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A density matrix based analytical model is developed to study the coherent probe field propagation through a four-level V type system in presence of a coherent control field. The model allows coupling of the probe field from the upper…

We investigate how the quantum control of a two-level system (TLS) coupled to photons can modify and tune the TLS's photon absorption spectrum. Tuning and controlling the emission and the absorption is of much interest e.g.\ for the…

Quantum Physics · Physics 2017-06-07 H. F. Fotso , V. V. Dobrovitski

We obtain gain of the probe field at multiple frequencies in a closed three-level V-type system using frequency modulated pump field. There is no associated population inversion among the atomic states of the probe transition. We describe…

Optics · Physics 2009-11-07 Harshawardhan Wanare

The transient signals derived from femtosecond pump-probe experiments are analyzed in terms of the coherent evolution of the energy levels perturbed by the excitation pulse. The model system is treated as the sum of independent two-level…

Atomic Physics · Physics 2016-09-13 A. Peralta Conde , R. Montero , A. Longarte

We calculate the transient absorption of an isolated attosecond pulse by helium atoms subject to a delayed infrared (\ir) laser pulse. With the central frequency of the broad attosecond spectrum near the ionization threshold, the absorption…

Atomic Physics · Physics 2015-06-12 Shaohao Chen , Mengxi Wu , Mette B. Gaarde , Kenneth J. Schafer

In recent years, ultrafast pump-probe spectroscopy has provided insightful information about nonequilibrium dynamics of excitations in materials. In a typical experiment of time-resolved x-ray absorption spectroscopy, the systems are…

Strongly Correlated Electrons · Physics 2019-05-29 Chen-Yen Lai , Jian-Xin Zhu

The effect of quantum interference on the optical properties of a pumped-probe three-level V-type atomic system is investigated. The probe absorption, dispersion, group index and optical bistability beyond the two-photon resonance condition…

Quantum Physics · Physics 2015-06-04 S. M. Mousavi , L. Safari , M. Mahmoudi , M. Sahrai

Spectroscopy is an important tool for probing the properties of materials, chemicals and biological samples. We design a practical transmitter-receiver system that exploits entanglement to achieve a provable quantum advantage over all…

Quantum Physics · Physics 2020-11-03 Haowei Shi , Zheshen Zhang , Stefano Pirandola , Quntao Zhuang

We have measured the photon statistics of pump and probe beams after interaction with Rb atoms in a situation of Electromagnetically Induced Transparency. Both fields present super-poissonian statistics and their intensities become…

Quantum Physics · Physics 2009-11-07 C. L. Garrido Alzar , L. S. Cruz , J. G. Aguirre Gomez , M. Franca Santos , P. Nussenzveig

Dynamics of materials under high-pressure conditions has been an important focus of materials science, especially in the timescale of pico- and femto-second of electronic and vibrational motion, which is typically probed by ultrafast laser…

Optics · Physics 2024-12-12 Zi-Qian Cheng , Xiao-Shuang Yin , Liu-Xiang Yang , Hui Dong

Nonlinear optics experiments measuring phase shifts induced in a weak probe pulse by a strong pump pulse must account for coherent effects that only occur when the pump and probe pulses are temporally overlapped. It is well known that a…

We study in detail coherent phase control of femtosecond resonance-mediated (2+1) three-photon absorption and its dependence on the spectral bandwidth of the excitation pulse. The regime is the weak-field regime of third perturbative order.…

Atomic Physics · Physics 2007-11-28 Andrey Gandman , Lev Chuntonov , Leonid Rybak , Zohar Amitay

The development of high-intensity ultrashort laser pulses unlocks the potential of pump-probe spectroscopy in sub-femtosecond timescale. Notably, subcycle pump pulses can generate electronic states unreachable by conventional multicycle…

Strongly Correlated Electrons · Physics 2025-06-17 Kazuya Shinjo , Shigetoshi Sota , Seiji Yunoki , Takami Tohyama

We study the emission spectrum and absorption spectrum of a quantum emitter when it is driven by various pulse sequences. We consider the Uhrig sequence of $\pi_x$ pulses, the periodic sequence of $\pi_x\pi_y$ pulses and the periodic…

Quantum Physics · Physics 2018-04-25 Herbert F Fotso

A theory of pump-probe spectroscopy is developed in which optical fields drive two-quantum, Raman-like transitions between ground state sublevels. Three fields are incident on an ensemble of atoms. Two of the fields act as the pump field…

Atomic Physics · Physics 2009-11-06 P. R. Berman , B. Dubetsky

Dispersion and absorption properties of a weak probe field in a three-level V-type atomic system is studied. By application of indirect incoherent pump fields the effect of populating upper levels on optical properties of the atomic medium…

Quantum Physics · Physics 2010-05-20 Khaled Saaidi , Bahareh Ruzbahani , S. Worya Rabiei , Mohammad Mahmoudi

In this paper, we present a theoretical simulation of 87Rb absorption spectrum in a thermal cm-cell which is adaptive to the experimental observation. In experiment, the coupling and probe beams are configured to copropagate but…

Atomic Physics · Physics 2017-03-09 Hong Cheng , Shan-Shan Zhang , Pei-Pei Xin , Yuan Cheng , Hong-Ping Liu

Optical pump-probe spectroscopy is a powerful tool for the study of non-equilibrium electronic dynamics and finds wide applications across a range of fields, from physics and chemistry to material science and biology. However, a shortcoming…

The physical interpretation of time-resolved photoabsorption experiments is not as straightforward as for the more conventional photoabsorption experiments conducted on equilibrium systems. In fact, the relation between the transient…

Atomic Physics · Physics 2015-06-24 E. Perfetto , G. Stefanucci

Standard optical pump-probe methods analyze a system's temporal response to a laser pulse within sub-femtoseconds to several nanoseconds, constrained by the optical delay line's length. While resistance is a sensitive detector in various…

Instrumentation and Detectors · Physics 2024-04-26 M. I. Blumenau , A. Yu. Kuntsevich