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The order-disorder transition of a sphere-forming block copolymer thin film was numerically studied through a Cahn-Hilliard model. Simulations show that the fundamental mechanisms of pattern formation are spinodal decomposition and…

Soft Condensed Matter · Physics 2017-08-28 Leopoldo R. Gómez , Nicolás A. García , Richard A. Register , Daniel A. Vega

We compare two theoretical approaches to dielectric diblock copolymer melts in an external electric field. The first is a relatively simple analytic expansion in the relative copolymer concentration, and includes the full electrostatic…

Soft Condensed Matter · Physics 2012-01-31 Yoav Tsori , David Andelman , Chin-Yet Lin , M. Schick

Using detailed atomistic simulations,we explore the conformational landscape of aggregates formed by biomimetic antimicrobial(AM) binary methacrylate copolymers,with hydrophobic and charged functional groups and the role of inclusion of…

Soft Condensed Matter · Physics 2020-02-25 Garima Rani , Kenichi Kuroda , Satyavani Vemparala

The phase behavior of linear dendritic triblock copolymer melts(AB2C4) is studied by self-consistent-field theory (SCFT) in order to find the effects of branching on the phase behavior of ABC linear triblock copolymer melts. We focus on a…

Soft Condensed Matter · Physics 2023-09-19 Danyang Chen , Xiaowei Ning

Polymeric micelles are used in a variety of applications, with the micelle's shape often playing an important role. Consequently, a scheme to design micelles of arbitrary shape is desirable. In this paper, we consider micelles formed from a…

Soft Condensed Matter · Physics 2018-03-16 Brian Moths

We report numerical simulation of the deposition of spherical particles on a planar surface, by ballistic, straight-line trajectory transport, and assuming irreversible adhesion on contact with the surface or previously deposited particles.…

Condensed Matter · Physics 2014-10-13 B. D. Lubachevsky , V. Privman , S. C. Roy

The elastic property of membranes self-assembled from AB diblock and ABA triblock copolymers, as coarse-grained model of lipids and the bolalipids, are studied using the self-consistent field theory (SCFT). Specifically, solutions of the…

Soft Condensed Matter · Physics 2019-05-17 Rui Xu , Ashkan Dehghan , An-Chang Shi , Jiajia Zhou

Supramolecular block copolymers (SBC) consist of covalent polymer building blocks that are connected into well-defined architectures via supramolecular bonds. Assisted by the dynamic and reversible supramolecular interactions, it is…

Soft Condensed Matter · Physics 2025-04-03 Xiangyu Zhang , Dong Meng

We apply monomer-resolved computer simulations of supercoiled ring polymers under shear, taking full account of the hydrodynamic interactions, accompanied, in parallel, by simulations in which these are switched off. The combination of…

Soft Condensed Matter · Physics 2024-04-17 Christoph Schneck , Jan Smrek , Christos N. Likos , Andreas Zöttl

The phase behavior of colloidal particles embedded in a binary fluid is influenced by wetting layers surrounding each particle. The free energy of the fluid film depends on its morphology, i.e., on size, shape and connectivity. Under rather…

Soft Condensed Matter · Physics 2007-05-23 Uwe Brodatzki , Klaus Mecke

The bending rigidity $k_c$ of bilayer vesicles self-assembled from amphiphilic diblock copolymers has been measured using single and dual-micropipet techniques. These copolymers are nearly a factor of 5 greater in hydrophobic membrane…

Soft Condensed Matter · Physics 2007-05-23 H. Bermudez , D. A. Hammer , D. E. Discher

In recent experiments, small, thick-walled vesicles with a narrow size distribution were formed from copolymers where the degree of polymerisation of the hydrophobic block, N_B, was significantly greater than that of the hydrophilic block,…

Soft Condensed Matter · Physics 2017-09-12 M. J. Greenall

Amorphous silica ($a-SiO_2$) is a widely used inorganic material. Interestingly, the relationship between the local atomic structures of $a-SiO_2$ and their effects on ductility and fracture is seldom explored. Here, we combine large-scale…

Mesoscale and Nanoscale Physics · Physics 2023-04-17 Jiahao Liu , Jingjie Yeo

We present a hybrid simulation method which allows one to study the dynamical evolution of self-assembling (co)polymer solutions in the presence of hydrodynamic interactions. The method combines an established dynamic density functional…

Soft Condensed Matter · Physics 2018-04-10 Johannes Heuser , G. J. Agur Sevink , Friederike Schmid

A simple phenomenological model for describing the conformational dynamics of biological macromolecules via the nonlinearity-induced instabilities is proposed. It is shown that the interaction between charges and bending degrees of freedom…

Soft Condensed Matter · Physics 2009-11-11 Yu. B. Gaididei , P. L. Christiansen , W. J. Zakrzewski

The linear and non-linear dynamic response to an oscillatory shear flow of giant wormlike micelles consisting of Pb-Peo block copolymers is studied by means of Fourier transform rheology. Experiments are performed in the vicinity of the…

Soft Condensed Matter · Physics 2009-11-13 B. Lonetti , J. Kohlbrecher , L. Willner , J. K. G. Dhont , M. P. Lettinga

The role of particle shape in evaporation-induced auto-stratification in dispersed colloidal suspensions is explored with molecular dynamics simulations of mixtures of solid spheres, aspherical particles, and hollow spheres. A unified…

Soft Condensed Matter · Physics 2025-02-25 Binghan Liu , Gary S. Grest , Shengfeng Cheng

Modeling the atomic structure of amorphous materials has long been a critical challenge in materials science. Recent advances in monolayer amorphous materials enable direct observation of their atomic structures, paving the way for a better…

Materials Science · Physics 2026-05-05 Le-Ye Zhu , Xi Zhang , Yun-Peng Wang , Jieheng Shi , Junwei Zhang , Shixuan Du , Yu-Yang Zhang

Adsorption of a symmetric (AB) random copolymer (RC) onto a symmetric (ab) random heterogeneous surface (RS) is studied in the annealed approximation by using a two-dimensional partially directed walk model of the polymer. We show that in…

Soft Condensed Matter · Physics 2015-06-15 A. A. Polotsky

The properties of diluted symmetric A-B diblock copolymers at the interface between A and B homopolymer phases are studied by means of Monte Carlo (MC) simulations of the bond fluctuation model. We calculate segment density profiles as well…

Chemical Physics · Physics 2015-06-26 A. Werner , F. Schmid , K. Binder , M. Mueller