Related papers: Robust two-level system control by a detuned and c…
We present a novel scheme for coherent manipulation of populations and robust creation of arbitrary coherent superposition of metastable states of a quantum system with lambda configuration of operating energy levels using laser pulses with…
We have studied the effects of chirped femtosecond laser pulses on the formation of ultracold molecules in a Rb magneto-optical trap. We have found that application of chirped femtosecond pulses suppressed the formation of 85Rb-2 and 87Rb-2…
We report an ultrafast and efficient way to create the maximum coherence between the two lower states in a -like atomic systems, driven by two nonlinearly chirped few-cycle pulses. The phenomenon of coherent population trapping and…
In this paper, we investigate coherent control of nonadiabatic dynamics at a conical intersection (CI) using engineered ultrafast laser pulses. Within a model vibronic system, we tailor pulse chirp and temporal profile and compute the…
Coherent control of two-state systems is traditionally achieved by resonant pulses of specific Rabi frequency and duration, by adiabatic techniques using level crossings or delayed pulses, or by sequences of pulses with precise relative…
A dual color, frequency and pulse duration agile laser system, capable of delivering laser pulses in arbitrary temporal profiles with ~1 ns to ~1 us pulse duration, chirping rates of ~27 MHz/ns with an achievable chirping range of several…
We report on coherent control of excitation processes of translationally ultracold rubidium dimers in a magneto-optical trap by using shaped femtosecond laser pulses. Evolution strategies are applied in a feedback loop in order to optimize…
The interaction of chirped femtosecond laser pulses with hybrid materials - materials comprised of plasmon sustaining structures and resonant molecules - is scrutinized using a self-consistent model of coupled Maxwell-Bloch equations. The…
We propose a chirped-pulse driving protocol and reveal its exceptional property for quantum coherent control. The nonadiabatic passage generated by the driving protocol, which includes the population inversion and the…
The first step in the coherent control of a photoinduced binary reaction is bond making or photoassociation. We have recently demonstrated coherent control of bond making in multi-photon femtosecond photoassociation of hot magnesium atoms,…
We have demonstrated that near complete coherence can be achieved in a four level double lambda-like systems using a train of ultra-short optical pulses. The effect of the Doppler broadening has been analyzed and a scheme has been proposed…
We study the efficiency of modulated laser pulses to produce efficient and fast charge localization transitions in a two-electron double quantum dot. We use a configuration interaction method to calculate the electronic structure of a…
The Bloch sphere is a generic picture describing a coupled two-level system and the coherent dynamics of its superposition states under control of electromagnetic fields. It is commonly employed to visualise a broad variety of phenomena…
Quantum coherent control of ultrafast bond making and the subsequent molecular dynamics is crucial for the realization of a new photochemistry, where a shaped laser field is actively driving the chemical system in a coherent way from the…
We report a study on the optical dipole force in a ladder like three level atomic systems in the context of coherent population transfer with the chirped few-cycle-pulse laser fields. The phenomenon of coherent population transfer is…
The effects of Coherent excitation of a two level system with a linearly chirped pulse are studied theoretically and experimentally (in Rb (5s - 5p)) in the low field regime. The Coherent Transients are measured directly on the excited…
The chirped-pulse interaction in the adiabatic coupling regime induces cyclic permutations of the energy states of a three-level system in the $V$-type configuration, which process is known as the three-level chirped rapid adiabatic…
We demonstrate for the first time coherent control of bond making, a milestone on the way to coherent control of photo-induced bimolecular chemical reactions. In strong-field multiphoton femtosecond photoassociation experiments, we find the…
We present a simple approach allowing to obtain analytical expressions for laser pulses that can drive a two-level system in an arbitrarily chosen way. The proposed scheme relates every desired population-evolution path to a single resonant…
We investigate with exact numerical calculation coherent control of a two-level quantum system's decay by subjecting the two-level system to many periodic ideal $2\pi$ phase modulation pulses. For three spectrum intensities (Gaussian,…