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We present a statistical model of a dilute polymer solution in good solvent in the presence of low-molecular weight cosolvent. We investigate the conformational changes of the polymer induced by a change of the cosolvent concentration and…

Statistical Mechanics · Physics 2014-11-10 Yu. A. Budkov , A. L. Kolesnikov , N. Georgi , M. G. Kiselev

We calculate the plateau moduli of several single-chain slip-link and slip-spring models for entangled polymers. In these models, the entanglement effects are phenomenologically modeled by introducing topological constraints such as…

Soft Condensed Matter · Physics 2023-01-20 Takashi Uneyama , Yuichi Masubuchi

Mechanically interlocked polymers (MIPs) are a novel class of polymer structures in which the components are connected by mechanical bonds instead of covalent bonds. We measure the single-molecule rheological properties of polyrotaxanes,…

Soft Condensed Matter · Physics 2025-12-19 Ali Seyedi , Alex Albaugh

The effect of fluctuating internal viscosity and hydrodynamic interactions on a range of rheological properties of dilute polymer solutions is examined using a finitely extensible dumbbell model for a polymer. Brownian dynamics simulations…

Soft Condensed Matter · Physics 2020-07-03 R. Kailasham , Rajarshi Chakrabarti , J. Ravi Prakash

Discrete mesoscale network models, in which explicitly modeled polymer chains are replaced by implicit pairwise potentials, are capable of predicting the macroscale mechanical response of polymeric materials such as elastomers and gels,…

Soft Condensed Matter · Physics 2024-07-16 Robert J. Wagner , Meredith N. Silberstein

We have developed a dynamic self-consistent field theory, without any adjustable parameters, for unentangled polymer blends under shear. Our model accounts for the interaction between polymers, and enables one to compute the evolution of…

Soft Condensed Matter · Physics 2009-11-10 Tak Shing Lo , Maja Mihajlovic , Yitzhak Shnidman , Wentao Li , Dilip Gersappe

Using the volume averaging technique of Jackson (1997), we derive a set of two-fluid equations that describe the dynamics of a mono-disperse non-Brownian colloidal suspension in the semi-dilute regime. The equations are tensorial and can be…

Fluid Dynamics · Physics 2025-01-06 Dalton J. E. Harvie

We study the stress distribution in a polymer brush material over a range of graft densities using molecular dynamics (MD) simulations and theory. Flexible polymer chains are treated as beads connected by nonlinear springs governed by a…

Applied Physics · Physics 2019-03-27 M. Manav , M. Ponga , A. Srikantha Phani

Non-equilibrium Markov State Modeling (MSM) has recently been proposed [Phys. Rev. E 94, 053001 (2016)] as a possible route to construct a physical theory of sliding friction from a long steady state atomistic simulation: the approach…

Statistical Mechanics · Physics 2017-10-17 M. Teruzzi , F. Pellegrini , A. Laio , E. Tosatti

Time-lapse microscopy imaging provides direct access to the dynamics of soft and living systems. At mesoscopic scales, such microscopy experiments reveal intrinsic fluctuations, which may have both thermal and non-equilibrium origins. These…

Biological Physics · Physics 2020-12-02 F. S. Gnesotto , G. Gradziuk , P. Ronceray , C. P. Broedersz

A simple mean-field micro-swimmer model is presented. The model is inspired by the nonequilibrium thermodynamics of multi-component fluids that undergo chemical reactions. These thermodynamics can be rigorously described in the context of…

Soft Condensed Matter · Physics 2022-08-16 Andrés Córdoba , Jay D. Schieber , Tsutomu Indei

The theory to reconstruct the atomistic-level chain diffusion from the accelerated dynamics that is measured in mesoscale simulations of the coarse-grained system, is applied here to the dynamics of cis-1,4-Polybutadiene melts where each…

Soft Condensed Matter · Physics 2015-06-12 I. Y. Lyubimov , M. G. Guenza

In this paper, we consider a diffuse-interface gas-liquid two-phase flow model with inhomogeneous temperatures, in which we employ the Peng-Robinson equation of state and the temperature-dependent influence parameter instead of the van der…

Numerical Analysis · Mathematics 2018-08-01 Jisheng Kou , Shuyu Sun

Active polymeric systems exhibit a rich spectrum of non-equilibrium phenomena arising from stochastic forces that explicitly break detailed balance. Despite the rapid growth of experimental and numerical studies, analytical progress remains…

Soft Condensed Matter · Physics 2026-03-09 Takahiro Sakaue , Enrico Carlon

Computer simulations are used to characterize the entropic force of one or more polymers tethered to the tip of a hard conical object that interact with a nearby hard flat surface. Pruned-enriched-Rosenbluth-method (PERM) Monte Carlo…

Soft Condensed Matter · Physics 2022-08-31 James M. Polson , Roland G. MacLennan

Molecular dynamics simulations of a short-chain polymer melt between two brush-covered surfaces under shear have been performed. The end-grafted polymers which constitute the brush have the same chemical properties as the free chains in the…

Soft Condensed Matter · Physics 2016-08-31 Claudio Pastorino , Torsten Kreer , Marcus Mueller , Kurt Binder

Nucleic acids have been regarded as stiff polymers with long-range flexibility and generally modeled using elastic rod models of polymer physics. Notwithstanding, investigations carried out over the past few years on single fragments of…

Soft Condensed Matter · Physics 2025-05-09 Marco Zoli

Flutter stability is a dominant design constraint of modern gas and steam turbines. To further increase the feasible design space, flutter-tolerant designs are currently explored, which may undergo Limit Cycle Oscillations (LCOs) of…

Computational Engineering, Finance, and Science · Computer Science 2021-02-12 Christian Berthold , Johann Gross , Christian Frey , Malte Krack

We study theoretically a model system of a transient network of microemulsion droplets connected by telechelic polymers and explain recent experimental findings. Despite the absence of any specific interactions between either the droplets…

Soft Condensed Matter · Physics 2009-11-10 A. Zilman , J. Kieffer , F. Molino , G. Porte , S. Safran

We consider a model mixture of hard colloidal spheres and non-adsorbing polymer chains in a theta solvent. The polymer component is modelled as a polydisperse mixture of effective spheres, mutually noninteracting but excluded from the…

Soft Condensed Matter · Physics 2009-11-10 A. R. Denton , M. Schmidt