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Ultrasound is a key technology in healthcare, and it is being explored for non-invasive, wearable, continuous monitoring of vital signs. However, its widespread adoption in this scenario is still hindered by the size, complexity, and power…

We present ultra-fast quantum chemical methods for the calculation of infrared and ultraviolet-visible spectra designed to provide fingerprint information during autonomous and interactive explorations of molecular structures.…

Chemical Physics · Physics 2022-08-30 Francesco Bosia , Thomas Weymuth , Markus Reiher

We demonstrate coherent Doppler-free three-photon excitation of the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{0}$ optical clock transition and the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{1}$ intercombination transition in free-space thermal clouds of…

Atomic Physics · Physics 2024-12-24 Guglielmo Panelli , Shaun C. Burd , Erik J. Porter , Mark Kasevich

In 1949, Ramsey's method of separated oscillating fields was elaborated boosting over many decades metrological performances of atomic clocks and becoming the standard technique for very high precision spectroscopic measurements. A…

Atomic Physics · Physics 2022-05-17 T. Zanon-Willette , D. Wilkowski , R. Lefevre , A. V. Taichenachev , V. I. Yudin

We show that the light shift in atomic clocks can be suppressed using time variation of the interrogation field intensity. By measuring the clock output at two intensity levels, error signals can be generated that simultaneously stabilize a…

We examine the influence of probe laser intensity fluctuations on hyper-Ramsey spectroscopy. We assume, as is appropriate for relevant cases of interest, that the probe laser intensity $I$ determines both the Rabi frequency…

Atomic Physics · Physics 2018-05-04 K. Beloy

A train of periodic optical pulses gives an optical frequency "comb" that acts as a precise ruler for light measurement due to its equally spaced frequencies. Today, such pulses last millionths of a billionth of a second (Femtoseconds/fs)…

Optics · Physics 2026-05-22 Tushar Malica

Controlling nonequilibrium responses in optically driven quantum materials is essential for advancing applications in energy conversion, ultrafast electronics, and quantum computation. Nonlinear optical spectroscopy serves as a powerful…

We have developed an ultra-stable source in the deep ultraviolet, suitable to fulfill the interrogation requirements of a future fully-operational lattice clock based on neutral mercury. At the core of the system is a Fabry-P\'erot cavity…

Atomic Physics · Physics 2015-03-13 S. T. Dawkins , R. Chicireanu , M. Petersen , J. Millo , D. V. Magalhães , C. Mandache , Y. Le Coq , S. Bize

We propose a novel pulsed optical field method that alternately switches the pump beam in conventional saturation absorption to time-division multiplex the same probe beam into both probe and reference beams, followed by digital…

In this paper, we present a unified computational method based on pseudospectral approximations for the design of optimal pulse sequences in open quantum systems. The proposed method transforms the problem of optimal pulse design, which is…

Chemical Physics · Physics 2009-08-17 Jr-Shin Li , Justin Ruths , Dionisis Stefanatos

We propose an iterative solution method for the 3D high-frequency Helmholtz equation that exploits a contour integral formulation of spectral projectors. In this framework, the solution in certain invariant subspaces is approximated by…

Numerical Analysis · Mathematics 2018-11-30 Xiao Liu , Yuanzhe Xi , Yousef Saad , Maarten V. de Hoop

Lensless imaging is an elegant approach to high-resolution microscopy, which is rapidly gaining popularity in applications where imaging optics are problematic. However, current lensless imaging methods require objects to be placed within a…

We introduce the first method to enable an optical amplification of a coherent Raman spectroscopy signal called radio frequency Doppler Raman spectroscopy. Doppler Raman measurements amplify the optical signals in coherent Raman…

We propose and experimentally demonstrate a scheme which effects hyperfine averaging during a Ramsey interrogation of a clock transition. The method eliminates the need to average over multiple optical transitions, reduces the sensitivity…

Quantum Physics · Physics 2020-03-04 R. Kaewuam , T. R. Tan , K. J. Arnold , S. R. Chanu , Zhiqiang Zhang , M. D. Barrett

Development of the optical frequency comb has revolutionised metrology and precision spectroscopy due to its ability to provide a precise and direct link between microwave and optical frequencies. A novel application of frequency comb…

Nonlinear spectroscopy is a cornerstone of quantum science, providing unique access to multi-point correlations, quantum coherence, and couplings that are invisible to linear methods. However, classical simulation of these phenomena is…

Quantum Physics · Physics 2026-04-20 Long Xiong , Xiaoyang Wang , Xiaoxia Cai , Xiao Yuan

Platforms for all-optical computing possess photonic circuits made of silicon-based channels, metal wires or optical fibers, etc. However, such solid waveguides suffer from the lack of reversibility and reconfigurability if facing the next…

Optics · Physics 2022-11-15 Jia-Yu Zhao

We investigate the system of a heavy impurity immersed in a degenerated Fermi gas, where the impurity's internal degree of freedom (pseudospin) is manipulated by a series of radiofrequency (RF) pulses at several different times. Applying…

Quantum Gases · Physics 2023-01-18 Jia Wang

We develop a model for quantum computation with Rydberg atom arrays, which only relies on global driving, without the need of local addressing of the qubits: any circuit is executed by a sequence of global, resonant laser pulses on a static…

Quantum Physics · Physics 2023-10-27 Francesco Cesa , Hannes Pichler