Related papers: Imaging ultrafast molecular wavepackets with a sin…
Four-wave mixing processes are ubiquitous in ultrafast optics and the determination of the coefficients of the $\chi^{(3)}$ tensor is thus essential. We introduce a novel time-resolved ultrafast spectroscopic method to characterize the…
We present a method for a complete characterization of a femtosecond ultraviolet pulse when a fundamental near-infrared beam is also available. Our approach relies on generation of second harmonic from the pre-characterized fundamental,…
We investigate ultrafast vibronic dynamics triggered by intense femtosecond infrared pulses in small molecules. Our study is based on numerical simulations performed with 2D model molecules, and analyzed in the perspective of the renown…
A chirped laser pulse focused by a chromatic lens exhibits a dynamic, or "flying," focus in which the trajectory of the peak intensity decouples from the group velocity. In a medium, the flying focus can trigger an ionization front that…
We develop photoelectron interferometry based on laser-assisted extreme ultraviolet ionization for flexible and robust control of photoelectron circular dichroism in randomly oriented chiral molecules. A comb of XUV photons ionizes a sample…
Split-pulse x-ray photon correlation spectroscopy has been proposed as one of the unique capabilities made possible with the x-ray free electron lasers. It enables characterization of atomic scale structural dynamics that dictates the…
Femtosecond extreme ultraviolet wave packet interferometry (XUV-WPI) was applied to study resonant inter-atomic Coulombic decay (ICD) in the HeNe dimer. The high demands on phase stability and sensitivity for vibronic XUV-WPI of…
Photoassociation of ultracold atoms is shown to lead to alignment of the product molecules along the excitation laser polarization axis. We theoretically investigate pulsed photoassociation of $^{87}Rb$ atoms into a specific weakly-bound…
We present a new method for ultrafast spectroscopy of molecular photoexcited dynamics. The technique uses a pair of femtosecond pulses: a photoexcitation pulse initiating excited state dynamics followed by a soft x-ray (SXR) probe pulse…
Recently developed circularly polarized X-ray light sources can probe ultrafast chiral electronic and nuclear dynamics through spatially localized resonant core transitions. We present simulations of time-resolved circular dichroism (TRCD)…
Ultra-intense laser-matter interaction experiments (>10$^{18}$ W/cm$^{2}$) with dense targets are highly sensitive to the effect of laser "noise" (in the form of pre-pulses) preceding the main ultra-intense pulse. These system-dependent…
Achromatic flying-focus enables programmable control of intensity peak velocity, with applications in ultrafast optics. However, spatiotemporal coupling inherently elongates ultrashort pulses by introducing frequency-dependent focusing and…
The ability to measure the bulk dynamic behavior of soft materials with combined time- and frequency-resolution is instrumental for improving our fundamental understanding of connections between the microstructural dynamics and the…
Coherent control of ultrafast quantum phenomena benefits from pulse-shaping capabilities allowing to modulate the envelope and instantaneous phase of optical fields on femtosecond time scales. While such control is available for optical…
We present a simple and robust technique to retrieve the phase of ultrashort laser pulses, based on a chirped mirror and glass wedges compressor. It uses the compression system itself as a diagnostic tool, thereby making unnecessary the use…
Broadband microwave waveforms with programmable chirp shapes are captivating in numerous practical applications. Compared with electronic technology, photonic-assisted solutions exhibit excellent performance in bandwidth and flexibility,…
We describe an electro-optic dual-comb system that operates in the near-infrared (near-IR) region to generate optical frequency combs in the near-UV by sum frequency generation in two configurations. The near-IR frequency combs are…
The coherent manipulation of wave packets is an important tool in many areas of physics. We demonstrate the experimental realization of quasi-free wave packets of ultra-cold atoms bound by an external harmonic trap. The wave packets are…
Interaction of a frequency-chirped laser pulse with single protons and a hydrogen plasma cell is studied analytically and by means of particle-in-cell simulations, respectively. Feasibility of generating ultra-intense (10^7 particles per…
It is shown theoretically that the use of accelerating spatiotemporal quasi-phase-matching (QPM) modulation patterns in media with parametric optical interactions makes it possible to generate a time-reversed replica of the pump pulse…