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We conduct a theoretical and numerical study on the second-harmonic (SH) optical response of a nano-structured metamaterial composed of a periodic array of inclusions. Both the inclusions and their surrounding matrix are made of…

Mesoscale and Nanoscale Physics · Physics 2019-03-13 Ulises R. Meza , Bernardo S. Mendoza , W. Luis Mochán

Efficient electrical generation of mid-infrared light is challenging because of the dearth of materials with natural dipole-active electronic transitions in this spectral region. One approach to solve this problem is through…

Mesoscale and Nanoscale Physics · Physics 2023-04-25 Christopher R. Gubbin , Simone De Liberato

We demonstrate second order optical nonlinearity in aluminum nitride on insulator substrates. Using sputter-deposited aluminum nitride thin films we realize nanophotonic waveguides coupled to micro-ring resonators that simultaneously…

Optics · Physics 2012-06-13 W. H. P. Pernice , C. Xiong , C. Schuck , H. X. Tang

We use ultrafast laser pulses to experimentally demonstrate that the second-order optical response of bulk single crystals of the topological insulator Bi$_2$Se$_3$ is sensitive to its surface electrons. By performing surface doping…

Materials Science · Physics 2011-02-02 D. Hsieh , J. W. McIver , D. H. Torchinsky , D. R. Gardner , Y. S. Lee , N. Gedik

Second harmonic generation is enhanced at the surface lattice resonance in plasmonic nanoparticle arrays. We carried out a parametric investigation on two-dimensional lattices composed of gold nanobars where the centrosymmetry is broken at…

The resonance effects on the optical second harmonic generation from 140 nm silver nanoparticles is studied experimentally by hyper-Rayleigh scattering and numerically by finite element method calculations. We find that the interferences…

By combining analytical and numerical approaches, we study resonantly enhanced second-harmonic generation (SHG) by individual high-index dielectric nanoparticles made of centrosymmetric materials. Considering both bulk and surface…

Optics · Physics 2018-01-08 Daria Smirnova , Alexander I. Smirnov , Yuri S. Kivshar

The second harmonic generation is one of the most important applications of nonlinear effect, which has attracted great interests in nonlinear optics and microwave in the past decades. To the best of our knowledge, however, generating the…

Plasmonic metasurfaces have emerged as a promising platform for enhancing a range of nonlinear optical processes, offering compact geometry and flexibility in light manipulation. Second order nonlinear processes, like second harmonic…

Organic cavity polaritons are bosonic quasi-particles that arise from the strong interaction between organic molecular excitons and photons within microcavities. The spectral dispersion of third harmonic generation near resonance with the…

Optics · Physics 2018-10-08 Bin Liu , Michael Crescimanno , Robert J. Twieg , Kenneth D. Singer

Second-harmonic generation (SHG) is a second-order nonlinear optical process that is not allowed in media with inversion sym-metry. However, due to the broken symmetry at the surface, surface SHG still occurs, but is generally small. We…

Second-order optical nonlinear effects (second-harmonic and sum-frequency generation) are demonstrated in the telecommunication band by periodic poling of thin films of lithium niobate wafer-bonded on silicon substrates and rib-loaded with…

The goal of nanophotonics is to control and manipulate light at length scales below the diffraction limit. Typically nanostructured metals are used for this purpose, light being confined by exploiting the surface plasmon-polaritons such…

Mesoscale and Nanoscale Physics · Physics 2017-05-24 Martin J. Gentile , William L. Barnes

Dielectric metasurfaces have shown prominent applications in nonlinear optics due to strong field enhancement and low dissipation losses at the nanoscale. Chalcogenide glasses are one of the promising materials for the observation of…

We present a combined experimental and theoretical study of enhanced third-harmonic generation (THG) in silicon nitride metasurfaces. These structures exhibit strong resonant nonlinear responses, enabling up to two orders of magnitude…

We experimentally demonstrate long-wave infrared-visible sum-frequency generation microscopy for imaging polaritonic resonances of infrared (IR) nanophotonic structures. This nonlinear-optical approach provides direct access to the resonant…

Efficient nonlinear wave mixing is of paramount importance for a wide range of applications. However, weak optical nonlinearities pose significant challenges for accessing nonlinear light-matter interaction in compact systems. Here, we…

We present a theoretical study of second-harmonic generation from a singular metasurface. The singular metasurfaces strongly interact with the incident light, where the large field enhancement forms an intense surface polarization that…

Optics · Physics 2023-01-10 Fan Yang , Cristian Ciracì

Resonant metasurfaces have received extensive attention due to their sharp spectral feature and extraordinary field enhancement. In this work, by breaking the in-plane symmetry of silicon nanopillars, we achieve a sharp Fano resonance. The…

Optics · Physics 2020-04-06 Chaobiao Zhou , Shiyu Li , Cheng Gong , Yi Wang , Xiaojun Liu , Mingsheng Zhan

The mid-infrared spectral region presents significant potential for sensing and spectroscopic applications. However, traditional plasmonic materials exhibit substantial optical losses within this range, thereby constraining their…