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The crossover from localized- to itinerant-electron behavior is associated with many intriguing phenomena in condensed-matter physics. In this paper, we investigate the crossover from localized to itinerant regimes in the spinel system…

Strongly Correlated Electrons · Physics 2015-07-20 J. Ma , J. H. Lee , S. E. Hahn , Tao Hong , H. B. Cao , A. A. Aczel , Z. L. Dun , M. B. Stone , W. Tian , Y. Qiu , J. R. D. Copley , H. D. Zhou , R. S. Fishman , M. Matsuda

We demonstrate via a muon spin rotation experiment that the electronic ground state of the iridium spinel compound, CuIr$_2$S$_4$, is not the presumed spin-singlet state but a novel paramagnetic state, showing a quasistatic spin glass-like…

Strongly Correlated Electrons · Physics 2014-02-27 K. M. Kojima , 2 R. Kadono , M. Miyazaki , M. Hiraishi , I. Yamauchi , A. Koda , Y. Tsuchiya , H. S. Suzuki , H. Kitazawa

We explore the magnetic phases in a Kondo lattice model on the geometrically frustrated Shastry-Sutherland lattice at metallic electron densities, searching for noncollinear and noncoplanar spin textures. Motivated by experimental…

Strongly Correlated Electrons · Physics 2017-12-05 Munir Shahzad , Pinaki Sengupta

We report a systematic enhancement of the pressure dependence of TN in A2+[V2]O4 spinels as the V-V separation approaches the critical separation for a transition to itinerant-electron behavior. An intermediate phase between localized and…

Frustrated systems are ubiquitous and interesting because their behavior is difficult to predict. Magnetism offers extreme examples in the form of spin lattices where all interactions between spins cannot be simultaneously satisfied. Such…

Strongly Correlated Electrons · Physics 2009-11-07 S. -H. Lee , C. Broholm , W. Ratcliff , G. Gasparovic , Q. Huang , T. H. Kim , S. -W. Cheong

We study the interplay between magnetic frustration and itinerant electrons. For example, how does the coupling to mobile charges modify the properties of a spin liquid, and does the underlying frustration favor insulating or conducting…

Statistical Mechanics · Physics 2015-06-03 L. D. C. Jaubert , Swann Piatecki , Masudul Haque , R. Moessner

Magnetic systems are fertile ground for the emergence of exotic states when the magnetic interactions cannot be satisfied simultaneously due to the topology of the lattice - a situation known as geometrical frustration. Spinels, AB2O4, can…

Strongly Correlated Electrons · Physics 2015-05-13 M. Matsuda , H. Ueda , A. Kikkawa , Y. Tanaka , K. Katsumata , Y. Narumi , T. Inami , Y. Ueda , S. -H. Lee

Electronic and magnetic properties of molybdenum pyrochlores A2Mo2O7 are studied by the fully relativistic density-functional theory plus on-site repulsion (U) method, with focusing on the spin-glass insulating material Y2Mo2O7. We find…

Strongly Correlated Electrons · Physics 2013-11-27 Hiroshi Shinaoka , Yukitoshi Motome , Takashi Miyake , Shoji Ishibashi

We report on x-ray diffraction, magnetic susceptibility, electron- spin resonance and heat- capacity studies of Co[Al_1-xCo_x]_2O_4 for Co concentrations 0<x<1. In this spinel system only the A-site Co^2+ cation is magnetic, while the…

Materials Science · Physics 2009-11-13 N. Tristan , V. Zestrea , G. Behr , R. Klingeler , B. Buechner , H. A. Krug von Nidda , A. Loidl , V. Tsurkan

The pronounced enhancement of the effective mass is the primary phenomenon associated with strongly correlated electrons. In the presence of local moments, the large effective mass is thought to arise from Kondo coupling, the interaction…

Strongly Correlated Electrons · Physics 2015-06-12 Yasuhiro Shimizu , Hikaru Takeda , Moe Tanaka , Masayuki Itoh , Seiji Niitaka , Hidenori Takagi

This work examines the effects of magnetic frustration due to competing ferromagnetic and antiferromagnetic Heisenberg interactions on the spin dynamics of the double-exchange model. When the local moments are non-colinear, a charge-density…

Strongly Correlated Electrons · Physics 2009-11-10 R. S. Fishman

The ground state of the frustrated A-site magnetic spinel CoAl2O4 has been a controversial issue whether it is a collinear antiferromagnetic ordering or a spiral spin - liquid state, as the ratio of the two competing interactions, J2/J1…

Strongly Correlated Electrons · Physics 2018-03-22 Somnath Ghara , N. V. Ter-Oganessian , A. Sundaresan

Spin textures with nontrivial topology, such as vortices and skyrmions, have attracted attention as a source of unconventional magnetic, transport, and optical phenomena. Recently, a new generation of topological spin textures has been…

Strongly Correlated Electrons · Physics 2021-11-08 Satoru Hayami , Yukitoshi Motome

By studying the dielectric properties of the geometrically frustrated spinel CdV2O4, we observe ferroelectricity developing at the transition into the collinear antiferromagnetic ground state. In this multiferroic spinel, ferroelectricity…

The inversion and volume effects on magnetism in a spinel-type magnetically frustrated compound, CoAl2O4, and its gallium-substituted system, CoAl2-xGaxO4, were investigated. Magnetically frustrated Co2+ with spin S = 3/2 on the tetrahedral…

Frustration in spin system can give rise to unique ordered states and as a consequence several physical phenomena are expected such as multiferroics, high temperature superconductors and anomalous hall effect. Here we report the "new…

Strongly Correlated Electrons · Physics 2018-08-01 GiBaik Sim , SungBin Lee

In both spinel compounds GeCo$_2$O$_4$ and GeNi$_2$O$_4$ which order antiferromagnetically (at $T_N = 23.5 K$ and $T_{N_1} = 12.13 K$, $T_{N_2} = 11.46 K$) with different Curie Weiss temperatures ($T_{CW}$=80.5 K and -15 K), the usual…

Strongly Correlated Electrons · Physics 2009-11-11 Sébastien Diaz , Sophie De Brion , G. Chouteau , Benjamin Canals , Virginie Simonet , P. Strobel

We performed nuclear magnetic resonance (NMR) and muon spin relaxation ({\mu}SR) experiments to identify the magnetic ground state of the frustrated quantum A-site spinel, CuAl2O4. Our results verify that the ground state does not exhibit a…

Magnetic frustration, which is well-defined in insulating systems with localized magnetic moments, yields exotic ground states like spin ices, spin glasses, or spin liquids. In metals magnetic frustration is less well defined because of the…

The combination of localized magnetic moments, their frustration and interaction with itinerant electrons is a key challenge of condensed matter physics. Frustrated magnetic interactions promote degenerate ground states with enhanced…

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