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We show that weakly bound He-containing van der Waals molecules can be produced and magnetically trapped in buffer-gas cooling experiments, and provide a general model for the formation and dynamics of these molecules. Our analysis shows…

We show that a large class of helium-containing cold polar molecules form readily in a cryogenic buffer gas, achieving densities as high as 10^12 cm^-3. We explore the spin relaxation of these molecules in buffer gas loaded magnetic traps,…

Atomic Physics · Physics 2011-04-29 N. Brahms , T. V. Tscherbul , P. Zhang , J. K los , H. R. Sadeghpour , A. Dalgarno , J. M. Doyle , T. G. Walker

The strong evanescent field around ultra-thin unclad optical fibers bears a high potential for detecting, trapping, and manipulating cold atoms. Introducing such a fiber into a cold atom cloud, we investigate the interaction of a small…

Quantum Physics · Physics 2009-11-13 G. Sagué , E. Vetsch , W. Alt , D. Meschede , A. Rauschenbeutel

Attaining viable thermoelectric cooling at cryogenic temperatures is of major fundamental and technological interest for novel electronics and quantum materials applications. In-device temperature control can provide a more efficient and…

Mesoscale and Nanoscale Physics · Physics 2024-03-13 T. Völkl , A. Aharon-Steinberg , T. Holder , E. Alpern , N. Banu , A. K. Pariari , Y. Myasoedov , M. E. Huber , M. Hücker , E. Zeldov

Lamellar crystalline materials, whose layers are bond by van der Waals forces, can be stacked to form ultrathin artificial heterostructures, and in particular vertical magnetic junctions when some of the stacked materials are…

We propose a method for laser cooling and trapping a substantial class of polar molecules, and in particular titanium (II) oxide (TiO). This method uses pulsed electric fields to nonadiabatically remix the ground-state magnetic sublevels of…

Atomic Physics · Physics 2008-12-13 Benjamin K. Stuhl , Brian C. Sawyer , Dajun Wang , Jun Ye

Thermally activated flux flow (TAFF) and flux flow Hall effect (FFHE) of Fe(Te,S) single crystal in the mixed state are studied in magnetic fields up to 35 T. Thermally activated energy (TAE) is analyzed using conventional Arrhenius…

Superconductivity · Physics 2010-10-20 Hechang Lei , Rongwei Hu , E. S. Choi , C. Petrovic

We describe a novel type of interaction between open-shell polar molecules at sub-millikelvin temperatures. This hyperfine van der Waals interaction occurs between two molecules in two rotational states that differ by one quantum. Normally,…

Atomic Physics · Physics 2025-09-23 Etienne F. Walraven , Tijs Karman

We present the first experimental observation of cold collisions between two different species of neutral polar molecules, each prepared in a single internal quantum state. Combining for the first time the techniques of Stark deceleration,…

We discuss laser dressed dipolar and Van der Waals interactions between atoms and polar molecules, so that a cold atomic gas with laser admixed Rydberg levels acts as a designed reservoir for both elastic and inelastic collisional…

Atomic Physics · Physics 2012-05-15 Bo Zhao , Alexander Glätzle , Guido Pupillo , Peter Zoller

We present a method to design a finite decay rate for excited rotational states in polar molecules. The setup is based on a hybrid system of polar molecules with atoms driven into a Rydberg state. The atoms and molecules are coupled via the…

Quantum Gases · Physics 2012-05-15 Sebastian D. Huber , Hans Peter Büchler

Quantum mechanical calculations are reported for the Li+HF(v=0,1,j=0)-->H+LiF(v',j') bimolecular scattering process at low and ultralow temperatures. Calculations have been performed for zero total angular momentum using a recent high…

Chemical Physics · Physics 2009-11-10 P. F. Weck , N. Balakrishnan

Cryogenic buffer gas sources are ubiquitous for producing cold, collimated molecular beams for quantum science, chemistry, and precision measurements. The molecules are typically produced by laser ablating a metal target in the presence of…

We reported a detailed experimental study of the cold collision of Barium monofluoride (BaF) with buffer gas and the high-resolution spectroscopy relevant with direct laser cooling. BaF molecules are efficiently produced with laser ablation…

Atomic Physics · Physics 2017-03-22 Wenhao Bu , Tao Chen , Guitao Lv , Bo Yan

We demonstrate cryogenic buffer-gas cooling of gas-phase methyltrioxorhenium (MTO). This molecule is closely related to chiral organometallic molecules where the parity-violating energy differences between enantiomers may be measurable. The…

Atomic Physics · Physics 2017-09-07 Sean Tokunaga , R. J. Hendricks , M. Tarbutt , B Darquié

We introduce a method for classical trajectory calculations to simulate collisions between atoms and large rigid asymmetric-top molecules. Using this method, we investigate the formation of molecule-helium complexes in buffer-gas cooling…

Chemical Physics · Physics 2015-06-03 Zhiying Li , Eric J. Heller

The methods producing cold molecules from cold atoms tend to leave molecular ensembles with substantial residual internal energy. For instance, Cs2 molecules initially formed via photoassociation of cold Cs atoms are in several vibrational…

An excellent molecule-based cryogenic magnetic refrigerant, gadolinium acetate tetrahydrate, is here used to decorate selected portions of silicon substrate. By quantitative magnetic force microscopy for variable applied magnetic field near…

We describe a method for cooling neutral molecules that have magnetic and electric dipole moments using collisions with cold ions. An external magnetic field is used to split the ground rovibrational energy levels of the molecule. The…

Atomic Physics · Physics 2014-08-22 F. Robicheaux

Alkaline-earth-like transition-metal atoms such as Zn and Cd are promising candidates for precision measurements and quantum many-body physics experiments. Here, we theoretically investigate the properties of diatomic molecules containing…

Atomic Physics · Physics 2021-11-02 Klaudia Zaremba-Kopczyk , Michał Tomza
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