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Charge separated interlayer excitons in transition metal dichalcogenide (TMDC) heterobilayers are being explored for moir\'e exciton lattices and exciton condensates. The presence of permanent dipole moments and the poorly screened Coulomb…

Mesoscale and Nanoscale Physics · Physics 2021-03-17 Jue Wang , Qianhui Shi , En-Min Shih , Lin Zhou , Wenjing Wu , Yusong Bai , Daniel A. Rhodes , Katayun Barmak , James Hone , Cory R. Dean , X. -Y. Zhu

We have combined spatially-resolved steady-state micro-photoluminescence ($\mu$PL) with time-resolved photoluminescence (TRPL) to investigate the exciton diffusion in a WSe$_2$ monolayer encapsulated with hexagonal boron nitride (hBN). At…

Mesoscale and Nanoscale Physics · Physics 2018-05-09 F. Cadiz , C. Robert , E. Courtade , M. Manca , L. Martinelli , T. Taniguchi , K. Watanabe , T. Amand , A. C. H. Rowe , D. Paget , B. Urbaszek , X. Marie

We consider the scenario of excitons in a semiconductor bilayer that are strongly coupled to cavity photons, leading to the formation of dipolar exciton polaritons (dipolaritons). Using a realistic pseudopotential for the dipolar…

Mesoscale and Nanoscale Physics · Physics 2026-02-27 Yasufumi Nakano , Olivier Bleu , Brendan C. Mulkerin , Jesper Levinsen , Meera M. Parish

Excitons in bilayer transition metal dichalcogenides (2L-TMDs) are Coulomb-bound electron/hole pairs that can be viewed as broadly tunable analogs of atomic or molecular systems. Here, we study the properties of 2L-TMD excitons under strong…

Mesoscale and Nanoscale Physics · Physics 2023-03-20 S. Kovalchuk , K. Greben , A. Kumar , S. Pessel , K. Watanabe , T. Taniguchi , D. Christiansen , M. Selig , A. Knorr , K. I. Bolotin

The region surrounding the excitonic insulator phase is a three-component plasma composed of electrons, holes, and excitons. Due to the extended nature of the excitons, their presence influences the surrounding electrons and holes. We…

Strongly Correlated Electrons · Physics 2015-06-22 B Zenker , D Ihle , F X Bronold , H Fehske

We report on scattering induced valley polarization enhancement in monolayer molybdenum disulfide. With thermally activated and charge doping introduced scattering, our sample exhibits seven? and twelve-folds of improvements respectively.…

Optics · Physics 2021-10-13 Yueh-Chun Wu , Takashi Taniguchi , Kenji Watanabe , Jun Yan

Transition metal dichalcogenide (TMDC) heterostructures have unique properties that depend on the twisting angle and stacking order of two or more monolayers. However, their practical applications are limited by the low photoluminescence…

We theoretically studied the exciton geometric structure in layered semiconducting transition metal dichalcogenides. Based on a three-orbital tight-binding model for Bloch electrons which incorporates their geometric structures, an…

Mesoscale and Nanoscale Physics · Physics 2024-03-11 Jianju Tang , Songlei Wang , Hongyi Yu

We have experimentally determined the energies of the ground and first four excited excitonic states of the fundamental optical transition in monolayer WS2, a model system for the growing class of atomically thin two-dimensional…

Optically generated excitons dictate the absorption and emission spectrum of doped semiconductor transition metal dichalcogenide monolayers. We show that upon increasing the electron density, the elementary optical excitations develop a…

Mesoscale and Nanoscale Physics · Physics 2020-05-20 Ovidiu Cotlet , Dominik S. Wild , Mikhail D. Lukin , Atac Imamoglu

Interlayer excitons are observed coexisting with intralayer excitons in bi-layer, few-layer, and bulk MoSe2 single crystals by confocal reflection contrast spectroscopy. Quantitative analysis using the Dirac-Bloch-Equations provides…

Materials Science · Physics 2018-06-13 Jason Horng , Tineke Stroucken , Long Zhang , Eunice Y. Paik , Hui Deng , Stephan W. Koch

Transition metal dichalcogenides represent an ideal testbed to study excitonic effects, spin-related phenomena and fundamental light-matter coupling in nanoscopic condensed matter systems. In particular, the valley degree of freedom, which…

Mesoscale and Nanoscale Physics · Physics 2017-05-16 N. Lundt , P. Nagler , A. Nalitov , S. Klembt , M. Wurdack , S. Stoll , T. H. Harder , S. Betzold , V. Baumann , A. V. Kavokin , C. Schüller , T. Korn , S. Höfling , C. Schneider

We report a rare atom-like interaction between excitons in monolayer WS2, measured using ultrafast absorption spectroscopy. At increasing excitation density, the exciton resonance energy exhibits a pronounced redshift followed by an…

As hosts for tightly-bound electron-hole pairs carrying quantized angular momentum, atomically-thin semiconductors of transition metal dichalcogenides provide an appealing platform for optically addressing the valley degree of freedom. In…

Mesoscale and Nanoscale Physics · Physics 2018-10-24 Shao-Yu Chen , Thomas Goldstein , Takashi Taniguchi , Kenji Watanabe , Jun Yan

Two-dimensional semiconductors exhibit pronounced many-body effects and intense optical responses due to strong coulombic interactions. Consequently, subtle differences in photoexcitation conditions can strongly influence how the material…

The electronic states at the direct band gap of monolayer WSe2 at the $K^+$ and $K^-$ valleys are related by time reversal and may be viewed as pseudo-spins. The corresponding optical interband transitions are governed by robust excitons.…

Materials Science · Physics 2015-09-16 G. Wang , M. M. Glazov , C. Robert , T. Amand , X. Marie , B. Urbaszek

Excitons -- bound electron-hole pairs -- play a central role in light-matter interaction phenomena, and are crucial for wide-ranging applications from light harvesting and generation to quantum information processing. A long-standing…

Mesoscale and Nanoscale Physics · Physics 2023-08-15 Jenny Hu , Etienne Lorchat , Xueqi Chen , Kenji Watanabe , Takashi Taniguchi , Tony F. Heinz , Puneet A. Murthy , Thibault Chervy

We address the properties of excitons in monolayer MoS$_2$ from a theoretical point of view, showing that low-energy excitonic states occur both at the Brillouin zone center and at the Brillouin-zone corners, that binding energies at the…

Mesoscale and Nanoscale Physics · Physics 2015-02-25 Fengcheng Wu , Fanyao Qu , A. H. MacDonald

In order to discuss the exciton fine-structure of transition-metal dichalcogenides mono-layers, excitons are first defined in the subspace of electron- and hole states, including the lowest conduction band (LCB) and the uppermost valence…

Mesoscale and Nanoscale Physics · Physics 2019-06-25 Pierre Gilliot , Mathieu Gallart , Bernd Hönerlage

Indirect excitons -- pairs of electrons and holes spatially separated in semiconductor bilayers or quantum wells -- are known to undergo Bose-Einstein condensation and to form a quantum fluid. Here we show that this superfluid may…

Quantum Gases · Physics 2015-03-17 J. Boening , A. Filinov , M. Bonitz
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