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Finite symmetry adaptation techniques are applied to the determination of the intensity strength of two-photon transitions for ions with one partly-filled shell nl in crystalline environments of symmetry G. We treat the case of intra-…

Atomic and Molecular Clusters · Physics 2007-05-23 M. Kibler , M. Daoud

Experimental measurements of the second order susceptibilities for the second harmonic generation are reported for YAl3(BO3)4 (YAB) single crystals for the two principal tensor components xyz and yyy. First principles calculation of the…

Materials Science · Physics 2008-05-13 Ali H. Reshak , S. Auluck , A. Majchrowski , I. V. Kityk

Surface-enhanced optical third-harmonic generation (THG) is observed in silver island films. The THG intensity from Ag nanoparticles is enhanced by more than two orders of magnitude with respect to the THG intensity from a smooth and…

Other Condensed Matter · Physics 2009-11-11 E. M. Kim , S. S. Elovikov , T. V. Murzina , A. A. Nikulin , O. A. Aktsipetrov , M. A. Bader , G. Marowsky

Structural, magnetic and electrical-transport properties of {\alpha}-LiFeO2, crystallizing in the rock salt structure with random distribution of Li and Fe ions, have been studied by synchrotron X-ray diffraction, 57Fe M\"ossbauer…

Strongly Correlated Electrons · Physics 2017-09-29 Samar Layek , Eran Greenberg , Weiming Xu , Gregory Kh. Rozenberg , Moshe P. Pasternak , Jean-Paul Itié , Dániel G. Merkel

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

We report ionic strength-dependent phase shifts in second harmonic generation (SHG) signals from charged interfaces that verify a recent model in which dispersion between the fundamental and second harmonic beams modulates observed signal…

Solution viscosities of a polycation and a polyanion in NaCl-water: HSAB-guided rheology The zero-shear viscosities of poly(3-acrylamido-propyl-trimethyl-ammonium-chloride) (PAPTMAC-Cl, M ~ 7.8 kDa) and poly(styrene-sulfonate sodium)…

Soft Condensed Matter · Physics 2026-01-30 Suresha P. Ranganath , Manohar V. Badiger , Bernhard A. Wolf

Experimentally determined empirical formulae for the concentration dependent relative permittivity of aqueous solutions of MgCl$_{2}$ and NiCl$_{2}$ are utilized to calculate the osmotic coefficient and the mean activity coefficient of…

Soft Condensed Matter · Physics 2025-04-01 A. O. Quiñones , Z. Abbas , C. W. Outhwaite , L. B. Bhuiyan

We experimentally study the optical second harmonic generation (SHG) from deep subwavelength gold-silver heterodimer and silver-silver and gold-gold homodimers. Our results show that the SHG from the heterodimer is about an order of…

We experimentally and theoretically investigate the second order nonlinear optical response of metallo-dielectric multilayer structures composed of Ag and Ta2O5 layers, deposited by magnetron sputtering. Second harmonic generation…

We study surface second-harmonic generation (SHG) from a singular plasmonic structure consisting of touching metallic wires. We use the technique of transformation optics and relate the structure to a rather simpler geometry, a slab…

We study the electric double layer near a charged soft surface by using a mean-field approach including non-uniform size effect and solvent polarization. Based on a free energy model, electrostatic potential and number densities of water…

Soft Condensed Matter · Physics 2022-02-10 Jun-Sik Sin , Nam-Hyok Kim , Chung-Sik Sin

Optical second-harmonic generation (SHG) is studied for the confined geometry of a circular cylindrical waveguide or optical fiber. A model situation of high symmetry is considered where the material with nonlinear susceptibility is…

Optics · Physics 2013-09-17 B. U. Felderhof , G. Marowsky

We combine modeling and experiments to investigate second- and third-harmonic generation (SHG/THG) in metal-indium tin oxide (ITO) metasurfaces. Linear optics at normal incidence show moderate field enhancement near the ITO…

Described experimental conditions, reproducibility and optimization for the nonlinear optical effects (SHG, THG) for the diagnostic of functionalization of vertically aligned mesoporous silica thin films activated by silver and copper ions.…

Optics · Physics 2018-06-14 M. Laskowska , D. Vynnyk , J. Jedryka , I. V. Kityk , A. Wojciechowski , D. Kulwas

We reported on the observation of extremely high-density ($>10^{14}$cm$^{-2}$) 2D electron gas in N-polar AlGaN/GaN heterostructures grown on sapphire substrates. Due to introducing the GaN/AlN superlattice (SL) back barrier between the GaN…

Mesoscale and Nanoscale Physics · Physics 2025-01-07 Maciej Matys , Atsushi Yamada , Toshihiro Ohki

Nanoporosity in silicon leads to completely new functionalities of this mainstream semiconductor. In recent years, it has been shown that filling the pores with aqueous electrolytes in addition opens a particularly wide field for modifying…

Materials Science · Physics 2023-12-08 Manuel Brinker , Patrick Huber

While all media can exhibit first-order conductivity describing current linearly proportional to electric field, $E$, the second-order conductivity, $\sigma^{(2)}$ , relating current to $E^2$, is nonzero only when inversion symmetry is…

The structure of the adsorbed layer of alkali ions on the surface of colloidal silica solutions with a particle size of ~27 nm has been studied by reflectometry and diffuse scattering of synchrotron radiation with a photon energy of about…

The extent of ion pairing in solution is an important phenomenon to rationalise transport and thermodynamic properties of electrolytes. A fundamental measure of this pairing is the potential of mean force (PMF) between solvated ions. The…

Chemical Physics · Physics 2024-04-11 Niamh O'Neill , Benjamin X. Shi , Kara Fong , Angelos Michaelides , Christoph Schran