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A direct band gap, remarkable light-matter coupling as well as strong spin-orbit and Coulomb interaction establish two-dimensional (2D) crystals of transition metal dichalcogenides (TMDs) as an emerging material class for fundamental…

Two-dimensional semiconductors feature valleytronics phenomena due to locking of the spin and momentum valley of the electrons. However, the valley polarization is intrinsically limited in monolayer crystals by the fast intervalley…

Mesoscale and Nanoscale Physics · Physics 2019-07-10 Long Zhang , Rahul Gogna , G. William Burg , Jason Horng , Eunice Paik , Yu-Hsun Chou , Kyounghwan Kim , Emanuel Tutuc , Hui Deng

Monolayer semiconducting transition metal dichalcogenides possess broken inversion symmetry and strong spin-orbit coupling, which leads to unique spin-valley locking effect. In 2H stacked pristine multilayers, the spin-valley locking yields…

Mesoscale and Nanoscale Physics · Physics 2023-06-07 Yinong Zhang , Chengxin Xiao , Dmitry Ovchinnikov , Jiayi Zhu , Xi Wang , Takashi Taniguchi , Kenji Watanabe , Jiaqiang Yan , Wang Yao , Xiaodong Xu

Excitons in monolayer transition metal dichalcogenides (TMDs) are formed at K and K' points at the boundary of the Brillouin zone. They acquire a valley degree of freedom, which may be used as a complementary platform for information…

Semiconductor microcavity polaritons, formed via strong exciton-photon coupling, provide a quantum many-body system on a chip, featuring rich physics phenomena for better photonic technology. However, conventional polariton cavities are…

Mesoscale and Nanoscale Physics · Physics 2018-05-09 Long Zhang , Rahul Gogna , Will Burg , Emanuel Tutuc , Hui Deng

Microscopic insights into nonlinear interactions are essential for advancing polaritonic devices. Existing studies often rely on phenomenological models that overlook important many-body processes. Based on a material-specific and…

Mesoscale and Nanoscale Physics · Physics 2026-03-31 Jonas K König , Jamie M Fitzgerald , Daniel Erkensten , Ermin Malic

Two-dimensional semiconducting transition metal dichalcogenides embedded in optical microcavities in the strong exciton-photon coupling regime may lead to promising applications in spin and valley addressable polaritonic logic gates and…

We report experimental observation of 2s exciton radiative emission from monolayer tungsten diselenide, enabled by hexagonal boron nitride protected high-quality samples. The 2s luminescence is highly robust and persists up to 150K,…

Mesoscale and Nanoscale Physics · Physics 2018-01-31 Shao-Yu Chen , Thomas Goldstein , Jiayue Tong , Takashi Taniguchi , Kenji Watanabe , Jun Yan

The direct gap interband transitions in transition metal dichalcogenides monolayers are governed by chiral optical selection rules. Determined by laser helicity, optical transitions in either the $K^+$ or $K^-$ valley in momentum space are…

Mesoscale and Nanoscale Physics · Physics 2016-10-26 G. Wang , X. Marie , B. L. Liu , T. Amand , C. Robert , F. Cadiz , P. Renucci , B. Urbaszek

We show that excitons and free carriers in K and K' valleys of transition metal dichalcogenide monolayers can be entangled with respect to their valley degree of freedom by absorbing linearly polarized single photons. This effect does not…

Mesoscale and Nanoscale Physics · Physics 2015-08-12 Mikhail Tokman , Yongrui Wang , Alexey Belyanin

Exciton-polaritons in semiconductor microcavities have advanced to become a model system for studying dynamical Bose-Einstein condensation, macroscopic coherence, many-body effects, nonclassical states of light and matter, and possibly…

Quantum Gases · Physics 2017-03-21 C. Schneider , K. Winkler , M. D. Fraser , M. Kamp , Y. Yamamoto , E. A. Ostrovskaya , S. Hoefling

In monolayer transition metal dichalcogenides, tightly bound excitons have been discovered with a valley pseudospin that can be optically addressed through polarization selection rules. Here, we show that this valley pseudospin is strongly…

Mesoscale and Nanoscale Physics · Physics 2014-05-20 Hongyi Yu , Guibin Liu , Pu Gong , Xiaodong Xu , Wang Yao

Monolayers of transition metal dichalcogenides (TMDCs) are atomically thin direct-gap semiconductors with potential applications in nanoelectronics, optoelectronics, and electrochemical sensing. Recent theoretical and experimental efforts…

Mesoscale and Nanoscale Physics · Physics 2013-02-26 Sanfeng Wu , Chunming Huang , Grant Aivazian , Jason S Ross , David H Cobden , Xiaodong Xu

Excitons in monolayer transition metal dichalcogenide are endowed with intrinsic valley-orbit coupling between their center-of-mass motion and valley pseudospin. When trapped in a confinement potential, e.g., generated by strain field, we…

Mesoscale and Nanoscale Physics · Physics 2023-05-11 Di Zhang , Sha Deng , Dawei Zhai , Wang Yao , Qizhong Zhu

We develop a microscopic theory for excitons and cavity exciton polaritons in transition metal dichalcogenide (TMD) monolayers under a perpendicular static magnetic field. We obtain numerically exact solutions for the ground and excited…

Mesoscale and Nanoscale Physics · Physics 2025-01-27 D. de la Fuente Pico , J. Levinsen , E. Laird , M. M. Parish , F. M. Marchetti

Due to high binding energy and oscillator strength, excitons in thin flakes of transition metal dichalcogenides constitute a perfect foundation for realizing a strongly coupled light-matter system. In this paper we investigate mono- and…

The coupling between spin, charge, and lattice degrees of freedom plays an important role in a wide range of fundamental phenomena. Monolayer semiconducting transitional metal dichalcogenides have emerged as an outstanding platform for…

Integrating two-dimensional van der Waals materials with optical cavities has revealed a fascinating platform to study exciton-polariton physics. Manipulating exciton polaritons often requires external control over the electrical and…

Optics · Physics 2023-11-08 Zhi Wang , Li He , Bumho Kim , Bo Zhen

Heterostructures comprising different monolayer semiconductors provide a new system for fundamental science and device technologies, such as in the emerging field of valleytronics. Here, we realize valley-specific interlayer excitons in…

Mesoscale and Nanoscale Physics · Physics 2016-01-13 Pasqual Rivera , Kyle L. Seyler , Hongyi Yu , John R. Schaibley , Jiaqiang Yan , David G. Mandrus , Wang Yao , Xiaodong Xu

Monolayers of transition metal dichalcogenides, namely, molybdenum and tungsten disulfides and diselenides demonstrate unusual optical properties related to the spin-valley locking effect. Particularly, excitation of monolayers by…

Mesoscale and Nanoscale Physics · Physics 2015-11-12 M. M. Glazov , E. L. Ivchenko , G. Wang , T. Amand , X. Marie , B. Urbaszek , B. L. Liu