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Successful phase-matching methods for Third Harmonics Generation (THG) include phase-matching in birefringent crystal and quasi-phase-matching (QPM) in crystal with periodically poled domains. However, these methods are not feasible in some…

Optics · Physics 2013-07-25 Tan Yizhou , Yang Yisheng , Liao Jiali , Zhang Ming

Thin film interference is integral to modern photonics and optoelectronics, e.g. allowing for precise design of high performance optical filters, efficiency enhancements in photovoltaics and light-emitting devices, as well as the…

We explore the electroluminescence efficiency for a quantum mechanical model of a large number of molecular emitters embedded in an optical microcavity. We characterize the circumstances under which a microcavity enhances harvesting of…

Mesoscale and Nanoscale Physics · Physics 2019-09-04 Luis A. Martínez-Martínez , Elad Eizner , Stéphane Kéna-Cohen , Joel Yuen-Zhou

Metasurfaces have emerged as a promising platform for integrated nonlinear optics. Nonlocal metasurfaces enable high nonlinear conversion efficiency, while the local ones can offer versatile wavefront control, yet achieving both within a…

Optics · Physics 2026-02-03 Yu Tian , Nuo Wang , Qi Liu , Shuyuan Xiao , Tingting Liu , Olivier J. F. Martin , Ying Gu

We experimentally demonstrate efficient third harmonic generation from an indium tin oxide (ITO) nanofilm (lambda/42 thick) on a glass substrate for a pump wavelength of 1.4 um. A conversion efficiency of 3.3x10^-6 is achieved by exploiting…

Optical microcavities and metallic nanostructures have been shown to significantly modulate the dynamics and spectroscopic response of molecular systems. We present a study of the nonlinear optics of a model consisting of $N$ anharmonic…

Photonic integrated circuits are emerging as a key technology for compact and energy-efficient optical information processing. Yet, their practical implementation remains limited by the intrinsically weak optical nonlinearities of…

We propose an unconventional scheme of photoluminescence in a semiconductor thin film, where the nonlocal correlation between an excitonic wave and a light wave prominently enhances the exciton-light coupling beyond the long-wavelength…

Mesoscale and Nanoscale Physics · Physics 2016-04-15 Takuya Matsuda , Nobuhiko Yokoshi , Hajime Ishihara

Nonlinear metasurfaces have become prominent tools for controlling and engineering light at the nanoscale. Usually, the polarization of the total generated third harmonic is studied. However, diffraction orders may present different…

We explore the nonlinear response of tailor-cut light-matter hybrid states in a novel regime, where both the Rabi frequency induced by a coherent driving field and the vacuum Rabi frequency set by a cavity field are comparable to the…

Quantum Physics · Physics 2021-05-05 J. Mornhinweg , M. Halbhuber , C. Ciuti , D. Bougeard , R. Huber , C. Lange

Ultrafast nonlinear photonics enables a host of applications in advanced on-chip spectroscopy and information processing. These rely on a strong intensity dependent (nonlinear) refractive index capable of modulating optical pulses on…

Strong coupling between light and matter in an optical cavity provides a pathway to giant polariton nonlinearity, where effective polariton-polariton interactions are mediated by materials' nonlinear responses. The pursuit of such enhanced…

Optics · Physics 2024-11-26 Zhi Wang , Li He , Bumho Kim , Bo Zhen

We report on time-resolved ultrafast terahertz third-harmonic generation spectroscopy of nonequilibrium dynamics of Weyl fermions in a nanometer thin film of the Weyl semimetal TaP. Terahertz third-harmonic generation is observed at room…

Strongly Correlated Electrons · Physics 2025-11-26 Patrick Pilch , Changqing Zhu , Sergey Kovalev , Renato M. A. Dantas , Amilcar Bedoya-Pinto , Stuart S. P. Parkin , Zhe Wang

The ultrastrong light-matter interaction regime was investigated in metallic and superconducting complementary split ring resonators coupled to the cyclotron transition of two dimensional electron gases. The sub-wavelength light confinement…

Heavily doped semiconductors have emerged as tunable low-loss plasmonic materials at mid-infrared frequencies. In this article we investigate nonlinear optical phenomena associated with high concentration of free electrons. We use a…

Optics · Physics 2021-03-17 Federico De Luca , Michele Ortolani , Cristian Ciracì

Harmonic generation is a general characteristic of driven nonlinear systems, and serves as an efficient tool for investigating the fundamental principles that govern the ultrafast nonlinear dynamics. In atomic gases, high-harmonic radiation…

We present a combined experimental and theoretical study of nonlinear light-matter interactions in a three-dimensional gold-polymer hybrid metasurface. In contrast to conventional two-dimensional designs, which by symmetry may support…

Molecular polaritons are hybrid states of photonic and molecular character that form when molecules strongly interact with light. Strong coupling tunes energy levels and importantly, can modify molecular properties (e.g. photoreaction…

Chemical Physics · Physics 2023-02-14 Francesca Fassioli , Kyu Hyung Park , Sarah E. Bard , Gregory D. Scholes

The polariton, a quasiparticle formed by strong coupling of a photon to a matter excitation, is a fundamental ingredient of emergent photonic quantum systems ranging from semiconductor nanophotonics to circuit quantum electrodynamics.…

Quantum Gases · Physics 2024-03-21 Joonhyuk Kwon , Youngshin Kim , Alfonso Lanuza , Dominik Schneble

We reveal a novel regime of photon-pair generation driven by the interplay of multiple bound states in the continuum resonances in nonlinear metasurfaces. This non-degenerate photon-pair generation is derived from the hyperbolic topology of…