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Related papers: On Ni-Sb-Sn based skutterudites

200 papers

Magnetization, specific heat, and electrical resistivity measurements were made on single crystals of the filled skutterudite compound PrOs$_{4}$As$_{12}$. Specific heat measurements indicate an electronic specific heat coefficient $\gamma$…

Filling the large voids in the crystal structure of the skutterudite CoSb$_3$ with rattler atoms $R$ provides an avenue for both increasing carrier concentration and disrupting lattice heat transport, leading to impressive thermoelectric…

Materials Science · Physics 2020-07-17 Eric B. Isaacs , Chris Wolverton

We report on systematic study of superconducting characteristics and Pr crystalline-electric-field (CEF) levels of filled-skutterudite \pra ($T_{\rm c}$ = 2.33 K). The temperature dependences of the upper critical field $H_{\rm c2}$ and the…

Strongly Correlated Electrons · Physics 2007-10-03 T. Namiki , Y. Aoki , H. Sato , C. Sekine , I. Shirotani , T. D. Matsuda , Y. Haga , T. Yagi

The filled skutterudite compound \PrOsSb{} has been found to exhibit superconductivity with a critical temperature $T_\mathrm{c} = 1.85$ K that develops out of a heavy Fermi liquid with an effective mass $m^{*} \approx 50 m_\mathrm{e}$. The…

Superconductivity · Physics 2016-08-31 M. B. Maple , P. -C. Ho , V. S. Zapf , W. M. Yuhasz , N. A. Frederick , E. D. Bauer

We report on two fold increase in superconducting transition temperature of La3Co4Sn13 by substituting indium at the tin site. The transition temperature of this skutterudite is observed to increase from 2.5 K to 5.1 K for 10 % indium…

Superconductivity · Physics 2015-09-17 P. Neha , P. Srivastava , R. Jha , Shruti , V. P. S. Awana , S. Patnaik

Thermal conductivity measurements were performed on single crystal samples of the superconducting filled skutterudite compounds PrOs$_4$Sb$_{12}$ and PrRu$_4$Sb$_{12}$ both as a function of temperature and magnetic field applied…

Superconductivity · Physics 2007-09-28 R. W. Hill , Shiyan Li , M. B. Maple , Louis Taillefer

X-ray diffraction, electrical resistivity, magnetization, specific heat, and thermoelectric power measurements are presented for single crystals of the new filled skutterudite compound {\CeOsAs}, which reveal phenomena that are associated…

Strongly Correlated Electrons · Physics 2009-11-13 R. E. Baumbach , P. C. Ho , T. A. Sayles , M. B. Maple , R. Wawryk , T. Cichorek , A. Pietraszko , Z. Henkie

We studied nanoprecipitates and defects in p-type filled skutterudite CeFe4Sb12 prepared by non-equilibrium melt-spinning plus spark plasma sintering method using transmission electron microscopy. Nanoprecipitates with mostly spherical…

Materials Science · Physics 2015-05-20 Juan Zhou , Qing Jie , Lijun Wu , Ivo Dimitrov , Xun Shi , Qiang Li

The optical conductivity [$\sigma(\omega)$] spectra of alkaline-earth-filled skutterudites with the chemical formula $A^{2+}M_{4}$Sb$_{12}$ ($A$ = Sr, Ba, $M$ = Fe, Ru, Os) and a reference material La$^{3+}$Fe$_{4}$Sb$_{12}$ were obtained…

Strongly Correlated Electrons · Physics 2009-11-13 Shin-ichi Kimura , Hojun Im , Takafumi Mizuno , Shota Narazu , Eiichi Matsuoka , Toshiro Takabatake

We report the electric transport and thermodynamic properties of the skutterudite-related La$_3$Co$_4$Sn$_{13}$ and La$_3$Rh$_4$Sn$_{13}$ superconductors. Applying an external pressure to La$_3$Rh$_4$Sn$_{13}$, the resistive superconducting…

Superconductivity · Physics 2014-03-25 A. Slebarski , M. Fijalkowski , M. M. Maska , M. Mierzejewski , B. D. White , M. B. Maple

First thermoelectric properties measurements on bulk nanostructured Ba8Ga16Ge30 clathrate-I are presented. A sol-gel-calcination route was developed for preparing amorphous nanosized precursor oxides. The further reduction of the oxides led…

This work presents theoretical calculations of the electrical transport properties of the Ag, Au, and La fractionally filled bulk skutterudites: CoSb3, CoAs3, and CoP3. Density functional theory (DFT), along with projector augmented wave…

Materials Science · Physics 2015-04-28 Maria Stoica , Cynthia S. Lo

In this article we present a neutron diffraction in-situ study of the thermal evolution and high-temperature structure of layered cobaltites Y(Ba, Sr)Co2 O5+{\delta}. Neutron thermodiffractograms and magnetic susceptibility measurements are…

Materials Science · Physics 2015-05-19 G Aurelio , R D Sánchez , J Curiale , G J Cuello

In this work, we try to understand the experimental thermoelectric (TE) properties of a ZrNiSn sample with DFT and semiclassical transport calculations using SCAN functional. SCAN and mBJ provide the same band gap $E_{g}$ of $\sim$0.54 eV.…

Strongly Correlated Electrons · Physics 2020-06-24 Shivprasad S. Shastri , Sudhir K. Pandey

The reliable calculation of electronic structures and understanding of electrical properties depends on an accurate model of the crystal structure. Here, we have reinvestigated the crystal structure of the high-zT thermoelectric material…

Materials Science · Physics 2018-08-14 I. Loa , S. R. Popuri , A. D. Fortes , J. W. G. Bos

We report $^{123}$Sb nuclear quadrupole resonance (NQR) measurements of the filled skutterudite heavy-fermion superconductor PrOs$_4$Sb$_{12}$ under high pressures of 1.91 and 2.34 GPa. The temperature dependence of NQR frequency and the…

We investigated the superconducting order parameter of the filled skutterudite LaPt4Ge12, with a transition temperature of Tc = 8.3 K. To this end, we performed temperature and magnetic-field dependent specific-heat and thermal-conductivity…

We present an ab initio study of the structural and electronic transport properties of tetrahedrite, Cu$_{12}$Sb$_4$S$_{13}$, in its high-temperature phase. We show how this complex compound can be seen as the outcome of an ordered…

Materials Science · Physics 2020-07-07 Cono di Paola , Francesco Macheda , Savio Laricchia , Cedric Weber , Nicola Bonini

Debye temperature decrease, residual resistivity increase and electron-phonon coupling constant increase as crystallite size decreases have been found from electrical resistivity in temperature range 5 K to 300 K of well-characterized Ag…

Mesoscale and Nanoscale Physics · Physics 2019-08-21 Vikash Sharma , Gunadhor Singh Okram

Crystallographic data and thermoelectric properties (from 240 K up to 380 K) of Yb3Co4Ge13, Yb3Co4Sn13 compounds and Yb2CeCo4Ge13 and Yb2.3La0.7Co4Ge13 solid solutions are reported. The Seebeck coefficients, electric resistance and thermal…

Materials Science · Physics 2012-11-28 A. V. Morozkin , V. Yu. Irkhin , V. N. Nikiforov