Related papers: Gain and loss in open quantum systems
The non-hermitian quantum dynamics of excitonic energy transfer in photosynthetic systems is investigated using a dissipative two-level dimer model. The approach is based on the Green's function formalism which permits consideration of…
Photosynthesis powers life on our planet. The basic photosynthetic architecture comprises antenna complexes to harvest solar energy and reaction centers to convert the energy into a stable charge separated state. In oxygenic photosynthesis,…
The present review is devoted to our recent studies on the excitonic motion in photosynthetic systems. In photosynthesis, the light photon is absorbed to create an exciton in the antenna complex of the photosynthetic pigments. This exciton…
Photosynthetic organisms use networks of chromophores to absorb sunlight and deliver the energy to reaction centres, where charge separation triggers a cascade of chemical steps to store the energy. We present a detailed model of the…
Do quantum computers already exist in Nature? It is proposed that they do. Photosynthesis is one example in which a 'quantum computer' component may play a role in the 'classical' world of complex biological systems. A 'translation' of the…
The phenomenon of upconversion, in which a system sequentially absorbs two or more photons and emits a photon of a higher frequency, has been used in numerous applications. These include high-resolution non-destructive bioimaging,…
Photosynthesis is a fundamental process for plants to produce energy and survive. It is a well known fact that the light reactions in photosynthesis are a significant part of the overall process, and are carried out by chlorophyll…
We study the light absorption and energy transferring in a donor-acceptor system with a bionic structure. In the optimal case with uniform couplings, it is found that the quantum dynamics of this seemingly complicated system is reduced as a…
The goal of this research is to determine and study a physical system that will enable a fast and intrinsically two-photon detector, which would be of interest for quantum information and metrology applications. We consider two types of…
Creation of electron or exciton by external fields in a system with initially statistically independent unrelaxed vibrational modes leads to an initial condition term. The contribution of this term in the time convolution generalized master…
Many living organisms can exploit quantum mechanical effects to gain distinct biological advantages. In plants, photosynthesis uses quantum coherence to achieve near 100% efficiency in energy transfer. With advances in experimental…
The decay of photoexcited quantum systems (examples are photodissociation of molecules and autoionization of atoms) can be viewed as a half-collision process (an incoming photon excites the system which subsequently decays by dissociation…
The photosynthetic reaction center of plants and bacteria is an extremely efficient energy to charge conversion device. Solar photons create excitons in the pigment molecules. These excitons are then transferred to the reaction center where…
The charge photogeneration process in organic molecules is investigated by a quantum heat engine model, in which two molecules are modeled by a two-spin system sandwiched between two bosonic baths at their own temperatures. The two baths…
Studies of emerging photovoltaics, such as organic and perovskite solar cells, have recently shown that the separation of photo-generated charge carriers is correlated with non-thermal, coherent oscillations within the illuminated device.…
Photosynthesis converts sunlight into the chemical free energy that feeds the Earth's biosphere, yet at levels much lower than what thermodynamics would allow for. I propose here that photosynthesis is nevertheless thermodynamically…
In this work we study the first step in photosynthesis for the limiting case of a single photon interacting with photosystem II (PSII). We model our system using quantum trajectory theory, which allows us to consider not only the average…
Photosynthesis is arguably the fundamental process of Life, since it enables energy from the Sun to enter the food-chain on Earth. It is a remarkable non-equilibrium process in which photons are converted to many-body excitations which…
In many important cases, the rate of excitation of a system embedded in an environment is significantly smaller than the internal system relaxation rates. An important example is that of light-induced processes under natural conditions, in…
The long-standing problem of nearly perfect photosynthetic yield in some types of bacteria and nearly all kinds of plants despite the interaction with a hot and noisy environment has witnessed quantum optical explanations in the last decade…