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The pursuit of ever-shorter time scales is a frontier in modern physics, exemplified by the synthesis of attosecond light pulses -- an achievement made possible by coherently superimposing a broad range of photon energies, as required by…

Mesoscale and Nanoscale Physics · Physics 2025-04-25 Xin Jin , Cruz I. Velasco , F. Javier García de Abajo

Diffraction imaging of non-equilibrium dynamics at atomic resolution is becoming possible with X-ray free-electron lasers. However, there are unresolved problems with applying this method to objects that are confined in only one dimension.…

Strongly Correlated Electrons · Physics 2018-02-19 Kenneth R. Beyerlein

A wide range of ultrafast phenomena in various atomic, molecular and condense matter systems is governed by electron dynamics. Therefore, the ability to image electronic motion in real space and real time would provide a deeper…

Atomic Physics · Physics 2018-02-27 Daria Popova-Gorelova

Metals exhibit nonequilibrium electron and lattice subsystems at transient times following femtosecond laser excitation. In the past four decades, various optical spectroscopy and time-resolved diffraction methods have been used to study…

Chemical Physics · Physics 2024-05-17 Xing He , Mithun Ghosh , Ding-Shyue Yang

Visualizing ultrafast dynamics at the atomic scale requires time-resolved pump-probe characterization with femtosecond temporal resolution. For single-shot ultrafast electron diffraction (UED) with fully relativistic electron bunch probes,…

Femtosecond electron bunches with keV energies and eV energy spread are needed by condensed matter physicists to resolve state transitions in carbon nanotubes, molecular structures, organic salts, and charge density wave materials. These…

We calculate the ferroelectric polarization dynamics induced by a femtosecond midinfrared pulse as measured in the recent experiment by R. Mankowsky et al., Phys. Rev. Lett. 118, 197601 (2017). It is due to the nonlinear coupling of the…

Materials Science · Physics 2020-01-15 Veniamin A. Abalmasov

The resolution of far-field optical microscopes, which rely on propagating optical modes, is widely believed to be limited because of diffraction to a value on the order of a half-wavelength $\lambda /2$ of the light used. Although…

Materials Science · Physics 2009-11-10 Igor I. Smolyaninov , Christopher C. Davis , Jill Elliott , Anatoly V. Zayats

In the last few decades the development of ultrafast lasers has revolutionized our ability to gain insight into light-matter interactions. The appearance of few-cycle light sources available from the visible to the mid-infrared spectral…

We have implemented a new approach for measuring the time-dependent intensity and phase of ultrashort optical pulses. It is based on the interaction between shaped pulses and atoms, leading to coherent transients.

Optics · Physics 2016-08-16 Antoine Monmayrant , Béatrice Chatel , Bertrand Girard

Femtosecond laser, owing to their ultrafast time scales and broad frequency bandwidths, have substantially changed fundamental science over the past decades, from chemistry and bio-imaging to quantum physics. Critically, many emerging…

Fabrication of large area (sub 1 cm cross-section) micro-optical components in a short period of time (approximately 10 min) and with lesser number of processing steps is highly desirable and cost-effective. In the recent years, femtosecond…

In analogy with optical near-field scanning methods, we use tapered dielectric waveguides as probes for a millimeter wave vector network analyzer. By scanning thin samples between two such probes we are able to map the spatially varying…

Soft Condensed Matter · Physics 2009-11-13 Nathan S. Greeney , John A. Scales

We report the development of an instrument combining an ultrafast, high-repetition-rate, polarization-tunable monochromatic extreme ultraviolet (XUV, 21.6 eV) beamline and a next-generation momentum microscope endstation. This setup enables…

Two-dimensional (2D) ferroelectric materials like NbOI$_{2}$ have garnered significant interest, yet their temporal response and synergetic interaction with light remain underexplored. Previous studies on the polarization of oxide…

Femtosecond laser pulses enable the synthesis of light across the electromagnetic spectrum and provide access to ultrafast phenomena in physics, biology, and chemistry. Chip-integration of femtosecond technology could revolutionize…

Ultra-fast transmission electron microscopy (UTEM) combines sub-picosecond time-resolution with the versatility of TEM spectroscopies. It allows one to study the dynamics of materials properties combining complementary techniques. However,…

Materials Science · Physics 2021-08-25 S. Meuret , L. H. G. Tizei , F. Houdellier , S. Weber , Y. Auad , M. Tencé , H. -C. Chang , M. Kociak , A. Arbouet

We use a new technique to disseminate microwave reference signals along ordinary optical fiber. The fractional frequency resolution of a link of 86 km in length is 10-17 for a one day integration time, a resolution higher than the stability…

Time-bin qubits, in which quantum information is encoded in a single photon at different times $\Delta$t, are suitable for long-distance transmission via optical fibers. However, detection of time-bin qubits has been limited to the…

Quantum Physics · Physics 2022-05-17 Yuta Kochi , Sunao Kurimura , Junko Ishi-Hayase

We propose a scheme for constructing a phase plate for use in an ultrafast Zernike-type phase contrast electron microscope, based on the interaction of the electron beam with a strongly focused, high-power femtosecond laser pulse and a…

Instrumentation and Detectors · Physics 2023-03-15 K. A. H. van Leeuwen , W. J. Schaap , B. Buijsse , S. Borelli , S. T. Kempers , W. Verhoeven , O. J. Luiten