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PbTe, one of the most promising thermoelectric materials, has recently demonstrated thermoelectric figure of merit ($ZT$) of above 2.0 when alloyed with group II elements. The improvements are due mainly to significant reduction of lattice…

Materials Science · Physics 2018-05-04 Yi Xia , James M. Hodges , Mercouri G. Kanatzidis , Maria K. Y. Chan

Tuning thermal transport in nanostructured materials is a powerful approach to develop high-efficiency thermoelectric materials. Using a recently developed approach based on the phonon mean free path dependent Boltzmann transport equation,…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Giuseppe Romano , Jeffrey C. Grossman

We present a comparative investigation of the influence of crystallinity and film thickness on the acoustic and thermal properties of 2D layered PtSe2 thin films of varying thickness (0.6-24 nm) by combining a set of experimental…

Metallic transition-metal nitrides (TMNs) are promising conductive ceramics for many applications, whose thermal transport is of great importance in device design. It is found metallic TiN and HfN hold anomalous thermal transport behaviors…

Materials Science · Physics 2020-06-30 Shouhang Li , Ao Wang , Yue Hu , Xiaokun Gu , Zhen Tong , Hua Bao

The lattice thermal conductivity plays a key role in the performance of thermoelectric materials, where the lower values lead to a higher figure of merit values. Two-dimensional group III-VI monolayers such as InTe are promising materials…

Computational Physics · Physics 2022-02-24 Hind Alqurashi , Abhiyan Pandit , Bothina Hamad

Thermal conductivity in dielectric crystals is the result of the relaxation of lattice vibrations described by the phonon Boltzmann transport equation. Remarkably, an exact microscopic definition of the heat carriers and their relaxation…

Materials Science · Physics 2016-10-26 Andrea Cepellotti , Nicola Marzari

This paper consists of two parts. The first part proposes a new methodological framework within which the heat conductivity in 1D lattices can be studied. The total process of heat conductivity is decomposed into two contributions where the…

Chaotic Dynamics · Physics 2011-03-21 T. Yu. Astakhova , V. N. Likhachev , G. A. Vinogradov

The Anderson localization of thermal phonons has been shown only in few nano-structures with strong random disorder by the exponential decay of transmission to zero and a thermal conductivity maximum when increasing system length. In this…

Mesoscale and Nanoscale Physics · Physics 2021-09-20 Yangyu Guo , Marc Bescond , Zhongwei Zhang , Shiyun Xiong , Kazuhiko Hirakawa , Masahiro Nomura , Sebastian Volz

Due to potential applications in nano- and opto-electronics, two-dimensional (2D) materials have attracted tremendous interest. Their thermal transport properties are closely related to the performance of 2D materials-based devices. Here,…

Materials Science · Physics 2019-02-20 San-Dong Guo

We show that the local temperature dependence of thermalized electron and phonon populations along metallic carbon nanotubes is the main reason behind this non-linear transport characteristics in the high bias regime. Our model that…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 M. A. Kuroda , J. -P. Leburton

Electron-crystal and phonon-glass are regarded as two essential factors for ideal thermoelectric materials, which require both an enhanced electronic transport and a depressed phononic transport. These two characteristics usually can not…

Materials Science · Physics 2016-06-29 Guangqian Ding , Guoying Gao , KailunYao

Modeling the high-$T$ paramagnetic state of bulk UO$_2$ by a non-spin-polarized calculation and neglecting the Hubbard-U correction for the $f$ electrons in U atoms, the lattice thermal conductivity of bulk UO$_2$ is investigated by the…

Materials Science · Physics 2020-08-25 Samira Sheykhi , Mahmoud Payami

Defects can significantly degrade the thermal conductivity of ThO2, an advanced nuclear fuel material as well as a surrogate for other fluorite-structured materials. We investigate how point defects in ThO2 impact phonon mode-resolved…

Materials Science · Physics 2024-09-24 Beihan Chen , Linu Malakkal , Marat Khafizov , David H. Hurley , Miaomiao Jin

For high efficiency thermoelectric power conversion not only improvement of materials properties but also prediction and synthesis of new thermoelectric materials is needed. Here we have carried out a systematic investigation on…

Materials Science · Physics 2021-01-25 Jayanta Bera , Atanu Betal , Satyajit Sahu

Using the linearized Boltzmann transport equation and perturbation theory, we analyze the reduction in the intrinsic thermal conductivity of few-layer graphene sheets accounting for all possible three-phonon scattering events. Even with…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 Dhruv Singh , Jayathi Y. Murthy , Timothy S. Fisher

Two-dimensional gallium nitride (2D-GaN) has great potential in power electronics and optoelectronics. Heat dissipation is a critical issue for these applications of 2D-GaN. Previous studies showed that higher-order phonon-phonon scattering…

Materials Science · Physics 2024-03-12 Jianshi Sun , Xiangjun Liu , Yucheng Xiong , Yuhang Yao , Xiaolong Yang , Cheng Shao , Shouhang Li

It has been argued that stanene has lowest lattice thermal conductivity among 2D group-IV materials because of largest atomic mass, weakest interatomic bonding, and enhanced ZA phonon scattering due to the breaking of an out-of-plane…

Mesoscale and Nanoscale Physics · Physics 2016-12-28 Bo Peng , Hao Zhang , Hezhu Shao , Yuanfeng Xu , Gang Ni , Rongjun Zhang , Heyuan Zhu

We calculate the thermal conductivity (\k{appa}) of both bulk crystalline and single-chain polyethylene (PE) using the first-principles-based anharmonic lattice dynamics. Despite its low \k{appa} in amorphous state, the predicted bulk…

Mesoscale and Nanoscale Physics · Physics 2017-01-11 Xinjiang Wang , Massoud Kaviany , Baoling Huang

Allotropes of carbon, such as diamond and graphene, are among the best conductors of heat. We monitored the evolution of thermal conductivity in thin graphite as a function of temperature and thickness and found an intimate link between…

Materials Science · Physics 2020-03-25 Yo Machida , Nayuta Matsumoto , Takayuki Isono , Kamran Behnia

Phonons, the quanta of lattice vibrations, are primary heat carriers for semiconductors and dielectrics. The demand of effective phonon manipulation urgently emerges, because the thermal management is crucial for the ongoing development of…