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We develop a quantum-mechanical theory for Landau damping of surface plasmons in metal nanostructures larger that the characteristic length for nonlocal effects. We show that the electron surface scattering, which facilitates plasmon decay…

Mesoscale and Nanoscale Physics · Physics 2016-12-28 Tigran V. Shahbazyan

Nanoscale localization of electromagnetic fields near metallic nanostructures underpins the fundamentals and applications of plasmonics. The unavoidable energy loss from plasmon decay, initially seen as a detriment, has now expanded the…

Surface plasmon mediated hot carrier generation is widely utilized for the manipulation of the electron-photon interactions in many types of optoelectronic devices including solar cells, photodiodes, and optical modulators. A diversity of…

We demonstrate that ultrafast carrier excitation can drastically affect electronic structures and induce brief surface plasmonic response in non-plasmonic metals, potentially creating a plasmonic switch. Using first-principles molecular…

Optics · Physics 2016-04-20 E. Bévillon , J. P. Colombier , V. Recoules , H. Zhang , C. Li , R. Stoian

Alloyed metal nanoparticles are a promising platform for plasmonically enabled hot-carrier generation, which can be used to drive photochemical reactions. Although the non-plasmonic component in these systems has been investigated for its…

Mesoscale and Nanoscale Physics · Physics 2024-08-15 Jakub Fojt , Tuomas P. Rossi , Priyank V. Kumar , Paul Erhart

Metal nanoparticles are attractive for plasmon-enhanced generation of hot carriers, which may be harnessed in photochemical reactions. In this work, we analyze the coherent femtosecond dynamics of photon absorption, plasmon formation, and…

Mesoscale and Nanoscale Physics · Physics 2021-01-14 Tuomas P. Rossi , Paul Erhart , Mikael Kuisma

Hot charge carrier extraction from metallic nanostructures is a very promising approach for applications in photo-catalysis, photovoltaics and photodetection. One limitation is that many metallic nanostructures support a single plasmon…

This study examines the Raman scattering and charge transfer properties of molecules adsorbed on the surface of a tetrahedral Au$_{120}$ nanoparticle based on the time-dependent density functional tight-binding (TD-DFTB) method. We study…

Chemical Physics · Physics 2024-09-18 Sajal Kumar Giri , George C. Schatz

The coherent oscillations of mobile charge carriers near the surface of good conductors-surface plasmons-are been exploited in many applications in information technologies, clean energy, high-density data storage, photovoltaics, chemistry,…

Mesoscale and Nanoscale Physics · Physics 2023-12-20 Jacob Khurgin , Anton Yu. Bykov , Anatoly V. Zayats

Surface plasmon enhanced processes and hot-carrier dynamics in plasmonic nanostructures are of great fundamental interest to reveal light-matter interactions at the nanoscale. Using plasmonic tunnel junctions as a platform supporting both…

The collective response of metal nanostructures to optical excitation leads to localized plasmon generation with nanoscale field confinement driving applications in e.g. quantum optics, optoelectronics, and nanophotonics, where a bottleneck…

Formation of nanoscale laser-induced periodic surface structures on thin metal films (of the size of the optical penetration depth) is a yet unexplored area that is expected to open new routes for laser patterning and a wealth of exciting…

We discuss the effect of the local field polarization in metallic nanostructures where large field enhancements can be induced by excitation of localized surface plasmons. To demonstrate the importance of these effects, we study a few model…

Chemical Physics · Physics 2007-05-23 E. C. Le Ru , P. G. Etchegoin

Localized surface plasmons in metal nanoparticles are widely used in nano-optics to confine and enhance optical fields. It has been previously shown that, if the nanoparticles are distributed periodically, an additional enhancement can be…

Optics · Physics 2024-06-04 Xiaorun Zang , Andriy Shevchenko

Efficient generation of charge carriers from a metallic surface is a critical challenge in a wide variety of applications including vacuum microelectronics and photo-electrochemical devices. Replacing semiconductors with vacuum/gas as the…

Applied Physics · Physics 2018-05-09 Shiva Piltan , Dan Sievenpiper

Plasmonic absorption of light can lead to significant local heating in metallic nanostructures, an effect that defines the sub-field of thermoplasmonics and has been leveraged in diverse applications from biomedical technology to…

Mesoscale and Nanoscale Physics · Physics 2014-02-21 Joseph B. Herzog , Mark W. Knight , Douglas Natelson

The resonant scattering of surface plasmon-polariton waves by embedded semiconductor quantum dots above the dielectric/metal interface is explored in the strong-coupling regime. In contrast to non-resonant scattering by a localized…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Danhong Huang , Michelle Easter , Godfrey Gumbs , A. A. Maradudin , Shawn-Yu Lin , Dave Cardimona , Xiang Zhang

We have observed laser-like emission of surface plasmon polaritons (SPPs) decoupled to the glass prism in an attenuated total reflection setup. SPPs were excited by optically pumped molecules in a polymeric film deposited on the top of the…

Optics · Physics 2009-11-13 M. A. Noginov , G. Zhu , M. F. Mayy , B. A. Ritzo , N. Noginova , V. A. Podolskiy

We have investigated the plasmonic enhancement of the radiation field at various nanostructured multilayer devices, that may be applied in surface enhanced Raman spectroscopy. We apply an image dipole method to describe the effect of…

We investigate the scattering and absorption properties of anisotropic metal-dielectric core-shell nanoparticles. It is revealed that the radially anisotropic dielectric layer can accelerate the evanescent decay of the localized resonant…

Optics · Physics 2016-08-24 Wei Liu , Bing Lei , Andrey E. Miroshnichenko
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