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Inversion symmetry eliminates the second-order nonlinear responses in materials commonly used in silicon photonics with electric-dipole approximation. The lack of effective methods to induce the second-order nonlinearity in silicon photonic…

Optics · Physics 2024-05-22 Ru Wang , Yue Dai , Jinsong Cheng , Ruoyu Wang , Xiaoqin Shen

The resonance effects on the optical second harmonic generation from 140 nm silver nanoparticles is studied experimentally by hyper-Rayleigh scattering and numerically by finite element method calculations. We find that the interferences…

Second harmonic generation (SHG) is a nonlinear optical response arising exclusively from broken inversion symmetry in the electric-dipole limit. Recently, SHG has attracted widespread interest as a versatile and noninvasive tool for…

The second order optical response of centrosymmetric materials manifests itself mostly at their surface, being strongly suppressed in their bulk. However, the overall surface response is also suppressed in nanoparticles with a…

Optics · Physics 2021-09-22 Raksha Singla , W. Luis Mochán

Nonlinear energy exchange between vibrational modes underlies phenomena ranging from internal resonance to wave mixing, yet modal interactions are typically inferred from frequency-domain signatures rather than directly observed in space.…

The second-order nonlinear optical coefficients associated with chirality differ in sign for the two mirror-image forms (enantiomers) of a chiral material. Structures comprised of alternating stacks of the enantiomers can therefore be used…

Chemical Physics · Physics 2019-05-16 Bertrand Busson , Martti Kauranen , Colin Nuckolls , Thomas Katz , André Persoons

The classical problem of three-wave mixing in a nonlinear optical medium is investigated using the homotopy analysis method (HAM). We show that the power series basis builds a generic polynomial expression that can be used to study…

Optics · Physics 2022-12-23 Nathan J. Dawson , Moussa Kounta

The nonlinear optical response of an excitonic insulator coupled to lattice degrees of freedom is shown to depend in strong and characteristic ways on whether the insulating behavior originates primarily from electron-electron or…

Strongly Correlated Electrons · Physics 2021-01-04 Denis Golez , Zhiyuan Sun , Yuta Murakami , Antoine Georges , Andrew J. Millis

Fano interferences in nanostructures are influenced by dissipation effects as well as many-body interactions. Two dimensional coherent spectroscopies have just begun to be applied to these systems where the spectroscopic signatures of a…

Chemical Physics · Physics 2019-05-21 Daniel Finkelstein-Shapiro , Tõnu Pullerits , Thorsten Hansen

This second paper of two companion papers on the estimation of power spectra specializes to the topic of estimating galaxy power spectra at large, linear scales using maximum likelihood methods. As in the first paper, the aims are…

Astrophysics · Physics 2008-11-26 Andrew J. S. Hamilton

Nonlinear processes lie at the heart of many technologies such as frequency converters and entangled photon sources. Historically, observation and manipulation of these processes, for instance through nanostructures, has been limited to…

We present a novel method to synthesize non-trivial speckles that can enable superresolving second-order correlation imaging. The speckles acquire a unique anti-correlation in the spatial intensity fluctuation by introducing the blue noise…

We consider nonlinear spectroscopic effects - interaction-enhanced double resonance and spectrum instability - that appear in ultracold quantum gases owing to collisional frequency shift of atomic transitions and, consequently, due to the…

Quantum Gases · Physics 2015-06-12 Alexander Safonov , Irina Safonova , Igor Yasnikov

Techniques for coherent multidimensional optical spectroscopy have been developed and utilised to understand many different processes, including energy transfer in photosynthesis and many-body effects in semiconductor nanostructures.…

Optics · Physics 2017-01-24 Jonathan Tollerud , Jeffrey Davis

Imposition methods of interface conditions for the second-order wave equation with non-conforming grids is considered. The spatial discretization is based on high order finite differences with summation-by-parts properties. Previously…

Numerical Analysis · Mathematics 2022-10-25 Gustav Eriksson

Two-dimensional spectroscopic techniques combining terahertz (THz), infrared (IR), and visible pulses offer a wealth of information about coupling among vibrational modes in molecular liquids, thus providing a promising probe of their local…

Chemical Physics · Physics 2023-04-21 Tomislav Begušić , Geoffrey A. Blake

Suppression of wave scattering and the realization of transparency effects in engineered optical media and surfaces have attracted great attention in the past recent years. In this work the problem of transparency is considered for optical…

Optics · Physics 2016-05-04 Stefano Longhi

We describe a method of analysis which allows for reconstructing the nonlinear disturbance of a high Q harmonic oscillator. When the oscillator is driven with two or more frequencies, the nonlinearity causes intermodulation of the drives,…

Mesoscale and Nanoscale Physics · Physics 2010-04-19 Carsten Hutter , Daniel Platz , E. A. Tholen , T. H. Hansson , D. B. Haviland

Second order optical nonlinear processes involve the coherent mixing of two electromagnetic waves to generate a new optical frequency, which plays a central role in a variety of applications, such as ultrafast laser systems, rectifiers,…

Mesoscale and Nanoscale Physics · Physics 2015-06-03 Sanfeng Wu , Li Mao , Aaron M. Jones , Wang Yao , Chuanwei Zhang , Xiaodong Xu

Second-harmonic generation in resonant structures is commonly evaluated in terms of intracavity field enhancement at the fundamental and harmonic frequencies. Here, we formulate nonlinear frequency conversion within a symmetry-resolved…