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Microparticle laser fragmentation in liquids has emerged as a promising approach to generate nanoparticles with high efficiency. Despite its advantages, the underlying fragmentation mechanisms, their connection to the nanoparticle size…
Thermo-osmosis refers to fluid migration due to temperature gradient. The mechanistic understanding of thermo-osmosis in charged nano-porous media is still incomplete, while it is important for several environmental and energy applications,…
Microscopic pathways of structural phase transitions are difficult to probe because they occur over multiple, disparate time and length scales. Using $in$ $situ$ nanoscale cathodoluminescence microscopy, we visualize the thermally-driven…
The absorptivity of a material is a major uncertainty in numerical simulations of laser welding and additive manufacturing, and its value is often calibrated through trial-and-error exercises. This adversely affects the capability of…
Laser excitation has emerged as a means to expose hidden states of matter and promote phase transitions on demand. Such laser induced transformations are often rendered possible owing to the delivery of spatially and/or temporally…
This thesis is focused on numerical simulations of the laser interaction with porous materials. A possibility of well-controlled processing is particularly important for the laser based micro-structuring of porous glass and nano-machining…
Exploiting the emerging nanoscale periodicities in epitaxial, single-crystal thin films is an exciting direction in quantum materials science: confinement and periodic distortions induce novel properties. The structural motifs of interest…
Control over the properties of nanoparticles obtained by laser ablation in liquids is experimentally demonstrated via modulation of the beam intensity profile on the target. Mask projection scheme was used with either a copper laser…
Femtosecond laser surface processing (FLSP) is an emerging fabrication technique to efficiently control the surface morphology of many types of materials including metals. However, the theoretical understanding of the FLSP formation…
This work reports on the fabrication of microbump structures on Ni films by single-pulse, localized laser irradiation. Conditions for the reproducible formation of such microstructures have been identified in terms of laser-irradiation and…
The fluid dynamics of the classical dewetting instability in ultrathin films is a non-linear process. However, the physical manifestation of the instability in terms of characteristic length and time scales can be described by a linearized…
We use ab-initio electromagnetic simulations to investigate light absorption by rough surfaces in the context of the formation of laser-induced periodic surface structures. Our approach involves modeling a realistic rough surface using a…
We investigate nanoscale friction in [LaMnO3]m/[SrMnO3]n superlattice films using lateral force microscopy, focusing on the effects of fluorine doping and top-layer thickness. For all samples, friction forces scale linearly with the sum of…
Ultrafast laser ablation is an extremely precise and clean method of removing material, applied in material processing as well as medical applications. And due to its violent nature, it tests our understanding of the interplay between…
We present topological derivative and energy based procedures for the imaging of micro and nanostructures using one beam of visible light of a single wavelength. Objects with diameters as small as 10 nm can be located, and their position…
A theory of lasing in a two-dimensional array of metal nanoparticles (MNPs) covered with a thin layer of fluorescent molecules is developed from first principles. The approach is based on a rigorous account of the local field in a close…
We analyze thermodynamics of water samples confined in nanopores and prove that although the freezing temperature can be dramatically lower, the suppression of the ice nucleation leading to the freezing temperature depression is a truly…
Due to its extremely short timescale, the non-equilibrium melting of metals is exceptionally difficult to probe experimentally. The knowledge of melting mechanisms is thus based mainly on the results of theoretical predictions. This work…
Active topological photonic systems enable robust light control and new pathways for semiconductor lasing. However, their intrinsically non-Hermitian nature, combining gain, radiation leakage, and material loss, makes the underlying physics…
We study the free-surface deformation dynamics of an immersed glassy thin polymer film supported on a substrate, induced by an air nanobubble at the free surface.We combine analytical and numerical treatments of the glassy thin film…