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Systematic Raman experiments performed on water and water-ethanol samples, stored in different containers (fused silica, polypropylene, soda-lime glass type III) for several hours, have shown that the luminescence contribution to the Raman…

Raman-based technologies have enabled many ground-breaking scientific discoveries related to surface science, single molecule chemistry and biology. For example, researchers have identified surface bound molecules by their Raman vibrational…

Optics · Physics 2020-03-12 Xiaoqin Shen , Hyungwoo Choi , Dongyu Chen , Wei Zhao , Andrea M. Armani

In this paper we discuss the field enhancement due to surface plasmons resonances of metallic nanostructures, in particular nano spheres on top of a metal, and find maximum field enhancement of the order of 10^2, intensities enhancement of…

Mesoscale and Nanoscale Physics · Physics 2012-12-06 Nicolas Garcia , Ming Bai

We theoretically investigate the interaction between a single molecule and a metallic nanoparticle. We develop a general quantum mechanical description for the calculation of the enhancement of radiative and non-radiative decay channels for…

Mesoscale and Nanoscale Physics · Physics 2008-01-28 Ulrich Hohenester , Andreas Truegler

A surrounding electromagnetic environment can engineer spontaneous emissions from quantum emitters through the Purcell effect. For instance, a plasmonic antenna can efficiently confine an electromagnetic field and enhance the fluorescent…

Optics · Physics 2021-12-22 Jingyi Zhao , Weidong Zhang , Te Wen , Lulu Ye , Hai Lin , Jinglin Tang , Qihuang Gong , Guowei Lu

We extend Lamb's reduced density matrix laser theory to analyze the inhomogeneous molecular couplings and the mode-correlation in a plasmonic nano-laser consisting of a gold sphere and many dye molecules interacting with a driving optical…

Optics · Physics 2017-04-27 Yuan Zhang , Klaus Mølmer

We propose a method for increasing the Raman scattering from an ensemble of molecules by up to four orders of magnitude. Our method requires an additional coherent source of IR radiation with the half-frequency of the Stokes shift. This…

Quantum Physics · Physics 2019-04-24 V. Yu. Shishkov , E. S. Andrianov , A. A. Pukhov , A. P. Vinogradov , A. A. Lisyansky

A tri-layer metamaterial perfect absorber of light, consisting of (Al/ZnS/Al) films with the top aluminium layer patterned as an array of circular disk nanoantennas, is investigated for resonantly enhancing Raman scattering from C-60…

Optics · Physics 2018-11-02 Sriram Guddala , Narayanarao Desai , S. Anantha Ramakrishna

Microscopic pyramidal pits in a reflective surface, a geometry similar to a retroreflector, are frequently used to enhance signal strength. The enhancement effect is generally attributed to surface plasmons, however, the sub-wavelength to…

Optics · Physics 2009-12-18 M. Mechler , S. V. Kukhlevsky , A. Mechler , D. McNaughton

Localized plasmons in metallic nanostructures have been widely used to enhance nonlinear optical effects due to their ability to concentrate and enhance light down to extreme-subwavelength scales. As alternatives to noble metal…

Mesoscale and Nanoscale Physics · Physics 2015-02-24 Joel D. Cox , F. Javier Garcia de Abajo

Photonic nanostructures provide means of tailoring the interaction between light and matter and the past decade has witnessed a tremendous experimental and theoretical progress in this subject. In particular, the combination with…

Quantum Physics · Physics 2015-06-05 Peter Lodahl , Sahand Mahmoodian , Søren Stobbe

A chiral near field with a highly contorted electromagnetic field builds a bridge to match the chiral molecules and light wavelengths with large size differences. It significantly enhances the circular dichroism of chiral molecules and has…

Optics · Physics 2022-03-23 Li Hu , Zhiguang Sun , Yingdong Nie , Yingzhou Huang , Yurui Fang

We have studied the plasmonic properties of aperiodic arrays of identical nanoparticles (NPs) formed by two opposite and equal graded-chains (a chain where interactions change gradually). We found that these arrays concentrate the external…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 Natalia Esteves-López , Horacio M. Pastawski , Raúl A. Bustos-Marún

Photoluminescence from a gold nanotip, which is induced by surface plasmons propagating over a curved tapered nanotip surface is considered in a co-moving accelerated reference frame. Similar to the surface-enhanced Raman scattering (SERS)…

Strongly Correlated Electrons · Physics 2008-11-11 Igor I. Smolyaninov

Single-molecule detection with chemical specificity is a powerful and much desired tool for biology, chemistry, physics, and sensing technologies. Surface-enhanced spectroscopies enable single molecule studies, yet reliable substrates of…

Mesoscale and Nanoscale Physics · Physics 2008-02-22 D. R. Ward , N. K. Grady , C. S. Levin , N. J. Halas , Y. Wu , P. Nordlander , D. Natelson

Conventional approaches to control and shape the scattering patterns of light generated by different nanostructures are mostly based on engineering of their electric response due to the fact that most metallic nanostructures support…

Optics · Physics 2014-05-05 Wei Liu , Andrey E. Miroshnichenko , Yuri S. Kivshar

The implementation of non-classical light sources is becoming increasingly important for various quantum applications. A particularly interesting approach is to integrate such functionalities on a single chip as this could pave the way…

Optics · Physics 2018-06-27 Frédéric Peyskens , Dirk Englund

The plasmon resonances (modes) of a metal nanostructure can be defined as a dipole, a quadrupole, or high-order modes depending on the surface charge distribution induced by the incident field. In a non-symmetrical environment or clusters,…

It is known that the more tractable Markovian models of coupling suited for weak interactions may overestimate the Rabi frequency notably when applied to the strong-coupling regime. Here, a more significant consequence of the non-Markovian…

Optics · Physics 2022-05-24 Kritika Jain , Murugesan Venkatapathi

Subwavelength aperture arrays in thin metal films can enable enhanced transmission of light and matter (atom) waves. The phenomenon relies on resonant excitation and interference of the plasmon or matter waves on the metal surface. We show…

Optics · Physics 2009-11-13 S. V. Kukhlevsky