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Related papers: The interplay between excitons and trions in a mon…

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Unconventional emissions from exciton and trion in monolayer WS2 are studied by photoexcitation. Excited by 532nm laser beam, the carrier species in the monolayer WS2 are affected by the excess electrons escaping from photoionization of…

Mesoscale and Nanoscale Physics · Physics 2016-08-08 Ke Wei , Yu Liu , Hang Yang , Xiangai Cheng , Tian Jiang

Charged excitons, or X$^{\pm}$-trions, in monolayer transition metal dichalcogenides have binding energies of several tens of meV. Together with the neutral exciton X$^0$ they dominate the emission spectrum at low and elevated temperatures.…

We revisit low-temperature optical spectra of transition-metal dichalcogenide monolayers and point to a possible crystallization of electrons (or holes) at low to moderate charge densities. To calculate the excitonic spectra under such…

Mesoscale and Nanoscale Physics · Physics 2023-08-16 Dinh Van Tuan , Hanan Dery

Optically dark excitonic states play a critical role in the valleytronic, electronic, and optical properties of monolayer semiconducting transition metal dichalcogenides. Here, we investigate how electrostatic doping affects the in-plane…

Doping substantially influences the electronic and photophysical properties of semiconducting single-wall carbon nanotubes (s-SWNTs). Although prior studies have noted that surplus charge carriers modify optical spectra and accelerate…

Materials Science · Physics 2023-07-19 Klaus H. Eckstein , Pascal Kunkel , Markus Voelckel , Friedrich Schöppler , Tobias Hertel

We present photoluminescence measurements in monolayer WSe$_2$, which point to the importance of the interaction between charged particles and excitonic complexes. The theoretical analysis highlights the key role played by exchange…

Materials Science · Physics 2022-02-15 Min Yang , Lei Ren , Cedric Robert , Dinh Van Tuan , Laurent Lombez , Bernhard Urbaszek , Xavier Marie , Hanan Dery

The effect of bis(trifluoromethane) sulfonimide (TFSI, superacid) treatment on the optical properties of MoS$_2$ monolayers is investigated by means of photoluminescence, reflectance contrast and Raman scattering spectroscopy employed in a…

Mesoscale and Nanoscale Physics · Physics 2019-02-14 Maciej R. Molas , Katarzyna Gołasa , Łukasz Bala , Karol Nogajewski , Miroslav Bartos , Marek Potemski , Adam Babiński

We present a detailed investigation of the exciton and trion dynamics in naturally doped MoSe2 and WSe2 single atomic layers as a function of temperature in the range 10-300K under above band-gap laser excitation. By combining…

In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results…

The optical properties of semiconducting transition metal dichalcogenides are dominated by both neutral excitons (electron-hole pairs) and charged excitons (trions) that are stable even at room temperature. While trions directly influence…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Kai Hao , Lixiang Xu , Philipp Nagler , Akshay Singh , Kha Tran , Chandriker Kavir Dass , Christian Schüller , Tobias Korn , Xiaoqin Li , Galan Moody

Optical excitation typically enhances electrical conduction and low-frequency radiation absorption in semiconductors. We have, however, observed a pronounced transient decrease of conductivity in doped monolayer molybdenum disulfide (MoS2),…

Mesoscale and Nanoscale Physics · Physics 2014-10-22 C. H. Lui , A. J. Frenzel , D. V. Pilon , Y. -H. Lee , X. Ling , G. M. Akselrod , J. Kong , N. Gedik

Radiative recombination of excitons dressed by the interactions with free charge carriers often occurs under simultaneous excitation of either electrons or holes to unbound states. This phenomenon, known as the electron recoil effect,…

Controlling exciton relaxation and energy conversion pathways via their coupling to photonic modes is a central task in cavity-mediated quantum materials research. In this context, the light-matter hybridization in optical cavities can lead…

Hyperspectral imaging at cryogenic temperatures is used to investigate exciton and trion propagation in MoSe$_2$ monolayers encapsulated with hexagonal boron nitride (hBN). Under a tightly focused, continuous-wave laser excitation, the…

Monolayer and multilayer MoS$_2$ are extremely fascinating materials for the use in lasers, compact optical parametric amplifiers, and high-power detectors which demands high excitation light-matter interaction. Consequently, it is…

Materials Science · Physics 2024-07-09 Durga Prasad Khatua , Asha Singh , Sabina Gurung , J. Jayabalan

Monolayers of semiconducting transition metal dichalcogenides are a strongly emergent platform for exploring quantum phenomena in condensed matter, building novel opto-electronic devices with enhanced functionalities. Due to their atomic…

We investigate with polarized microphotoluminescence the optical pumping of the valley degree of freedom in charge-tunable MoS2 monolayers encapsulated with hexagonal boron nitride at cryogenic temperatures. We report a large steady state…

Mesoscale and Nanoscale Physics · Physics 2021-10-15 Sangjun Park , Steve Arscott , Takashi Taniguchi , Kenji Watanabe , Fausto Sirotti , Fabian Cadiz

Two-dimensional semiconductors exhibit pronounced many-body effects and intense optical responses due to strong coulombic interactions. Consequently, subtle differences in photoexcitation conditions can strongly influence how the material…

We measure the optical absorption spectra and optical conductivities of excitons and trions in monolayers of metal dichalcogenide MoS$_{2}$ and compare the results with theoretical models. Our results show that the Wannier-Mott model for…

Mesoscale and Nanoscale Physics · Physics 2014-06-04 Changjian Zhang , Haining Wang , Weimin Chan , Christina Manolatou , Farhan Rana

The optical spectra of transition metal dichalcogenide (TMDC) monolayers are dominated by excitons and trions. Here we establish the dependences of these optical transitions on disorder from hyperspectral imaging of h-BN encapsulated…

Mesoscale and Nanoscale Physics · Physics 2022-12-13 Jue Wang , Christina Manolatou , Yusong Bai , James Hone , Farhan Rana , Xiaoyang Zhu
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