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We have developed experimental methods for the generation of chirped laser pulses of controlled frequency evolution in the nanosecond pulse length range for coherent atomic interaction studies. The pulses are sliced from the radiation of a…

Intracavity frequency-doubled solid-state lasers exhibit intensity fluctuations of their light output, which are cause by nonlinear dynamical processes. Up to now, there are different solutions to this problem, but they reduce the output…

Statistical Mechanics · Physics 2016-08-31 F. Lange , T. Letz , K. Pyragas , A. Kittel

We report, for the first time, a multi-confocal Fluorescence Correlation Spectroscopy (mFCS) technique which allows parallel measurements at different locations, by combining a Spatial Light Modulator (SLM), with an Electron Multiplying-CCD…

Controlling the carrier envelope phase (CEP) in mode-locked lasers over practically long timescales is crucial for real-world applications in ultrafast optics and precision metrology. We present a hybrid solution that combines a…

Ultra-stable lasers and optical frequency combs have been the enabling technologies for the tremendous progress of precise optical spectroscopy in the last ten years. To improve laser frequency stabilization beyond the thermal-noise…

The advancement of technologies for the precise interrogation of molecules offers exciting possibilities for new studies in the realms of precision spectroscopy and quantum technologies. Experiments in these domains often address molecular…

Optics · Physics 2022-09-15 Mudit Sinhal , Anatoly Johnson , Stefan Willitsch

Harmonic frequency combs, in which the lasing modes are separated by a period of tens of free spectral ranges from each other, have been recently discovered in quantum cascade lasers (QCLs). There is an ongoing debate how the harmonic combs…

Optics · Physics 2020-08-05 Yongrui Wang , Alexey Belyanin

We demonstrate a frequency-stabilized, all-solid laser source at 589 nm with up to 800 mW output power. The laser relies on sum-frequency generation from two laser sources at 1064 nm and 1319 nm through a PPKTP crystal in a doubly-resonant…

We report on a frequency measurement of the $(3s^2)^1S_0\to(3s3p)^3P_1$ clock transition of $^{24}$Mg on a thermal atomic beam. The intercombination transition has been referenced to a portable primary Cs frequency standard with the help of…

Achieving accurate arbitrary frequency excursions with a laser can be quite a technical challenge, especially when steep slopes (GHz/$\mu$s) are required, due to both deterministic and stochastic frequency fluctuations. In this work we…

We have quantified a short term instability budget for an optical frequency standard based on cold, freely expanding calcium atoms. Such systems are the subject of renewed interest due to their high frequency stability and relative…

Atomic Physics · Physics 2011-08-17 J. A. Sherman , C. W. Oates

The use of averaging has long been known to reduce noise in statistically independent systems that exhibit similar levels of stochastic fluctuation. This concept of averaging is general and applies to a wide variety of physical and man-made…

Fourier transform spectroscopy (FTS) has been widely used as an analytical tool for many applications in science and engineering. In this paper, we describe the operation principle and practical implementation of an FTS prototype. First,…

Instrumentation and Detectors · Physics 2023-02-02 Sohrab Sheikh-Sofla , Mohammad Neshat

Triple sum-frequency (TSF) spectroscopy is a recently-developed methodology that enables collection of multidimensional spectra by resonantly exciting multiple quantum coherences of vibrational and electronic states. This work reports the…

Optics · Physics 2018-08-23 Darien J. Morrow , Daniel D. Kohler , Kyle J. Czech , John C. Wright

Long-distance measurements (10 m - 1000 m) with an accuracy of 10-7 is a challenge for many applications. We show that it is achievable with Frequency Shifted Feedback (FSF) laser interferometry technique, provided that the determination of…

Optics · Physics 2015-06-05 Jean-Paul Pique

We present a computer-based active interferometer stabilization method that can be set to an arbitrary phase difference and does not rely on modulation of the interfering beams. The scheme utilizes two orthogonal modes propagating through…

We stabilized the frequencies of two independent Nd:YAG lasers to two adjacent longitudinal modes of a high-finesse Fabry-P\'erot resonator and obtained a beat frequency instability of 6.3 mHz at an integration time of 40 s. Referred to a…

Optics · Physics 2012-12-19 Qun-Feng Chen , Alexander Nevsky , Stephan Schiller

Laser decoherence limits the stability of optical clocks by broadening the observable resonance linewidths and adding noise during the dead time between clock probes. Correlation spectroscopy avoids these limitations by measuring correlated…

We present frequency-matched strobo-spectroscopy (FMSS) of charge migration (CM) in bromobutadiyne, simulated with time-dependent density-functional theory. CM+FMSS is a pump-probe scheme that uses a frequency-matched HHG-driving laser as…

Quantum Cascade Lasers (QCL) are increasingly being used to probe the mid-infrared "molecular fingerprint" region. This prompted efforts towards improving their spectral performance, in order to reach ever-higher resolution and precision.…