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The process of internal conversion from excited electronic states is investigated theoretically for the case of the vacuum-ultraviolet nuclear transition of $^{229}{\mathrm Th}$. Due to the very low transition energy, the $^{229}{\mathrm…

Atomic Physics · Physics 2017-03-22 Pavlo V. Bilous , Georgy A. Kazakov , Iain D. Moore , Thorsten Schumm , Adriana Pálffy

The isomeric first excited state of the isotope 229Th exhibits the lowest nuclear excitation energy in the whole landscape of known atomic nuclei. For a long time this energy was reported in the literature as 3.5(5) eV, however, a new…

Nuclear Experiment · Physics 2015-06-12 L. v. d. Wense , P. G. Thirolf , D. Kalb , M. Laatiaoui

The first excited isomeric state of $^{229}$Th possesses the lowest energy among all known excited nuclear states. The expected energy is accessible with today's laser technology and in principle allows for a direct optical laser excitation…

Nuclear Experiment · Physics 2018-01-17 Benedict Seiferle , Lars von der Wense , Peter G. Thirolf

The first excited isomeric state of Th-229 has an exceptionally low energy of only a few eV and could form the gateway to high-precision laser spectroscopy of nuclei. The excitation energy of the isomeric state has been inferred from…

Theoretical considerations are made for the nuclear excitation from the ground state to the 8 eV $^{229m}$Th isomer via near-resonant electron transitions in Sb-like ($q=39+$) thorium ions. The energy of the first excited atomic state…

Atomic Physics · Physics 2025-04-17 Karol Kozioł , Jacek Rzadkiewicz

Direct laser excitation of the lowest known nuclear excited state in $^{229}$Th has been a longstanding objective. It is generally assumed that reaching this goal would require a considerably reduced uncertainty of the isomer's excitation…

The low-lying isomeric state of $^{229}$Th provides unique opportunities for high-resolution laser spectroscopy of the atomic nucleus. We determine the energy of this isomeric state by taking the absolute energy difference between the…

Excitation of the anomalously low lying nuclear isomer $^{229m}$Th$(3/2^+, 8.28 \pm 0.17$ eV) in the process of inelastic electron scattering is studied theoretically in the framework of the perturbation theory for the quantum…

Nuclear Theory · Physics 2020-07-01 E. V. Tkalya

The 7.6 eV electromagnetic transition between the nearly degenerate ground state and first excited state in the Th-229 nucleus may be very sensitive to potential changes in the fine-structure constant, $\alpha = e^2/\hbar c$. However, the…

Atomic Physics · Physics 2010-04-22 J. C. Berengut , V. A. Dzuba , V. V. Flambaum , S. G. Porsev

$^{229}$Th is the only known nucleus with an excited state that offers the possibility for a direct laser excitation using existing laser technology. Its excitation energy has been measured indirectly to be 7.8(5) eV ($\approx$160 nm). The…

Instrumentation and Detectors · Physics 2018-12-14 Benedict Seiferle , Lars von der Wense , Ines Amersdorffer , Nicolas Arlt , Benjamin Kotulski , Peter G. Thirolf

The Thorium-229 isotope features a nuclear isomer state with an extremely low energy. The currently most accepted energy value, 7.8 +- 0.5 eV, was obtained from an indirect measurement using a NASA x-ray microcalorimeter with an…

We consider the excitation of the nuclear transition ^{229g}Th - ^{229m}Th near 7.6 eV in singly ionized thorium via an electronic bridge process. The process relies on the excitation of the electron shell by two laser photons whose sum…

Atomic Physics · Physics 2010-10-27 S. G. Porsev , V. V. Flambaum , E. Peik , Chr. Tamm

We estimate the range of the radiative lifetime and energy of the anomalous, low-energy $3/2^+(7.8 \pm 0.5$ eV) state in the $^{229}$Th nucleus. Our phenomenological calculations are based on the available experimental data for the…

Atomic Physics · Physics 2015-12-09 E. V. Tkalya , Christian Schneider , Justin Jeet , Eric R. Hudson

The first nuclear excited state of $^{229}$Th offers the unique opportunity for laser-based optical control of a nucleus. Its exceptional properties allow for the development of a nuclear optical clock which offers a complementary…

A process of the decay of the anomalously low lying nuclear isomer $^{229m}$Th$(3/2^+,8.28 \pm 0.17$ eV) in the Thorium anion (Th$^-$) via the internal conversion (IC) channel is studied. We show that the half life of the nuclear isomer in…

Nuclear Theory · Physics 2020-05-20 E. V. Tkalya , R. Si

The nuclear transition between the ground and the low-energy isomeric state in the ^{229}Th nucleus is of interest due to its high sensitivity to a hypothetical temporal variation of the fundamental constants and a possibility to build a…

Atomic Physics · Physics 2021-05-04 S. G. Porsev , C. Cheung , M. S. Safronova

Nuclear excitation cross section of $^{229}$Th from the ground state to the low-lying isomeric state via inelastic electron scattering is calculated, on the level of Dirac distorted wave Born approximation. With electron energies below 100…

Nuclear Theory · Physics 2022-07-19 Hanxu Zhang , Wu Wang , Xu Wang

We present a measurement of the low-energy (0--60$\,$keV) $\gamma$ ray spectrum produced in the $\alpha$-decay of $^{233}$U using a dedicated cryogenic magnetic micro-calorimeter. The energy resolution of $\sim$$10\,$eV, together with…

The excitation energy of $ {}^{229m} \mathrm{Th} $ is extremely low at $ 8.4 \, \mathrm{eV} $; thus, this isotope exhibits changes in its decay modes depending on the chemical state, specifically the outermost electronic states. However,…

Here, we report the first demonstration of laser-induced conversion electron M\"{o}ssbauer spectroscopy of the $^{229}$Th nuclear isomeric state, which provides the ability to probe the nuclear transition in a material that is opaque to…

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