Related papers: Discriminating Cascading Processes in Nonlinear Op…
Nonlinear optical signals in the condensed phase are often accompanied by sequences of lower-order processes, known as cascades, which share the same phase matching and power dependence on the incoming fields and are thus hard to…
Microscopic cascading of second-order nonlinearities between two molecules has been proposed to yield an enhanced third-order molecular nonlinear-optical response. In this contribution, we investigate the two-molecule cascaded second…
We investigate whether microscopic cascading of second-order nonlinearities of two molecules in the side-by-side configuration can lead to a third-order molecular nonlinear-optical response that exceeds the fundamental limit. We find that…
Nonlinear optical signals from an assembly of N noninteracting particles consist of an incoherent and a coherent component, whose magnitudes scale \sim N and \sim N(N-1), respectively. A unified microscopic description of both types of…
We propose and theoretically investigate a model to realize cascaded optical nonlinearity with few atoms and photons in one-dimension (1D). The optical nonlinearity in our system is mediated by resonant interactions of photons with…
We propose a method to study the quantum nonlinearity and observe the multiphoton transitions in a multiatom CQED system. We show that by inducing simultaneously destructive quantum interference for the single-photon and two-photon…
Quantum cascaded systems offer the possibility to manipulate a target system with the quantum state of a source system. Here, we study in detail the differences between a direct quantum cascade and coherent/incoherent driving for the case…
Plasmon-enhanced Raman scattering can push single-molecule vibrational spectroscopy beyond a regime addressable by classical electrodynamics. We employ a quantum electrodynamics (QED) description of the coherent interaction of plasmons and…
In broadband quantum optical systems, nonlinear interactions among a large number of frequency components induce complex dynamics that may defy heuristic analysis. In this work we introduce a perturbative framework for factoring out…
Since the discovery of the laser, optical parametric nonlinearities have been at the core of efficient light conversion sources. Typically, thick transparent crystals or quasi-phase matched waveguides, are utilized in conjunction with…
This work introduces a theoretical framework to model the collective dynamics of quantum emitters in highly non-Markovian environments, interacting through the exchange of photons with significant retardations. The formalism consists on a…
In this letter, we investigate the quantum optical properties of driven-dissipative nonlinear systems in a cascade configuration. We show that pumping a nonlinear system with a state having a noncoherent statistics, can improve the…
Nonlinear processes in the quantum regime are essential for many applications, such as quantum-limited amplification, measurement and control of quantum systems. In particular, the field of quantum error correction relies heavily on…
It has now been possible to prepare chain of ions in an entangled state and thus question arises --- how the optical properties of a chain of entangled ions differ from say a chain of independent particles. We investigate nonlinear optical…
New processes associated with the nonlinear optical properties of the electromagnetic vacuum, as predicted by quantum electrodynamics are described. We consider the presence of a static and a rotating magnetic field. The cases of harmonic…
Waveguide QED with cold atoms provides a potent platform for the study of non-equilibrium, many-body, and open-system quantum dynamics. Even with weak coupling and strong photon loss, the collective enhancement of light-atom interactions…
Spontaneous parametric down-conversion is a well-known process in quantum nonlinear optics in which a photon incident on a nonlinear crystal spontaneously splits into two photons. Here we propose an analogous physical process where one…
A cascade of two-level superconducting artificial atoms -- a source and a probe -- strongly coupled to a semi-infinite waveguide is a promising tool for observing nontrivial phenomena in quantum nonlinear optics. The probe atom can scatter…
We investigate simultaneous multiphoton-multiatom processes in atomic gases exposed to laser fields under specific frequency conditions, where multiple atoms are simultaneously excited through the absorption of one laser photon each. These…
Optical microcavities are often used to realize enhanced nonlinear optical interactions for highly efficient second-harmonic generation. With increased pump power, the efficiency of nonlinear frequency conversion can be increased further,…