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Related papers: Molecular Plasmonics: strong coupling at the low m…

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We demonstrate strong coupling between molecular excited states and surface plasmon modes of a slit array in a thin metal film. The coupling manifests itself as an anti-crossing behavior of the two newly formed polaritons. As the coupling…

Mesoscale and Nanoscale Physics · Physics 2012-08-17 Adi Salomon , Robert J. Gordon , Yehiam Prior , Tamar Seideman , Maxim Sukharev

Strong coupling between light and molecular matter is currently attracting interest both in chemistry and physics, in the fast-growing field of molecular polaritonics. The large near-field enhancement of the electric field of plasmonic…

Mesoscale and Nanoscale Physics · Physics 2024-10-03 Álvaro Buendía , Jose A. Sánchez-Gil , Vincenzo Giannini , William L. Barnes , Marie S. Rider

The strong coupling of molecules with surface plasmons results in hybrid states which are part molecule, part surface-bound light. Since molecular resonances may acquire the spatial coherence of plasmons, which have mm-scale propagation…

Optics · Physics 2022-05-26 Marie S Rider , Rakesh Arul , Jeremy J Baumberg , William L Barnes

Achieving and controlling strong light-matter interactions in many-body systems is of paramount importance both for fundamental understanding and potential applications. In this paper we demonstrate both experimentally and theoretically how…

Mesoscale and Nanoscale Physics · Physics 2016-12-26 Pierre Fauche , Christian Gebhardt , Maxim Sukharev , Renaud A. L. Vallee

The possibility of strong coupling between a single molecule and surface plasmons is analyzed on the basis of a microscopic classical description. It is predicted that strong single molecule - plasmon coupling can happen for a silver…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Mykhaylo M. Dvoynenko

Strong coupling is a phenomenon which occurs when the interaction between two resonance systems is so strong that the oscillatory energy exchange between them exceeds all dissipative loss channels. Each resonance can then no longer be…

We present a consistent analysis of linear spectroscopy for arrays of nearest neighbor dipole-coupled two-level molecules that reveals distinct signatures of weak and strong coupling regimes separated for infinite size arrays by a quantum…

Quantum Physics · Physics 2015-06-16 A. A. Kocherzhenko , J. Dawlaty , B. P. Abolins , F. Herrera , D. B. Abraham , K. B. Whaley

We study spatial coherence properties of a system composed of periodic silver nanoparticle arrays covered with a fluorescent organic molecule (DiD) film. The evolution of spatial coherence of this composite structure from the weak to the…

When in close contact, plasmonic resonances interact and become strongly correlated. In this work we develop a quantum mechanical model, using the language of continuous variables and quantum information, for an array of coupled particle…

Mesoscale and Nanoscale Physics · Physics 2014-09-09 Javier del Pino , Johannes Feist , F. J. García-Vidal , Juan Jose García-Ripoll

We present a rigorous photonic mode model to describe the strong coupling between a monolayer of $\rm MoSe_2$ and a single gold nanoparticle. The onset of strong coupling is quantified by computing the three-dimensional hybrid quasinormal…

Light-matter interactions can occur when an ensemble of molecular resonators is placed in a confined electromagnetic field. In the strong coupling regime the rapid exchange of energy between the molecules and the electromagnetic field…

Mesoscale and Nanoscale Physics · Physics 2020-08-10 Philip A. Thomas , Wai Jue Tan , Henry A. Fernandez , William L. Barnes

Strong coupling of plasmonic excitations and dipolar emitters, such as organic molecules, have been studied extensively in the last years. The questions whether strong coupling can be achieved with a single molecule only and how this is…

Photonic resonances are a powerful tool for controlling light-matter interactions. However, unlocking many of the most scientifically intriguing and technologically promising phenomena requires entering the strong coupling regime, where…

We study the role of non-Markovian effects in the emission spectrum of a quantum emitter resonantly coupled to a surface plasmon in a metal-dielectric structure as the system transitions to strong coupling regime. By using a recent quantum…

Mesoscale and Nanoscale Physics · Physics 2022-07-08 Tigran V. Shahbazyan

The interaction between excited states of a molecule and excited states of metal nanostructure (e.g. plasmons) leads to hybrid states with modified optical properties. When plasmon resonance is swept through molecular transition frequency…

Chemical Physics · Physics 2022-05-04 Monosij Mondal , Maicol A. Ochoa , Maxim Sukharev , Abraham Nitzan

We demonstrate that a ionising transition can be strongly coupled to a photonic resonance. The strong coupling manifests itself with the appearance of a narrow optically active resonance below the ionisation threshold. Such a resonance is…

We provide a simple method that enables readily acquired experimental data to be used to predict whether or not a candidate molecular material may exhibit strong coupling. Specifically, we explore the relationship between the hybrid…

We simulate the near-field effects of strong coupling between molecular excitons and localized surface plasmons, supported by aluminum nanodisks. The simulations are done using a simple model of a two-level system, implemented in a…

Mesoscale and Nanoscale Physics · Physics 2020-01-29 Nadav Fain , Tal Ellenbogen , Tal Schwartz

We present a quantum theory for the interaction of a two level emitter with surface plasmon polaritons confined in single-mode waveguide resonators. Based on the Green's function approach, we develop the conditions for the weak and strong…

Mesoscale and Nanoscale Physics · Physics 2015-03-20 T. Hümmer , F. J. García-Vidal , L. Martín-Moreno , D. Zueco

Hybrid molecular-plasmonic nanostructures have demonstrated their potential for surface enhanced spectroscopies, sensing or quantum control at the nanoscale. In this work, we investigate the strong coupling regime and explicitly describe…

Quantum Physics · Physics 2017-07-05 H. Varguet , B. Rousseaux , D. Dzsotjan , H. Jauslin , S. Guerin , G. Colas des Francs
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