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Breaking space-time symmetries in two-dimensional crystals (2D) can dramatically influence their macroscopic electronic properties. Monolayer transition-metal dichalcogenides (TMDs) are prime examples where the intrinsically broken crystal…

Mesoscale and Nanoscale Physics · Physics 2015-09-04 Edbert J. Sie , James W. McIver , Yi-Hsien Lee , Liang Fu , Jing Kong , Nuh Gedik

Increasing the speed limits of conventional electronics requires innovative approaches to manipulate other quantum properties of electrons besides their charge. An alternative approach utilizes the valley degree of freedom in…

Mesoscale and Nanoscale Physics · Physics 2023-03-29 A. O. Slobodeniuk , P. Koutenský , M. Bartoš , F. Trojánek , P. Malý , T. Novotný , M. Kozák

Charge carriers in two-dimensional transition metal dichalcogenides (TMDs), such as WSe$_2$, have their spin and valley-pseudospin locked into an optically-addressable index that is proposed as a basis for future information processing. The…

Mesoscale and Nanoscale Physics · Physics 2021-03-17 Weijie Li , Xin Lu , Jiatian Wu , Ajit Srivastava

Optical selection rule fundamentally determines the optical transition between energy states in a variety of physical systems from hydrogen atoms to bulk crystals such as GaAs. It is important for optoelectronic applications such as lasers,…

Materials Science · Physics 2016-04-01 Jun Xiao , Ziliang Ye , Ying Wang , Hanyu Zhu , Yuan Wang , Xiang Zhang

The ability to monitor and control distinct states is at the heart of emerging quantum technologies. The valley pseudospin in transition metal dichalcogenide (TMDC) monolayers is a promising degree of freedom for such control, with the…

The robust spin and momentum valley locking of electrons in two-dimensional semiconductors make the valley degree of freedom of great utility for functional optoelectronic devices. Owing to the difference in optical selection rules for the…

Interactions between two excitons can result in the formation of bound quasiparticles, known as biexcitons. Their properties are determined by the constituent excitons, with orbital and spin states resembling those of atoms. Monolayer…

Mesoscale and Nanoscale Physics · Physics 2015-09-23 Edbert J. Sie , Alex J. Frenzel , Yi-Hsien Lee , Jing Kong , Nuh Gedik

Monolayer (1L) transition metal dichalcogenides (TMDs) provide a unique opportunity to control the valley degree of freedom of optically excited charge carriers due to the spin-valley locking effect. Despite extensive studies of the…

A new degree of freedom, the valley pseudospin, emerges in atomically thin two-dimensional transition metal dichalcogenides (MX2) and has attracted great scientific interest. The capability to manipulate the valley pseudospin, in analogy to…

Mesoscale and Nanoscale Physics · Physics 2014-12-10 Jonghwan Kim , Xiaoping Hong , Chenhao Jin , Su-Fei Shi , Chih-Yuan S. Chang , Ming-Hui Chiu , Lain-Jong Li , Feng Wang

In monolayer Transition Metal Dichalcogenides (TMDs) the valence and conduction bands are spin split because of the strong spin-orbit interaction. In tungsten-based TMDs the spin-ordering of the conduction band is such that the so-called…

The coherent manipulation of spin and pseudospin underlies existing and emerging quantum technologies, including NMR, quantum communication, and quantum computation. Valley polarization, associated with the occupancy of degenerate, but…

Mesoscale and Nanoscale Physics · Physics 2017-02-01 Ziliang Ye , Dezheng Sun , Tony F. Heinz

Two-dimensional (2D) van-der-Waals materials are a promising platform for exciton state engineering. In this paper, we study the properties of excitons in 2D group VI transition-metal dichalcogenide (TMD) semiconductors that are modified by…

Strongly Correlated Electrons · Physics 2026-05-08 Jose M. Torres-Lopez , Sudipta Kundu , Felipe H. da Jornada , Tony Heinz , Allan H. MacDonald

Transition metal dichalcogenide (TMD) monolayers present a singular coupling in their spin and valley degrees of freedom. Moreover, by applying an external magnetic field it is possible to break the energy degeneracy between their K and…

Coherent light-matter interaction can be used to manipulate the energy levels of atoms, molecules and solids. When light with frequency {\omega} is detuned away from a resonance {\omega}o, repulsion between the photon-dressed (Floquet)…

Mesoscale and Nanoscale Physics · Physics 2017-03-22 Edbert J. Sie , Chun Hung Lui , Yi-Hsien Lee , Liang Fu , Jing Kong , Nuh Gedik

For monolayer transition metal chalcogenides (TMDs), electrons and excitons in different valleys can be driven to opposite directions by the Berry curvature, serving as a valley-dependent effective magnetic field. In addition to monolayer…

Mesoscale and Nanoscale Physics · Physics 2019-04-23 Zumeng Huang , Yuanda Liu , Kévin Dini , Zhuojun Liu , Hanlin Fang , Jin Liu , Timothy Liew , Weibo Gao

Transition metal dichalcogenides (TMDs) constitute a versatile platform for atomically thin optoelectronics devices and spin-valley memory applications. In monolayers optical absorption is strong, but the transition energy is not tunable as…

Monolayers of transition metal dichalcogenides are promising materials for valleytronic applications, since they possess two individually addressable excitonic transitions at the non-equivalent $K$ and $K'$ points with different spins,…

Mesoscale and Nanoscale Physics · Physics 2020-07-01 Malte Selig , Florian Katsch , Samuel Brem , Garnik F. Mkrtchian , Ermin Malic , Andreas Knorr

Monolayer transition-metal dichalcogenides (TMDCs) have recently emerged as possible candidates for valleytronic applications, as the spin and valley pseudospin are directly coupled and stabilized by a large spin splitting. In these…

Many-body exciton interactions shape the optoelectronic response of atomically-thin transition metal dichalcogenides, yet optical control of these interactions remains largely unexplored. To date, modulation of exciton-exciton interactions…

Transition metal dichalcogenides (TMDs) are layered materials that have a semiconducting phase with many advantageous optoelectronic properties, including tightly bound excitons and spin-valley locking. In Tungsten-based TMDs, spin and…

Mesoscale and Nanoscale Physics · Physics 2022-04-27 Saroj B. Chand , John M. Woods , Enrique Mejia , Takashi Taniguchi , Kenji Watanabe , Gabriele Grosso
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