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The appropriateness of including Hg among the transition metals has been debated for a long time. Although the synthesis of HgF$_{4}$ molecules in gas phase was reported before, the molecules show strong instabilities and dissociate.…

Materials Science · Physics 2012-06-14 Xiaoli Wang , Haiqing Lin , Yanming Ma , Mao-Sheng Miao

X-ray diffraction studies showed that the structure of (Sr$_{1-x}$Pr$_x$)TiO$_3$ solid solutions at 300 K changes from the cubic $Pm3m$ to the tetragonal $I4/mcm$ with increasing $x$. The analysis of XANES and EXAFS spectra of the solid…

Materials Science · Physics 2012-07-26 I. A. Sluchinskaya , A. I. Lebedev , A. Erko

Monodispersed strontium titanate nanoparticles were prepared and studied in detail. It is found that ~10 nm as-prepared stoichiometric nanoparticles are in a polar structural state (with possibly ferroelectric properties) over a broad…

The question whether excess electrons in SrTiO3 form free or trapped carriers is a crucial aspect for the electronic properties of this important material. This fundamental ambiguity prevents a consistent interpretation of the puzzling…

Strongly Correlated Electrons · Physics 2018-03-15 Xianfeng Hao , Zhiming Wang , Michael Schmid , Ulrike Diebold , Cesare Franchini

The ability to partially oxidize methane at low temperatures and pressures would have important environmental and economic applications. Although methane oxidation on gold nanoparticles has been observed experimentally, our density…

Materials Science · Physics 2014-08-28 Duncan J. Mowbray , Annapaola Migani , Guido Walther , David M. Cardamone , Angel Rubio

The addition of electron donors to the vacant A site of defect-perovskite structure tungsten trioxide causes a series of structural and chemical phase transitions; for instance, in the well-known case of the sodium tungsten bronzes…

Materials Science · Physics 2009-11-10 Andrew D. Walkingshaw , Nicola A. Spaldin , Emilio Artacho

We suggest that the lithiation of pristine SnO forms a layered Li$_\text{X}$O structure while the expelled tin atoms agglomerate into 'surface' planes separating the Li$_\text{X}$O layers. The proposed lithiation model widely differs from…

Computational Physics · Physics 2015-03-17 Andreas Pedersen , Mathieu Luisier

As titanium is a highly utilized metal for structural light-weighting, its phases, transformation pathways (transition states), and structures have scientific and industrial importance. Impurities, pressure, and temperature control the…

Materials Science · Physics 2017-11-28 N. A. Zarkevich , D. D. Johnson

The equilibrium crystal shape (ECS) of oxygen-covered tungsten micricrystal is studied as a function of temperature. The specially designed ultrafast crystal quenching setup with the cooling rate of 6000 K/s allows to draw conclusions about…

Statistical Mechanics · Physics 2015-05-27 Andrzej Szczepkowicz

Precise control of the chemical valence or oxidation state of vanadium in vanadium oxide thin films is highly desirable for not only fundamental research, but also technological applications that utilize the subtle change in the physical…

Materials Science · Physics 2015-06-23 Shinbuhm Lee , Tricia L. Meyer , Sungkyun Park , Takeshi Egami , Ho Nyung Lee

Data for inelastic processes due to hydrogen atom collisions with manganese and titanium are needed for accurate modeling of the corresponding spectra in late-type stars. In this work excitation and charge transfer in low-energy Mn+H and…

Solar and Stellar Astrophysics · Physics 2020-05-13 Jon Grumer , Paul S. Barklem

Relative abundances of the five stable isotopes of titanium (^46Ti to ^50Ti) are measured for 11 M dwarfs belonging to the thin disk (four stars), thick disk (three stars), the halo (one star), and either the thick or the thin disk (three…

Solar and Stellar Astrophysics · Physics 2009-07-24 J. Chavez , D. L. Lambert

The structural features of the charge ordering states in LuFe2O4 are characterized by in-situ cooling TEM observations from 300K down to 20K. Two distinctive structural modulations, a major q1= (1/3, 1/3, 2) and a weak q2=q1/10 + (0, 0,…

Materials Science · Physics 2009-11-13 Y. Zhang , H. X. Yang , C. Ma , H. F. Tian , J. Q. Li *

The low-temperature (T = 17.5 K) structure of titanium(III)-oxybromide, TiOBr, is reported as a two-fold superstructure of the crystal structure at room temperature. Weak superlattice reflections could be measured with synchrotron radiation…

Materials Science · Physics 2007-05-23 L. Palatinus , A. Schoenleber , S. van Smaalen

Here we present results of accurate wet-chemical redox analyses, revealing that the oxidation number of cobalt in the newly discovered CoO2-layer superconductor, NaxCoO2 yH2O (x ~ 0.36, y ~ 1.3) is ~ 3.46. This value is significantly lower…

Superconductivity · Physics 2007-05-23 Maarit Karppinen , Isao Asako , Teruki Motohashi , Hisao Yamauchi

X-ray and neutron powder diffraction data as a function of temperature are analyzed for the colossal dielectric constant material CaCu3Ti4O12. The local structure is studied using atomic pair distribution function analysis. No evidence is…

Materials Science · Physics 2009-11-10 E. S. Bozin , V. Petkov , P. W. Barnes , P. M. Woodward , T. Vogt , S. D. Mahanti , S. J. L. Billinge

The relatively low Tc of Bi2Sr2CuO6+D allows to study normal-state down to low temperatures and the non-substituted compound is intrinsically strongly overdoped. Hole concentration can be adjusted trough oxygen excess, but few data exist in…

Superconductivity · Physics 2007-05-23 F. Jean , D. Colson , G. Collin , N. Blanchard , A. Forget

Microstructure properties, phase transitions, and charge ordering in the LuFe2O4 materials have been extensively investigated by means of transmission electron microscopy (TEM). The (001) twins as a common defect frequently appear in the…

Strongly Correlated Electrons · Physics 2007-05-23 Y. Zhang , H. X. Yang , C. Ma , H. F. Tian , J. Q. Li *

The physical properties of La$_4$Ni$_3$O$_{10}$ with a 2D-like Ruddlesden-Popper-type crystal structure are extraordinarily dependent on temperature and chemical substitution. By introducing Al$^{3+}$ atoms ($x$) randomly at the Ni-sites,…

The structure and thermodynamic properties of Ti$_x$(HfNbTaZr)$_{(1-x)/4}$ from Refractory High Entropy multicomponent Alloys to pure titanium are investigated employing comprehensive MCSQS realizations of the disordered atomic structure…

Materials Science · Physics 2024-07-18 Asif I. Bhatti , Marwa Al-Houcine , David Tingaud , Sylvain Queyreau
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