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Mott insulators with localized magnetic moments will exhibit a quantum spin liquid (QSL) state when the quantum fluctuations are strong enough to suppress the ordering of the spins. Such an entangled state will give rise to collective…

Strongly Correlated Electrons · Physics 2025-04-17 Haiyang Chen , Fo-Hong Wang , Qiang Gao , Xue-Jian Gao , Zhenhua Chen , Yaobo Huang , Kam Tuen Law , Xiao Yan Xu , Peng Chen

We present a theory of a hybrid quantum liquid state, $\textit{quantum spin-dipole liquid}$ (QSDL), in a hydrogen-bonded electron system, by combining a quantum proton ice and Anderson's resonating valence bond spin liquid theory, motivated…

Strongly Correlated Electrons · Physics 2020-10-16 Masahiko G. Yamada , Yasuhiro Tada

Quantum spin liquid (QSL) is an exotic quantum phase of matter whose ground state is quantum-mechanically entangled without any magnetic ordering. A central issue concerns emergent excitations that characterize QSLs, which are…

Strongly Correlated Electrons · Physics 2018-05-08 Y. Tokiwa , T. Yamashita , D. Terazawa , K. Kimura , Y. Kasahara , T. Onishi , Y. Kato , M. Halim , P. Gegenwart , T. Shibauchi , S. Nakatsuji , E. -G. Moon , Y. Matsuda

A new quantum spin liquid (QSL) candidate material H$_{3}$LiIr$_{2}$O$_{6}$ was synthesized recently and was found not to show any magnetic order or phase transition down to low temperatures. In this work, we study the quantum dynamics of…

Strongly Correlated Electrons · Physics 2020-08-17 Shuai Wang , Long Zhang , Fa Wang

The existence of a quantum spin liquid (QSL) in which quantum fluctuations of spins are sufficiently strong to preclude spin ordering down to zero temperature was originally proposed theoretically more than 40 years ago, but its…

The search of quantum spin liquid (QSL), an exotic magnetic state with strongly-fluctuating and highly-entangled spins down to zero temperature, is a main theme in current condensed matter physics. However, there is no smoking-gun evidence…

Strongly Correlated Electrons · Physics 2023-10-27 Z. H. Zhu , B. L. Pan , L. P. Nie , J. M. Ni , Y. X. Yang , C. S. Chen , Y. Y. Huang , E. J. Cheng , Y. J. Yu , A. D. Hillier , X. H. Chen , T. Wu , Y. Zhou , S. Y. Li , L. Shu

In Mott insulators, the strong electron-electron Coulomb repulsion prevents metallicity and charge excitations are gapped. In dimensions greater than one, their spins are usually ordered antiferromagnetically at low temperatures.…

Strongly Correlated Electrons · Physics 2012-10-02 D. Watanabe , M. Yamashita , S. Tonegawa , Y. Oshima , H. M. Yamamoto , R. Kato , I. Sheikin , K. Behnia , T. Terashima , S. Uji , T. Shibauchi , Y. Matsuda

Mott insulators are commonly pictured with electrons localized on lattice sites. Their low-energy degrees of freedom involve spins only. Here we observe emerging charge degrees of freedom in a molecule-based Mott insulator…

Currently under active study in condensed matter physics, both theoretically and experimentally, are quantum spin liquid (QSL) states, in which no long-range magnetic ordering appears at low temperatures due to strong quantum fluctuations…

Strongly Correlated Electrons · Physics 2019-07-04 Ruidan Zhong , Shu Guo , Guangyong Xu , Zhijun Xu , Robert J. Cava

At sufficiently low temperatures, interacting electron systems tend to develop orders. Exceptions are quantum critical point (QCP) and quantum spin liquid (QSL), where fluctuations prevent the highly entangled quantum matter to an ordered…

Strongly Correlated Electrons · Physics 2022-09-30 Yuan Da Liao , Xiao Yan Xu , Zi Yang Meng , Yang Qi

A quantum spin liquid (QSL) is a state of matter in which magnetic spins interact strongly, but quantum fluctuations inhibit long-range magnetic order even at zero temperature. A QSL has been predicted to have a host of exotic properties,…

At sufficiently low temperatures, condensed-matter systems tend to develop order. An exception are quantum spin-liquids, where fluctuations prevent a transition to an ordered state down to the lowest temperatures. While such states are…

Strongly Correlated Electrons · Physics 2010-04-15 Z. Y. Meng , T. C. Lang , S. Wessel , F. F. Assaad , A. Muramatsu

The emergence of a quantum spin liquid (QSL), a state of matter that can result when electron spins are highly correlated but do not become ordered, has been the subject of a considerable body of research in condensed matter physics. Spin…

A quantum spin liquid (QSL) is an exotic state in which electron spins are highly entangled, yet keep fluctuating even at zero temperature. Experimental realization of model QSLs has been challenging due to imperfections, such as antisite…

Strongly Correlated Electrons · Physics 2022-10-25 Huanpeng Bu , Malik Ashtar , Toni Shiroka , Helen C. Walker , Zhendong Fu , Jinkui Zhao , Jason S. Gardner , Gang Chen , Zhaoming Tian , Hanjie Guo

Magnetic structures of organic Mott insulators X[Pd(dmit)2]2 (X=Me4P, Me4Sb), of which electronic states are located near quantum spin liquid (X=EtMe3Sb), are demonstrated by 13C NMR. Antiferromagnetic spectra and nuclear relaxations show…

Strongly Correlated Electrons · Physics 2019-05-01 Shigeki Fujiyama , Reizo Kato

Quantum spin liquids~(QSLs) represent a unique quantum disordered state of matter that hosts long-range quantum entanglement and fractional excitations. However, structural disorder resulting from site mixing between different types of ions…

Quantum entanglement effects between the electronic spin and charge degrees of freedom are examined in an organic molecular solid, termed a dimer-Mott insulating system, in which molecular dimers are arranged in a crystal as fundamental…

Strongly Correlated Electrons · Physics 2016-05-18 Makoto Naka , Sumio Ishihara

Liquid He-4 is free from magnetic defects, making it an ideal substrate for electrons with long-lived spin states. Such states can serve as qubit states. Here we consider the spin states of electrons electrostatically localized in quantum…

Mesoscale and Nanoscale Physics · Physics 2023-02-08 M. I. Dykman , Ofek Asban , Qianfan Chen , Dafei Jin , S. A. Lyon

Correlation among particles in finite quantum systems leads to complex behaviour and novel states of matter. One remarkable example is predicted to occur in a semiconductor quantum dot (QD) where at vanishing density the Coulomb correlation…

We investigate the emergence of quantum spin liquid phases in pyrochlore oxides with non-Kramers ions, in which structural randomness effectively acts as a transverse field, introducing quantum fluctuations on top of the spin ice manifold.…

Strongly Correlated Electrons · Physics 2026-01-09 Marcus V. Marinho , Eric C. Andrade
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