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Broadband dielectric spectroscopy (BDS) of pure 5OCB and nanocolloids consisting of 5OCB and paraelectric or ferroelectric BaTiO${_3}$ nanoparticles (NPs) was performed on varying pressure or temperature. We found strong impact of NPs on…

Soft Condensed Matter · Physics 2017-08-16 S. Starzonek , S. J. Rzoska , A. Drozd-Rzoska , Krzysztof Czupryński , S. Kralj

An incommensurate modulated structure was found recently in a light group V element phosphorous in the phase P-IV stable in the pressure range 107-137 GPa. We consider configurations of the Brillouin zone and Fermi sphere within a…

Materials Science · Physics 2015-05-14 Valentina F. Degtyareva

Using first-principles calculations, the phonon frequencies at the $\Gamma$ point and the dielectric tensor are determined and analysed for the cubic and rhombohedral phases of BaTiO$_{3}$. The dipole-dipole interaction is then separated…

mtrl-th · Physics 2009-10-30 Ph. Ghosez , X. Gonze , J. -P. Michenaud

Gadolinium molybdate is a classical example of an improper ferroelectric and ferroelastic material. It is established that the spontaneous polarization arises as a secondary effect, induced by a structural instability in the paraelectric…

Materials Science · Physics 2021-11-29 Inger-Emma Nylund , Maria Tsoutsouva , Tor Grande , Dennis Meier

The effective pair potentials of liquid 3d transition metals have been derived from the experimental diffraction data by means of the inverse self-consistent method. The obtained potentials provide highly accurate coincidence of the…

Materials Science · Physics 2007-05-23 A. Kimmel , I. Gusenkov

While the tetragonal antiferro-electrically distorted (AFD) phase with space group $I4/mcm$ is well known for SrTiO$_3$ to occur below 105 K, there are also some hints in literature of an orthorhombic phase, either at lower temperature at…

Materials Science · Physics 2018-09-27 Churna Bhandari , Walter R. L. Lambrecht

Neutron diffraction and nuclear quadrupole resonance (NQR) measurements were employed to investigate magnetic order in the non-ferroelectric phase preceding the low-temperature multiferroic state in FeTe2O5Br. Refnement of the neutron…

Strongly Correlated Electrons · Physics 2013-04-10 M. Pregelj , P. Jeglič , A. Zorko , O. Zaharko , T. Apih , A. Gradišek , M. Komelj , H. Berger , D. Arčon

Results of the first-principles calculations are presented for the group-VB metals V, Nb and Ta up to couple of megabar pressure. An unique structural phase transition sequence BCC-->(at 60 GPa) rhombohedral (angle=110.5 degree)-->(at ~ 160…

Materials Science · Physics 2009-11-13 Ashok K. Verma , P. Modak

Understanding the response of ceramics operating in extreme environments is of interest for a variety of applications. Ab initio molecular dynamic simulations have been used to investigate the effect of structure and $B$-site (=Ti, Zr)…

Materials Science · Physics 2019-06-04 Michel Sassi , Tiffany Kaspar , Kevin M. Rosso , Steven R. Spurgeon

First-principles calculations were performed to investigate the ferroelectric properties of barium titanate and bismuth ferrite, as well as phonon dispersion of BaTiO3, using density functional theory and density functional perturbation…

Materials Science · Physics 2014-12-08 Hong-Jian Feng

Evidences of a monoclinic phase in unpoled (PbMg1/3Nb2/3O3)1-x-(PbTiO3)x with x=0.35 (PMN-PT 35%) and unpoled (PbZn1/3Nb2/3O3)1-x-(PbTiO3)x with x=0.09 (PZN-PT 9%) are presented from a neutron Rietveld analysis. This monoclinic phase is…

Materials Science · Physics 2009-11-07 J-M. Kiat , Y. Uesu , B. Dkhil , MX. Matsuda , C. Malibert , G. Calvarin

Despite being successfully synthesized [Zhang $et$ $al.$, Nat. Mater. \textbf{20}, 1073 (2021)], the monolayer structure of stable hexagonal TiO$_2$ is unknown, and it is not even clear whether it can exist in a freestanding form. Through…

Materials Science · Physics 2024-04-30 Xiangtian Bu , Haitao Liu , Yuanchang Li

Metal-insulator transitions strongly coupled with lattice were found in Bi1-xLaxNiO3. Synchrotron X-ray powder diffraction revealed that pressure (P ~ 3 GPa, T = 300 K), temperature (T ~ 340 K, x = 0.05), and La-substitution (x ~ 0.075, T =…

Strongly Correlated Electrons · Physics 2009-11-11 S. Ishiwata , M. Azuma , M. Hanawa , Y. Moritomo , Y. Ohishi , K. Kato , M. Takata , E. Nishibori , M. Sakata , I. Terasaki , M. Takano

Polycrystalline La and Ti co-substituted ceramics were synthesized by the tartaric acid modified sol-gel technique. It was observed that the co-substitution of La & Ti at Bi & Fe sites in BiFeO3 suppress the impurity phase formation which…

Materials Science · Physics 2015-06-19 Pawan Kumar , Chandrakanta Panda , Manoranjan Kar

The structural and magnetic properties of YVO3, NdVO3 and TbVO3 were investigated by single-crystal and powder neutron diffraction. YVO3 shows a structural phase transition at 200 K from an orthorhombic structure with the space group Pbnm…

Strongly Correlated Electrons · Physics 2009-11-11 M. Reehuis , C. Ulrich , P. Pattison , B. Ouladdiaf , M. C. Rheinstadter , M. Ohl , L. P. Regnault , M. Miyasaka , Y. Tokura , B. Keimer

The electrodynamics near the metal-to-insulator transitions (MIT) induced, in V3O5 single crystals, by both temperature (T) and pressure (P) has been studied by infrared spectroscopy. The T- and P-dependence of the optical conductivity may…

Strongly Correlated Electrons · Physics 2009-11-13 L. Baldassarre , A. Perucchi , E. Arcangeletti , D. Nicoletti , D. Di Castro , P. Postorino , V. A. Sidorov , S. Lupi

$VO_2$ undergoes the insulator-metal transition (IMT) and monoclinic-rutile structural phase transition (SPT) near $67^oC$. The IMT switching has many applications. However, there is an unresolved issue whether the IMT is a Mott transition…

Strongly Correlated Electrons · Physics 2021-01-18 Chang-Yong Kim , Tetiana Slusar , Jinchul Cho , Hyun-Tak Kim

We have carried out systematic temperature-dependent neutron diffraction measurements in conjunction with dielectric spectroscopy from 6 to 300 K for sodium niobate based compounds (1-x) NaNbO3 -xBaTiO3 (NNBTx). The dielectric constant is…

Materials Science · Physics 2018-05-23 S. K. Mishra , Mrinal Jauhari , R. Mittal , P. S. R. Krishna , V. R. Reddy , S. L. Chaplot

Transition metal oxides are considered promising thermoelectric materials for harvesting high-temperature waste heat due to their stability, abundance and low toxicity. Despite their typically strong ionic character, they can exhibit…

Materials Science · Physics 2019-12-04 Simon Thébaud , Christophe Adessi , Georges Bouzerar

Cooperative Jahn-Teller ordering is well-known to drive the cubic $Fd\overline{3}m$ to tetragonal $I$4$_1$/$amd$ structural distortion in Mn$_3$O$_4$ at 1170 $^{\circ}$C. Further structural distortion occurs in Mn$_3$O$_4$ upon magnetic…

Materials Science · Physics 2014-08-26 Moureen C. Kemei , Jaye K. Harada , Ram Seshadri , Matthew R. Suchomel
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