spins on the kagome lattice still…

We report 51V-NMR study on a high-quality powder sample of volborthite Cu3V2O7(OH)2/2H2O, a spin-1/2 Heisenberg antiferromagnet on a distorted kagome lattice formed by isosceles triangles. In the magnetic fields below 4.5 T, a sharp peak in…

Strongly Correlated Electrons · Physics 2017-12-01 M. Yoshida , M. Takigawa , H. Yoshida , Y. Okamoto , Z. Hiroi

When quantum fluctuations destroy underlying long-range ordered states, novel quantum states emerge. Spin-liquid (SL) states of frustrated quantum antiferromagnets, in which highly-correlated spins keep to fluctuate down to very low…

Recent numerical studies have provided strong evidence for a gapped $Z_2$ quantum spin liquid in the kagome lattice spin-1/2 Heisenberg model. A special feature of spin liquids is that symmetries can be fractionalized, and different…

Strongly Correlated Electrons · Physics 2018-01-01 Yuan-Ming Lu , Gil Young Cho , Ashvin Vishwanath

In Volborthite, spin-1/2 moments form a distorted Kagom\'e lattice, of corner sharing isosceles triangles with exchange constants $J$ on two bonds and $J'$ on the third bond. We study the properties of such spin systems, and show that…

Strongly Correlated Electrons · Physics 2007-09-29 Fa Wang , Ashvin Vishwanath , Yong Baek Kim

A three-dimensional system of interacting spins typically develops static long-range order when it is cooled. If the spins are quantum (S = 1/2), however, novel quantum paramagnetic states may appear. The most highly sought state among them…

Strongly Correlated Electrons · Physics 2015-05-13 S. -H. Lee , H. Kikuchi , Y. Qiu , B. Lake , Q. Huang , K. Habicht , K. Kiefer

Thermodynamic investigations on volborthite (Cu3V2O7(OH)2 2H2O), which possesses a two-dimensional kagome structure of S-1/2 spins, are presented. The low-temperature heat capacities of volborthite and its Zn analogue compound were measured…

Strongly Correlated Electrons · Physics 2010-08-12 Satoshi Yamashita , Tomoya Moriura , Yasuhiro Nakazawa , Hiroyuki Yoshida , Yoshihiko Okamoto , Zenji Hiroi

A novel cuprate Volborthite, Cu3V2O7(OH)2-2H2O, containing an S-1/2 (Cu 2+ spin) kagome-like lattice is studied by magnetic susceptibility, specific heat, and 51 V NMR measurements. Signs for neither long-range order nor spin-gapped singlet…

Strongly Correlated Electrons · Physics 2009-11-07 Z. Hiroi , M. Hanawa , N. Kobayashi , M. Nohara , H. Takagi , Y. Kato , M. Takigawa

Recent experiments suggest a quantum spin liquid ground state in the material PbCuTe$_2$O$_6$, where $S=1/2$ moments are coupled by antiferromagnetic Heisenberg interactions into a three dimensional structure of corner sharing triangles…

Strongly Correlated Electrons · Physics 2021-09-15 Li Ern Chern , Yong Baek Kim

We determined the spin exchanges between the Cu2+ ions in the kagome layers of volborthite, Cu3V2O7(OH)2x2H2O, by performing the energy-mapping analysis based on DFT+U calculations, to find that the kagom\'e layers of Cu2+ ions are hardly…

Strongly Correlated Electrons · Physics 2022-03-02 Myung-Hwan Whangboa , Hyun-Joo Koo , Eva Brücher , Pascal Puphal , Reinhard K. Kremer

The spin-$\frac{1}{2}$ kagome antiferromagnet is considered an ideal host for a quantum spin liquid ground state. We find that when the bonds of the kagome lattice are modulated with a periodic pattern, new quantum ground states emerge.…

Exotic quantum spin liquid (QSL) is formed with such hypothetic particles as fermionic spinons carrying spin 1/2 and no charge. Here we calculate its thermodynamic and relaxation properties. Our calculations unveil the fundamental…

Strongly Correlated Electrons · Physics 2012-03-02 V. R. Shaginyan , A. Z. Msezane , K. G. Popov , G. S. Japaridze , V. A. Stephanovich

We argue for the existence of a liquid ground state in a class of square lattice models of orbitally degenerate insulators. Starting with the SU(4) symmetric Kugel-Khomskii model, we utilize a Majorana Fermion representation of spin-orbital…

Strongly Correlated Electrons · Physics 2009-08-22 Fa Wang , Ashvin Vishwanath

The ground state of the spin$-1/2$ kagome antiferromagnet remains uncertain despite decades of active research. Here we step aside from this debated question to address the ground-state nature of a related, and potentially just as rich,…

Strongly Correlated Electrons · Physics 2019-12-11 Tristan Lugan , L. D. C Jaubert , Arnaud Ralko

The doped quantum spin liquid on the kagome lattice provides a fascinating platform to explore exotic quantum states, such as the reported holon Wigner crystal at low doping. By extending the doping range to $\delta = 0.027$ - $0.36$, we…

Strongly Correlated Electrons · Physics 2025-12-01 Xu-Yan Jia , Wen Huang , D. N. Sheng , Shou-Shu Gong

Quantum spin liquids (QSLs) represent an exotic quantum many-body state characterized by the suppression of long-range magnetic order due to strong quantum fluctuations. The kagome spin-1/2 antiferromagnet (AFM) is a prime candidate for…

Strongly Correlated Electrons · Physics 2024-07-24 S. Suetsugu , T. Asaba , S. Ikemori , Y. Sekino , Y. Kasahara , K. Totsuka , B. Li , Y. Zhao , Y. Li , Y. Kohama , Y. Matsuda

The search for exotic quantum spin liquid states in simple yet realistic spin models remains a central challenge in the field of frustrated quantum magnetism. Here we consider the canonical nearest-neighbor kagome Heisenberg antiferromagnet…

Strongly Correlated Electrons · Physics 2018-08-29 Amir M-Aghaei , Bela Bauer , Kirill Shtengel , Ryan V. Mishmash

Motivated by recent experimental observations of Kondo resonances in cobalt atoms on single layer 1T-TaSe$_{2}$, we theoretically investigate the effect of coupling a U(1) quantum spin liquid with a spinon Fermi surface to a lattice of…

Strongly Correlated Electrons · Physics 2024-04-01 Xia-Ming Zheng , Mehdi Kargarian

The exotic normal state of iron chalcogenide superconductor FeSe, which exhibits vanishing magnetic order and possesses an electronic nematic order, triggered extensive explorations of its magnetic ground state. To understand its novel…

Strongly Correlated Electrons · Physics 2017-08-22 Shou-Shu Gong , W. Zhu , D. N. Sheng , Kun Yang
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