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Excitation of a metallic ferromagnet such as Ni with an intensive femtosecond laser pulse causes an ultrafast demagnetization within approximately 300 fs. It was proposed that the ultrafast demagnetization measured in femtosecond…

Materials Science · Physics 2016-09-27 Ritwik Mondal , Marco Berritta , Karel Carva , Peter M. Oppeneer

We theoretically investigate the generation of ultrafast currents in insulators induced by strong few-cycle laser pulses. Ab initio simulations based on time-dependent density functional theory give insight into the atomic-scale properties…

Laser-induced ultrafast demagnetization is a phenomenon of utmost interest and attracts significant attention because it enables potential applications in ultrafast optoelectronics and spintronics. As a spin-orbit coupling assisted magnetic…

Stoner and Heisenberg excitations in magnetic materials are inherently different. The former involves an effective reduction of the exchange splitting, whereas the latter comprises excitation of spin-waves. In this work, we test the impact…

Materials Science · Physics 2022-03-14 Mohamed F. Elhanoty , Olle Eriksson , Ronny Knut , Olof Karis , Oscar Grånäs

Femtosecond laser excitation of materials that exhibit magnetic spin textures promises advanced magnetic control via the generation of ultrafast and non-equilibrium spin dynamics. We explore such possibilities in ferrimagnetic [Fe(0.35…

Recent developments of the sources of intense and ultrashort X-ray pulses stimulate theoretical studies of phenomena occurring on ultrafast timescales. In the present study, spin-flip dynamics in transition metal complexes triggered by…

Chemical Physics · Physics 2020-08-26 Vladislav Kochetov , Huihui Wang , Sergey I. Bokarev

Optical pump-probe setups are commonly used for excitation and investigation of the spin dynamics in various types of magnetic materials. However, usually the spatially homogeneous excitation is considered. In the present study we describe…

Real-time time-dependent density functional theory, in conjunction with the Ehrenfest molecular dynamics scheme, is becoming a popular methodology to investigate ultrafast phenomena on the nanoscale. Thanks to recent developments, it is…

Materials Science · Physics 2020-08-18 Jannis Krumland , Ana M. Valencia , Stefano Pittalis , Carlo A. Rozzi , Caterina Cocchi

All-optical switching in a ferromagnetic spin valve is studied here using atomistic spin drift-diffusion dynamics, which includes contributions from spin pumping and superdiffusive transport. We find the switching is governed principally by…

Mesoscale and Nanoscale Physics · Physics 2026-02-23 Serban Lepadatu , Mohammed Gija , Alexey Dobrynin , Kevin McNeill , Mark Gubbins , Tim Mercer , Steven M. McCann , Philip Bissell

Synthetic ferrimagnets are composite magnetic structures formed from two or more anti- ferromagnetically coupled magnetic sublattices with different magnetic moments. Here we report on atomistic spin simulations of the laser-induced…

Materials Science · Physics 2014-06-10 Richard F. L. Evans , Thomas A. Ostler , Roy W. Chantrell , Ilie Radu , Theo Rasing

Experimentally observed ultrafast all-optical magnetization reversal in ferrimagnetic metals and heterostructures based on antiferromagnetically coupled ferromagnetic $d-$ and $f-$metallic layers relies on intricate energy and angular…

Strongly Correlated Electrons · Physics 2016-03-02 Alexandra Kalashnikova , Veniamin Kozub

Understanding how fast short-range interactions build up long-range order is one of the most intriguing topics in condensed matter physics. FeRh is a test specimen for studying this problem in magnetism, where the microscopic spin-spin…

Deterministic all-optical control of magnetization without an applied magnetic field has been reported for different materials such as ferrimagnetic and ferromagnetic thin films and granular recording media. These findings have challenged…

Quantum mechanical superexchange interactions form the basis of quantum magnetism in strongly correlated electronic media. We report on the direct measurement of superexchange interactions with ultracold atoms in optical lattices. After…

Other Condensed Matter · Physics 2008-04-17 S. Trotzky , P. Cheinet , S. Fölling , M. Feld , U. Schnorrberger , A. M. Rey , A. Polkovnikov , E. A. Demler , M. D. Lukin , I. Bloch

We have performed time-resolved resonant x-ray scattering studies in the Lanthanide metal Dy to reveal the dynamic response of the helical order exchange coupling to injection of unpolarized spins. The observed spin dynamics are…

By combining interface-sensitive non-linear magneto-optical experiments with femtosecond time resolution and ab-initio time-dependent density functional theory, we show that optically excited spin dynamics at Co/Cu(001) interfaces proceeds…

Materials Science · Physics 2019-02-20 J. Chen , U. Bovensiepen , A. Eschenlohr , T. Müller , P. Elliott , E. K. U. Gross , J. K. Dewhurst , S. Sharma

Faster magnetic recording technology is indispensable to massive data storage and big data sciences. {All-optical spin switching offers a possible solution}, but at present it is limited to a handful of expensive and complex rare-earth…

Materials Science · Physics 2016-11-03 G. P. Zhang , Y. H. Bai , T. F. George

The ultimate control of magnetic states of matter at femtosecond (or even faster) timescales defines one of the most pursued paradigm shifts for future information technology. In this context, ultrafast laser pulses developed into extremely…

Mesoscale and Nanoscale Physics · Physics 2022-03-15 Hanan Hamamera , Filipe Souza Mendes Guimarães , Manuel dos Santos Dias , Samir Lounis

The anti-Stoner excitations are a spin-flips in which, effectively, an electron is promoted from a minority to a majority spin state, i.e., complementary to Stoner excitations and spin-waves. Since their spectral power is negligible in…

Materials Science · Physics 2024-06-21 S. Paischer , D. Eilmsteiner , M. I. Katsnelson , A. Ernst , P. A. Buczek

Starting from the continuity equation for the magnetization in time-dependent spin-density functional theory, we derive an expression for the effective time-dependent magnetic fields driving the out-of-equilibrium spin dynamics in magnetic…

Mesoscale and Nanoscale Physics · Physics 2017-01-18 Jacopo Simoni , Maria Stamenova , Stefano Sanvito