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We present an excited-state-specific coupled-cluster approach in which both the molecular orbitals and cluster amplitudes are optimized for an individual excited state. The theory is formulated via a pseudoprojection of the traditional…

Chemical Physics · Physics 2023-11-27 Harrison Tuckman , Eric Neuscamman

Coupled cluster theory has had a momentous impact on the ab initio prediction of molecular properties, and remains a staple ingratiate in high-accuracy thermochemical model chemistries. However, these methods require inclusion of at least…

Chemical Physics · Physics 2025-03-26 James H. Thorpe , Zachary W. Windom , Rodney J. Bartlett , Devin A. Matthews

In this paper, we have analysed the time series associated with the iterative scheme of a double similarity transformed Coupled Cluster theory. The coupled iterative scheme to solve the ground state Schr{\"o}dinger equation is cast as a…

Statistical Mechanics · Physics 2020-07-29 Valay Agarawal , Anish Chakraborty , Rahul Maitra

While limited coupled cluster theory is \textit{formally} nonvariational, it is not broadly appreciated whether this is a major issue \textit{in practice}. We carried out a detailed comparison with \textit{de facto} full CI energies for a…

Chemical Physics · Physics 2024-10-03 Jan M. L. Martin , Emmanouil Semidalas

We introduce a new type of cluster expansion which generalizes a previous formula of Brydges and Kennedy. The method is especially suited for performing a phase-space multiscale expansion in a just renormalizable theory, and allows the…

High Energy Physics - Theory · Physics 2009-07-09 A. Abdesselam , V. Rivasseau

A univariate clustering criterion for stationary processes satisfying a $\beta$-mixing condition is proposed extending the work of \cite{KB2} to the dependent setup. The approach is characterized by an alternative sample criterion function…

Statistics Theory · Mathematics 2013-11-19 Karthik Bharath

A Cumulant based method has been introduced to extract quantum corrections in distribution function with the equilibrium Wigner-Boltzmann equation. It is shown that unlike the moment expansion used in hydrodynamic model, cumulant expansion…

Statistical Mechanics · Physics 2019-03-14 Xiyue Li , Everett X. Wang

We develop a quantum algorithm for solving high-dimensional fractional Poisson equations. By applying the Caffarelli-Silvestre extension, the $d$-dimensional fractional equation is reformulated as a local partial differential equation in…

Numerical Analysis · Mathematics 2025-05-06 Shi Jin , Nana Liu , Yue Yu

We propose two improvements to the well-known power series method for confined one-dimensional quantum-mechanical problems. They consist of the addition of a variational step were the energy plays the role of a variational parameter. We…

Quantum Physics · Physics 2016-02-25 Francisco M. Fernández

The quantum Monte Carlo methods represent a powerful and broadly applicable computational tool for finding very accurate solutions of the stationary Schroedinger equation for atoms, molecules, solids and a variety of model systems. The…

Computational Physics · Physics 2011-01-28 Jindrich Kolorenc , Lubos Mitas

The complexity of the standard hierarchy of quantum chemistry methods is not invariant to the choice of representation. This work explores how the scaling of common quantum chemistry methods can be reduced using real-space, momentum-space,…

Chemical Physics · Physics 2018-02-14 Narbe Mardirossian , James D. McClain , Garnet Kin-Lic Chan

We discuss diagrammatic modifications to the coupled cluster doubles (CCD) equations, wherein different groups of terms out of rings, ladders, crossed-rings and mosaics can be removed to form approximations to the coupled cluster method, of…

Chemical Physics · Physics 2014-05-06 James J. Shepherd , Thomas. M. Henderson , Gustavo E. Scuseria

We introduce a hybrid method to couple continuous Galerkin finite element methods and high-order finite difference methods in a nonconforming multiblock fashion. The aim is to optimize computational efficiency when complex geometries are…

Numerical Analysis · Mathematics 2021-11-24 Tuan Anh Dao , Ken Mattsson , Murtazo Nazarov

We develop a high order reconstructed discontinuous approximation (RDA) method for solving a mixed formulation of the quad-curl problem in two and three dimensions. This mixed formulation is established by adding an auxiliary variable to…

Numerical Analysis · Mathematics 2024-07-12 Ruo Li , Qicheng Liu , Shuhai Zhao

We study quantum spin systems in the 1D, 2D square and 3D cubic lattices with nearest-neighbour XY exchange. We use the coupled-cluster method (CCM) to calculate the ground-state energy, the T=0 sublattice magnetisation and the excited…

Condensed Matter · Physics 2009-10-30 D. J. J. Farnell , S. E. Krueger , J. B. Parkinson

Solitons confined in a channel are studied in the two-dimensional nonlinear Schroedinger equation. When a channel branches into two channels, a soliton is split into two solitons, if the initial kinetic energy exceeds a critical value. The…

Pattern Formation and Solitons · Physics 2010-09-20 Hidetsugu Sakaguchi , Yusuke Kageyama

In this paper, by combining of fractional centered difference approach with alternating direction implicit method, we introduce a mixed difference method for solving two-dimensional Riesz space fractional advection-dispersion equation. The…

Numerical Analysis · Mathematics 2020-06-09 A. Borhanifar , M. A. Ragusa , S. Valizadehaz

This chapter presents the theory behind the CASPT2 method and its adaptation to a multi-state formalism. The chapter starts with an introduction of the theory of the CASPT2 method - an application of Rayleigh-Schr\"odinger perturbation…

Chemical Physics · Physics 2023-05-12 Stefano Battaglia , Ignacio Fdez. Galván , Roland Lindh

For a singular oscillator, the Schrodinger equation is obtained an equation of eigenvalues, and the dependence of energy on the self-adjoint extension parameter is established. It is shown that the self-adjoint extension violates the…

Quantum Physics · Physics 2024-06-21 Anzor Khelashvili , Teimuraz Nadareishvili

Unitary coupled cluster (UCC), originally developed as a variational alternative to the popular traditional coupled cluster method, has seen a resurgence as a functional form for use on quantum computers. However, the number of excitors…

Chemical Physics · Physics 2021-01-07 Maria-Andreea Filip , Alex J. W. Thom