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We calculate linear and nonlinear optical susceptibilities arising from the excitonic states of mono- layer MoS2 for in-plane light polarizations, using second-quantized bound and unbound exciton operators. Optical selection rules are…

Mesoscale and Nanoscale Physics · Physics 2018-04-11 Daniel B. S. Soh , Christopher Rogers , Dodd J. Gray , Eric Chatterjee , Hideo Mabuchi

Optical selection rule fundamentally determines the optical transition between energy states in a variety of physical systems from hydrogen atoms to bulk crystals such as GaAs. It is important for optoelectronic applications such as lasers,…

Materials Science · Physics 2016-04-01 Jun Xiao , Ziliang Ye , Ying Wang , Hanyu Zhu , Yuan Wang , Xiang Zhang

Interlayer valley excitons in bilayer MoS2 feature concurrently large oscillator strength and long lifetime, and hence represent an advantageous scenario for valleytronic applications. However, control of valley pseudospin of interlayer…

We show that excitons and free carriers in K and K' valleys of transition metal dichalcogenide monolayers can be entangled with respect to their valley degree of freedom by absorbing linearly polarized single photons. This effect does not…

Mesoscale and Nanoscale Physics · Physics 2015-08-12 Mikhail Tokman , Yongrui Wang , Alexey Belyanin

The modulation of the valley structure in two-dimensional valley materials is vital in the field of valleytronics. The multiferroicity provides possibility for multiple modulations of the valley, including the magnetic and electric means.…

Materials Science · Physics 2023-07-10 Huiqian Wang , Li Liang , Xiaohui Wang , Xiaoyu Wang , Xiao Li

The coupled spin-valley physics in transition metal dichalcogenides (TMDs) endows exciton states with valley degrees of freedom, making them promising for valleytronic applications in TMDs monolayers and/or their heterostructures. Although…

Applied Physics · Physics 2022-12-07 Yingying Chen , Zeyi Liu , Junchao Hu , Junze Li , Wendian Yao , Dehui Li

Transition metal dichalcogenide (TMD) monolayers are two-dimensional semiconductors with two valleys in their band structure that can be selectively addressed using circularly polarized light. Their photoluminescence spectrum is…

Mesoscale and Nanoscale Physics · Physics 2020-10-26 Joris J. Carmiggelt , Michael Borst , Toeno van der Sar

Local energy extrema of the bands in momentum space, or valleys, can endow electrons in solids with pseudo-spin in addition to real spin. In transition metal dichalcogenides this valley pseudo-spin, like real spin, is associated with a…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Grant Aivazian , Zhirui Gong , Aaron M Jones , Rui-Lin Chu , Jiaqiang Yan , David G Mandrus , Chuanwei Zhang , David Cobden , Wang Yao , Xiaodong Xu

Monolayered MoSe2 is a promising new material to investigate advanced light-matter coupling as it hosts stable and robust excitons with comparably narrow optical resonances. In this work, we investigate the evolution of the lowest lying…

Mesoscale and Nanoscale Physics · Physics 2017-03-28 N. Lundt , A. Maryński , E. Cherotchenko , A. Pant , X. Fan , G. Sęk , S. Tongay , A. V. Kavokin , S. Höfling , C. Schneider

We investigate the interaction of excitons in a two dimensional lattice and photons in a planar cavity in the presence of disorder. The strong exciton-photon coupling is described in terms of polariton quasi-particles, which are scattered…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Michal Grochol , Carlo Piermarocchi

Degenerate extrema in the energy dispersion of charge carriers in solids, also referred to as valleys, can be regarded as a binary quantum degree of freedom, which can potentially be used to implement valleytronic concepts in van der Waals…

Photoluminescence (PL) of transition metal dichalcogenide (TMD) monolayers is strongly influenced by the dielectric environment. The defect states present in the substrate induces uncontrollable doping in the TMD monolayer and thereby…

The robust spin and momentum valley locking of electrons in two-dimensional semiconductors make the valley degree of freedom of great utility for functional optoelectronic devices. Owing to the difference in optical selection rules for the…

The origin of the variation of photoluminescence (PL) spectra of monolayer tungsten disulfide (WS2) is investigated systematically. Dependence of the PL spectrum on the excitation power show that the relatively sharp component corresponds…

Mesoscale and Nanoscale Physics · Physics 2018-06-01 Yongjae Kwon , Kangwon Kim , Wontaek Kim , Sunmin Ryu , Hyeonsik Cheong

High degree of valley polarization of optically active excitons in transition-metal dichalcogenide monolayers (TMD-MLs) is vital in valley-based photonic applications but known to be likely spoiled by the intrinsic electron-hole exchange…

Mesoscale and Nanoscale Physics · Physics 2021-06-15 Ping-Yuan Lo , Guan-Hao Peng , Wei-Hua Li , Yi Yang , Shun-Jen Cheng

The optical spectra of transition metal dichalcogenide (TMDC) monolayers are dominated by excitons and trions. Here we establish the dependences of these optical transitions on disorder from hyperspectral imaging of h-BN encapsulated…

Mesoscale and Nanoscale Physics · Physics 2022-12-13 Jue Wang , Christina Manolatou , Yusong Bai , James Hone , Farhan Rana , Xiaoyang Zhu

Using temperature dependent photoluminescence (PL), polarization resolved PL and Raman spectroscopy, we investigate the effect of in situ vacuum annealing as well as the relaxation of strain on the luminescence and the valley polarization…

Materials Science · Physics 2022-12-09 Poulab Chakrabarti , Faiha Mujeeb , Subhabrata Dhar

Momentum-indirect excitons composed of electrons and holes in different valleys define optoelectronic properties of many semiconductors, but are challenging to detect due to their weak coupling to light. The identification of an excitons'…

Integrating 2D materials into high-quality optical microcavities opens the door to fascinating many-particle phenomena including the formation of exciton-polaritons. These are hybrid quasi-particles inheriting properties of both the…

Mesoscale and Nanoscale Physics · Physics 2024-01-10 Beatriz Ferreira , Roberto Rosati , Jamie M. Fitzgerald , Ermin Malic

Monolayers of transition metal dichalcogenides (TMdC) are promising candidates for realization of a new generation of optoelectronic devices. The optical properties of these two-dimensional materials, however, vary from flake to flake, or…

Materials Science · Physics 2020-01-22 Pavel V. Kolesnichenko , Qianhui Zhang , Changxi Zheng , Michael S. Fuhrer , Jeffrey A. Davis