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Analytic approximations to the ground-state energy of closed-shell quantum dots (number of electrons from 2 to 210) are presented in the form of two-point Pade approximants. These Pade approximants are constructed from the small- and…

Condensed Matter · Physics 2009-10-30 A. Gonzalez , B. Partoens , F. M. Peeters

The applicability of the Hartree-Fock and random phase approximations to models of strongly correlated electrons is discussed. The 2D Hubbard model is analyzed. An antiferromagnetic phase (at half filling) and Fermi liquid behavior (at low…

Condensed Matter · Physics 2007-05-23 F. Guinea , E. Louis , J. A. Verges

We perform Random Phase Approximation (RPA) study of collective excitations in the bose-fermi mixed degenerate gas of Alkali-metal atoms at T=0. The calculation is done by diagonalization in a model space composed of particle-hole type…

Condensed Matter · Physics 2009-11-07 T. Sogo , T. Miyakawa , T. Suzuki , H. Yabu

We report an improved implementation for evaluating the analytical gradients of the random phase approximation (RPA) electron-correlation energy based on atomic orbitals and the localized resolution of identity scheme. The more efficient…

Materials Science · Physics 2024-04-17 Muhammad N. Tahir , Honghui Shang , Jia Li , Xinguo Ren

We present a new methodology to analyze complicated multi-physics simulations by introducing a fictitious parameter. Using the method, we study quantum mechanical aspects of an organic molecule in water. The simulation is variationally…

Chaotic Dynamics · Physics 2007-05-23 Toshiya Takami , Jun Maki , Jun-ichi Ooba , Taizo Kobayashi , Rie Nogita , Mutsumi Aoyagi

With increasing inter-electronic distance, the screening of the electron-electron interaction by the presence of other electrons becomes the dominant source of electron correlation. This effect is described by the random phase approximation…

Chemical Physics · Physics 2022-09-29 Arno Förster

Nonperturbative renormalization and explicit construction of the effective potential of the Hartree approximation of the two-particle-irreducible formalism are carried out in an inhomogeneous field configuration describing a uniform…

High Energy Physics - Phenomenology · Physics 2015-06-23 G. Fejos

We analyzed the Hartree-Fock approximation for an electron system. The interaction between particles is modeled by a non-Coulombian potential. We analyzed both the three-dimensional and two-dimensional systems. We obtained accurate…

Quantum Gases · Physics 2024-08-28 Vlad-Mihai Ene , Ilinca Lianu , Ioan Grosu

We present a formulation and implementation of second-order quasidegenerate N-electron valence perturbation theory (QDNEVPT2) that provides a balanced and accurate description of spin-orbit coupling and dynamic correlation effects in…

Chemical Physics · Physics 2024-06-19 Rajat Majumder , Alexander Yu. Sokolov

A new efficient numerical algorithm for interacting fermion systems is proposed and examined in detail. The ground state is expressed approximately by a linear combination of numerically chosen basis states in a truncated Hilbert space. Two…

Strongly Correlated Electrons · Physics 2007-05-23 Tsuyoshi Kashima , Masatoshi Imada

A practical electronic structure method in which a two-body functional is the fundamental variable is constructed. The basic formalism of our method is equivalent to Hartree-Fock density matrix functional theory [M. Levy in {\it Density…

Other Condensed Matter · Physics 2008-04-23 Balazs Hetenyi , Andreas W. Hauser

By coupling a doorway state to a see of random background states, we develop the theory of doorway states in the framework of the random-phase approximation (RPA). Because of the symmetry of the RPA equations, that theory is radically…

Nuclear Theory · Physics 2015-06-22 A. De Pace , A. Molinari , H. A. Weidenmueller

Atomic properties such as field shift constants, magnetic dipole and electric quadrupole hyperfine structure constants, Land\'e $g_J$ factors, and electric quadrupole moments that are described by electronic operators with different ranks…

Atomic Physics · Physics 2018-03-14 Pradeep Kumar , Cheng-Bin Li , B. K. Sahoo

We reconsider the theory of the half-filled lowest Landau level using the Chern-Simons formulation and study the grand-canonical potential in the random-phase approximation (RPA). Calculating the unperturbed response functions for current-…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 J. Dietel , Th. Koschny , W. Apel , W. Weller

Many modern semiempirical molecular orbital models are built on the neglect of diatomic differential overlap (NDDO) approximation. An in-depth understanding of this approximation is therefore indispensable to rationalize the success of…

Chemical Physics · Physics 2018-10-30 Tamara Husch , Markus Reiher

We use a spin-rotational invariant Gutzwiller energy functional to compute random-phase-approximation-like (RPA) fluctuations on top of the Gutzwiller approximation (GA). The method can be viewed as an extension of the previously developed…

Strongly Correlated Electrons · Physics 2008-06-16 G. Seibold , F. Becca , P. Rubin , J. Lorenzana

The Pauli exclusion principle can be stated as inequality $<\psi|\rho|\psi>\le 1$ for the electron density matrix $\rho$. Nowadays it is replaced by skew symmetry of the multi-electron wave function. The replacement leads to numerous…

Quantum Physics · Physics 2009-04-15 Alexander A. Klyachko

We test a set of multiconfigurational wavefunction approaches for calculating the ground state electron population for a two-site Anderson model representing a molecule on a metal surface. In particular, we compare (i) a Hartree Fock like…

Chemical Physics · Physics 2022-07-19 Junhan Chen , Wenjie Dou , Joseph Subotnik

The connections between the Random Phase Approximation (RPA) and Many-Body Perturbation Theory (MBPT) and its all order generalisation, the Coupled- Cluster Theory (CCT) have been explored. Explicit expressions have been derived for the…

We show that the spin-and-space unrestricted Hartree-Fock method, in conjunction with the companion step of the restoration of spin and space symmetries via Projection Techniques (when such symmetries are broken), is able to describe the…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Constantine Yannouleas , Uzi Landman